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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Coherent strong-field coupling of a ferromagnetic nanomagnet with a photonic cavity

Öney O. Soykal, Michael E. Flatté

Published Aug 17, 2010• 2 citations
Publisher

Abstract

We predict that strong coupling is feasible between photons and a ferromagnetic nanomagnet, due to exchange interactions that cause very large numbers of spins to coherently lock together with a significant increase in oscillator strength while still maintaining very long coherence times. The interaction of a ferromagnetic nanomagnet with a single photonic mode of a cavity is analyzed in a fully quantum-mechanical treatment. Exceptionally large quantum-coherent magnet-photon coupling with coupling terms in excess of several THz are predicted to be achievable in a spherical cavity of ~ 1 mm radius with a nanomagnet of ~ 100 nm radius and ferromagnet resonance frequency of ~ 200 GHz. This should substantially exceed the coupling observed in solids between orbital transitions and light. Eigenstates of the nanomagnet-photon system correspond to entangled states of spin orientation and photon number over 105 values of each quantum number. Initial coherent state of definite spin and photon number evolve dynamically to produce large coherent oscillations in the microwave power with exceptionally long dephasing times of few seconds. In addition to dephasing, several decoherence mechanisms including elementary excitation of magnons and crystalline magnetic anisotropy are investigated and shown to not substantially affect coherence upto room temperature. The optimal nanomagnet size is predicted to be just below the threshold for failure of the macrospin approximation.

DOI
10.1117/12.860725

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We predict that strong coupling is feasible between photons and a ferromagnetic nanomagnet, due to exchange interactions that cause very large numbers of spins to coherently lock together with a significant increase in oscillator strength while still maintaining very long coherence times. The interaction of a ferromagnetic nanomagnet with a single photonic mode of a cavity is analyzed in a fully quantum-mechanical treatment. Exceptionally large quantum-coherent magnet-photon coupling with coupling terms in excess of several THz are predicted to be achievable in a spherical cavity of ~ 1 mm radius with a nanomagnet of ~ 100 nm radius and ferromagnet resonance frequency of ~ 200 GHz. This should substantially exceed the coupling observed in solids between orbital transitions and light. Eigenstates of the nanomagnet-photon system correspond to entangled states of spin orientation and photon number over 105 values of each quantum number. Initial coherent state of definite spin and photon number evolve dynamically to produce large coherent oscillations in the microwave power with exceptionally long dephasing times of few seconds. In addition to dephasing, several decoherence mechanisms including elementary excitation of magnons and crystalline magnetic anisotropy are investigated and shown to not substantially affect coherence upto room temperature. The optimal nanomagnet size is predicted to be just below the threshold for failure of the macrospin approximation.
Strong coupling of light and matter is an essential element of cavity quantum electrodynamics (cavity-QED) and quantum optics, which may lead to novel mixed states of light and matter and to applications such as quantum computation. In the strong-coupling regime, where the coupling strength exceeds the dissipation, the light-matter interaction produces a characteristic vacuum Rabi splitting. Therefore, strong coupling can be utilized as an effective coherent interface between light and matter (in the form of electron charge, spin or superconducting Cooper pairs) to achieve components of quantum information technology including quantum memory, teleportation, and quantum repeaters. Semiconductor quantum dots, nuclear spins and paramagnetic spin systems are only some of the material systems under investigation for strong coupling in solid-state physics. Mixed states of light and matter coupled via electric dipole transitions often suffer from short coherence times (nanoseconds). Even though magnetic transitions appear to be intrinsically more quantum coherent than orbital transitions, their typical coupling strengths have been estimated to be much smaller. Hence, they have been neglected for the purposes of quantum information technology.\nHowever, we predict that strong coupling is feasible between photons and a ferromagnetic nanomagnet, due to exchange interactions that cause very large numbers of spins to coherently lock together with a significant increase in oscillator strength while still maintaining very long coherence times. In order to examine this new exciting possibility, the interaction of a ferromagnetic nanomagnet with a single photonic mode of a cavity is analyzed in a fully quantum-mechanical treatment. Exceptionally large quantum-coherent magnet-photon coupling with coupling terms in excess of several THz are predicted to be achievable in a spherical cavity of ∼ 1 mm radius with a nanomagnet of ∼ 100 nm radius and ferromagnet resonance frequency of ∼ 200 GHz. This should substantially exceed the coupling observed in solids between orbital transitions and light. Eigenstates of the nanomagnet-photon system correspond to entangled states of spin orientation and photon number over 105 values of each quantum number. Initial coherent state of definite spin and photon number evolve dynamically to produce large coherent oscillations in the microwave power with exceptionally long dephasing times of few seconds. In addition to dephasing, several decoherence mechanisms including elementary excitation of magnons and crystalline magnetic anisotropy are investigated and shown to not substantially affect coherence upto room temperature. For small nanomagnets the crystalline magnetic anisotropy of the magnet strongly localize the eigenstates in photon and spin number, quenching the potential for coherent states and for a sufficiently large nanomagnet the macrospin approximation breaks down and different domains of the nanomagnet may couple separately to the photonic mode. Thus the optimal nanomagnet size is predicted to be just below the threshold for failure of the macrospin approximation. Moreover, it is shown that initially unentangled coherent states of light (cavity field) and spin (nanomagnet spin orientation) can be phase-locked to evolve into a coherent entangled states of the system under the influence of strong coupling.
We analyze the interaction of a nanomagnet (ferromagnetic) with a single photonic mode of a cavity in a fully quantum-mechanical treatment and find that exceptionally large quantum-coherent magnet-photon coupling can be achieved. Coupling terms in excess of several THz are predicted to be achievable in a spherical cavity of approximately 1 mm radius with a nanomagnet of approximately 100 nm radius and ferromagnetic resonance frequency of approximately 200 GHz. Eigenstates of the magnet-photon system correspond to entangled states of spin orientation and photon number, in which over 10{5} values of each quantum number are represented; conversely, initial (coherent) states of definite spin and photon number evolve dynamically to produce large oscillations in the microwave power (and nanomagnet spin orientation), and are characterized by exceptionally long dephasing times.
The coherent dynamics of a coupled photonic cavity and a nanomagnet is explored as a function of nanomagnet size. For sufficiently strong coupling eigenstates involving highly entangled photon and spin states are found, which can be combined to create coherent states. As the size of the nanomagnet increases its coupling to the photonic mode also monotonically increases, as well as the number of photon and spin states involved in the system's eigenstates. For small nanomagnets the crystalline anisotropy of the magnet strongly localizes the eigenstates in photon and spin number, quenching the potential for coherent states. For a sufficiently large nanomagnet the macrospin approximation breaks down and different domains of the nanomagnet may couple separately to the photonic mode. Thus the optimal nanomagnet size is just below the threshold for failure of the macrospin approximation.
Coupled microwave photon-magnon hybrid systems offer promising applications by harnessing various magnon physics. At present, in order to realize high coupling strength between the two subsystems, bulky ferromagnets with large spin numbers are utilized, which limits their potential applications for scalable quantum information processing. By enhancing single spin coupling strength using lithographically defined superconducting resonators, we report high cooperativities between a resonator mode and a Kittel mode in nanometer thick Permalloy wires. The on-chip, lithographically scalable, and superconducting quantum circuit compatible design provides a direct route towards realizing hybrid quantum systems with nanomagnets, whose coupling strength can be precisely engineered and dynamic properties can be controlled by various mechanisms derived from spintronic studies.
Rigidity of an ordered phase in condensed matter results in collective excitation modes spatially extending in macroscopic dimensions. Magnon is a quantum of an elementary excitation in the ordered spin system, such as ferromagnet. Being low dissipative, dynamics of magnons in ferromagnetic insulators has been extensively studied and widely applied for decades in the contexts of ferromagnetic resonance, and more recently of Bose-Einstein condensation as well as spintronics. Moreover, towards hybrid systems for quantum memories and transducers, coupling of magnons and microwave photons in a resonator have been investigated. However, quantum-state manipulation at the single-magnon level has remained elusive because of the lack of anharmonic element in the system. Here we demonstrate coherent coupling between a magnon excitation in a millimetre-sized ferromagnetic sphere and a superconducting qubit, where the interaction is mediated by the virtual photon excitation in a microwave cavity. We obtain the coupling strength far exceeding the damping rates, thus bringing the hybrid system into the strong coupling regime. Furthermore, we find a tunable magnon-qubit coupling scheme utilising a parametric drive with a microwave. Our approach provides a versatile tool for quantum control and measurement of the magnon excitations and thus opens a new discipline of quantum magnonics.
Coherent conversion of microwave and optical photons in the single quantum level can significantly expand our ability to process signals in various fields. Efficient up-conversion of a feeble signal in the microwave domain to the optical domain will lead to quantum-noise-limited microwave amplifiers. Coherent exchange between optical photons and microwave photons will also be a stepping stone to realize long-distance quantum communication. Here we demonstrate bidirectional and coherent conversion between microwave and light using collective spin excitations in a ferromagnet. The converter consists of two harmonic oscillator modes, a microwave cavity mode and a magnetostatic mode called the Kittel mode, where microwave photons and magnons in the respective modes are strongly coupled and hybridized. An itinerant microwave field and a traveling optical field can be coupled through the hybrid system, where the microwave field is coupled to the hybrid system through the cavity mode, while the optical field addresses the hybrid system through the Kittel mode via Faraday and inverse Faraday effects. The conversion efficiency is theoretically analyzed and experimentally evaluated. The possible schemes for improving the efficiency are also discussed.