Fluorescence and absorption spectra of the Lambda-system in the case of Raman resonance

Lorenzo M. Narducci, D.H. Feng, G. S. Agarwal +1 more

Arza Ron, Amiram Ron

Igor Bargatin, B. A. Grishanin, Victor N. Zadkov

Our investigation is focused on obtaining analytical results describing the resonance fluorescence and weak probe absorption spectra of a driver Lambda-system under the Raman resonance condition. For the saturation field limit and within the rotating wave approximation (RWA) the resonance fluorescence and weak probe absorption spectra are calculated for the case of unequal driving fields strengths and non-zero one-photon detunings, generalizing the previously known results. A novel contribution derived is the nonpositive nonlorentzian part of the spectrum, originating from the specific quantum properties of the atomic correlation functions. This contribution is asymptotically small under given conditions and, therefore, determines behavior of the resonance fluorescence spectrum wings and the absorption spectrum in the vicinities of the driving field frequencies. Beyond the RWA, the spectral structures due to the off-resonant four-photon atomic excitations are calculated. They consist of a coherent and two broadened spectral lines centered at the four-photon frequencies 2(omega) L-(omega) 1L and 2(omega) +1)/ - (omega) L4/ respectively, where (omega l and (omega) (superscript 1$L are the driving laser frequencies.

Heide Doss, A. Manka, P. Ru +3 more

The coherent coupling of atomic levels under the action of driving electromagnetic fields is known to create unusual and interesting effects, such as the well-known population trapping phenomenon and subnatural line narrowing. In this paper we discuss two alternative configurations of three-level atoms, the cascade model and the inverted-V (lambda) model, in an effort to provide alternative options for experimental tests. In both cases we focus on the fluorescent emission spectrum of atom driven by two resonant fields and on the absorption spectrum of a weak probe passing through a gas in such a driven system. Subnatural line narrowing can be obtained from the cascade system but not from the lambda system. The lambda system, however, is characterized by strong population trapping so that it is not suitable for fluorescence studies (except out of resonance) because of its strongly reduced emission rate. The absorption spectrum of a weak probe displays gain features under high field conditions which suggest that useful amplification of a probe or laser-like emission should be possible over appropriate frequency ranges. We give a physical interpretation of the origin of the gain and explain why that in the case of a lambda system, but not a cascade system, steady-state population inversion can be obtained between both excited states relative to the lowest state of the atom. We also discuss the effect of Doppler broadening on the predicted emission and absorption lineshapes.

PAUCHANON DAS

Robin M. Hochstrasser, Frank A. Novak