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Optics Communications

A semiclassical approach for two-color four-mode solid-state superfluorescence

Carlos L. Pando Lambruschini

Published Sep 1, 1991• 2 citations
Publisher
DOI
10.1016/0030-4018(91)90410-f

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Single crystals of KCl containing $\mathrm{O}_{2}^{}{}_{}{}^{\ensuremath{-}}$ centers (8\ifmmode\times\else\texttimes\fi{}${10}^{16}$-7\ifmmode\times\else\texttimes\fi{}${10}^{17}$ ${\mathrm{cm}}^{\ensuremath{-}3}$) were excited at low temperatures ($T<30$ K) using frequency-quadrupled single pulses of a mode-locked Nd-doped yttrium aluminum garnet laser. At excitation intensities above 20 GW/${\mathrm{cm}}^{2}$ a spontaneous emission of coherent light was observed which could be identified as Dicke superfluorescence. This superfluorescence was observed on two of the zero-phonon lines in the vibrational progression of the $\mathrm{O}_{2}^{}{}_{}{}^{\ensuremath{-}}$ fluorescence spectrum (0-10 and 0-11 at 592.8 and 629.1 nm, respectively). We have studied the time dependence, the statistics of the delay times, and the intensities. The observed delay times vary between 0.5 and 10 ns, the observed pulse widths between 0.5 and 6 ns, and the coherence time was found to be longer than 100 ps. The observed linewidths of the superfluorescence ($0.016\mathrm{nm}\ensuremath{\cong}14\mathrm{GHz}$) is a factor of 2.5 smaller than that of the spontaneous fluorescence (0.042 nm at 4.2 K). The superfluorescence is observed only below a critical temperature which depends on the $\mathrm{O}_{2}^{}{}_{}{}^{\ensuremath{-}}$ concentration (8 to 28 K for concentrations between 8\ifmmode\times\else\texttimes\fi{}${10}^{16}$ and 7\ifmmode\times\else\texttimes\fi{}${10}^{17}$ ${\mathrm{cm}}^{\ensuremath{-}3}$).

Physical Review A•May 1, 1984•144 citations
The simulation of superfluorescence of a thin layer of two-level atoms was performed on the basis of semiclassical approach without using approximation of slowly varying in space amplitudes of electric field and medium polarization (paraxial approximation). The evolution of atomic characteristics and the structure of the radiation directivity pattern inside the total solid angle have been investigated. The comparison of the results obtained with the results based on the paraxial approximation has been done.
Single crystals of KCl containing $\mathrm{O}_{2}^{}{}_{}{}^{\ensuremath{-}}$ centers (8\ifmmode\times\else\texttimes\fi{}1016{10}^{16}1016-7\ifmmode\times\else\texttimes\fi{}1017{10}^{17}1017 ${\mathrm{cm}}^{\ensuremath{-}3}$) were excited at low temperatures (T<30T<30T<30 K) using frequency-quadrupled single pulses of a mode-locked Nd-doped yttrium aluminum garnet laser. At excitation intensities above 20 GW/cm2{\mathrm{cm}}^{2}cm2 a spontaneous emission of coherent light was observed which could be identified as Dicke superfluorescence. This superfluorescence was observed on two of the zero-phonon lines in the vibrational progression of the $\mathrm{O}_{2}^{}{}_{}{}^{\ensuremath{-}}$ fluorescence spectrum (0-10 and 0-11 at 592.8 and 629.1 nm, respectively). We have studied the time dependence, the statistics of the delay times, and the intensities. The observed delay times vary between 0.5 and 10 ns, the observed pulse widths between 0.5 and 6 ns, and the coherence time was found to be longer than 100 ps. The observed linewidths of the superfluorescence ($0.016\mathrm{nm}\ensuremath{\cong}14\mathrm{GHz}$) is a factor of 2.5 smaller than that of the spontaneous fluorescence (0.042 nm at 4.2 K). The superfluorescence is observed only below a critical temperature which depends on the $\mathrm{O}_{2}^{}{}_{}{}^{\ensuremath{-}}$ concentration (8 to 28 K for concentrations between 8\ifmmode\times\else\texttimes\fi{}1016{10}^{16}1016 and 7\ifmmode\times\else\texttimes\fi{}1017{10}^{17}1017 ${\mathrm{cm}}^{\ensuremath{-}3}$).