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IEEE Journal of Quantum Electronics

Constraints on coherent control of quantum-well excitons for high-speed all-optical switching

David S. Citrin, Theodore B. Norris

Published Mar 1, 1997• 17 citations
Publisher

Abstract

Coherent control of excitons in quantum wells at high repetition rates is investigated theoretically to determine the practical constraints for application in high-bit-rate optical switching. A tradeoff between optical pathlength (number of quantum wells) and excitation density is found that severely limits the applicability of this mechanism for implementation in 100-Gb/s optical systems.

DOI
10.1109/3.556009

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Journal of the Optical Society of America B•Jun 1, 1996•41 citations
Coherent control of excitons in quantum wells at high repetition rates is investigated theoretically to determine the practical constraints for application in high-bit-rate optical switching. A tradeoff between optical pathlength (number of quantum wells) and excitation density is found that severely limits the applicability of this mechanism for implementation in 100-Gb/s optical systems.
We have carried out an extensive series of experiments on coherent control of semiconductor quantum microcavities. In these experiments, a phase-locked femtosecond optical pulse pair is used to excite the lower normal mode (cavity polariton), thereby controlling the reflection of a signal pulse tuned to the upper normal mode. Such a controlled reflection may be used as an all-optical switch with picosecond switching time. We have demonstrated that the effect of the microcavity is to provide a huge enhancement of the coherently controlled response compared to bare quantum wells. We have investigated in detail the microscopic physical processes responsible for the nonlinear optical response; the measured response fits well with theories based on the electron-hole Hamiltonian in the coherent-X(5) and 2nd-Born approximations. The physical limits to the coherent control are determined by excitation-induced dephasing; this limits the applicability of the switch in practical terms. We have discovered that the use of phase-locked excitation pulses is that one can generate novel intraband coherences in the quantum wells, arising from true quantum correlations between the cavity field and the carrier populations. The discovery of this effect was perhaps the first genuinely quantum optical effect observed in semiconductor microcavities.
Summary form only given. The optical coherent control of quantum mechanical systems enables the direct manipulation of quantum states, and has been demonstrated on excitonic transitions in semiconductors. We have demonstrated the coherent control of the nonlinear optical response of quantum-well excitons in a resonant high-Q microcavity. There are two significant advantages to using excitons in microcavities instead of bare quantum wells: first, the multiple reflections which occur in the cavity strongly enhance the optical nonlinearity, enabling large-signal coherent control, and second, 2-color coherent control may be implemented, where a pump pulse tuned to one of the normal modes of the coupled exciton-microcavity system can control the response of a probe tuned to the other normal mode. The nonlinear response of the normal modes is due to the nonlinearity of the underlying exciton transition.
The dynamics of the coherent superposition of exciton states in a semiconductor quantum well excited by the joint action of two successive light pulses with the time interval between them t 12 has been theoretically studied. The dependences of the amplitude and initial phase of the quantum bits on t 12 have been found. It has been shown that the time dependence of the Kerr rotation of the reflected probe pulse is determined not only by the dynamics of the excited state, but also by the optical properties of the heterostructure containing the quantum well. The dependence of the decay rate of the excited state on t 12 has been predicted.
Electron-spin relaxation has been investigated in a variety of quantum confined structures including GaAs-based quantum wells and quantum wires as well as InP-based quantum wells, and it has been shown to exhibit ultrafast relaxation in the picosecond, and even in the femtosecond, range. This ultrafast relaxation has been used together with the exciton absorption nonlinearity as an novel principle of all-optical switching device which can avoid the speed limit due to the slow carrier lifetime in conventional switching devices. Experiments on GaAs-based quantum-well spin switches have shown 4-ps gate switch operation. Also, experimental analyses have shown the feasibility of these devices at a high contrast ratio (13 dB) and high repetition rate (40 GHz). The application of this device to a demultiplexer has been proposed.
We report the coherent control of excitons in quantum wells with pairs of 150-fs infrared pulses. Oscillations in the exciton density versus inter-pump-pulse separation, which correspond to the resonant transition energy, yield new insight into coherent exciton dynamics when their phase is analyzed. We demonstrate that these oscillations are caused when the second laser pulse destroys or enhances excitons that were created by the first pulse. The coherent carrier destruction generates ultrafast exciton dynamics that are not limited by the linewidth of the optical transition.