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Journal of Luminescence

Nonlinear dynamics of spin-boson systems: Quantum mechanical and quasi-classical treatment

R. Steib, J. L. Schoendorff, H. J. Korsch, P. Reineker

Published Feb 1, 1998• 2 citations
Publisher
DOI
10.1016/s0022-2313(97)00256-1

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We consider the hybrid system-bath dynamics, based on the Yan's dissipaton formalism [Y. J. Yan, J. Chem. Phys. 140, 054105 (2014)]. This theory provides a unified quasi-particle treatment on three distinct classes of quantum bath, coupled nonperturbatively to arbitrary quantum systems. In this work, to study the entangled system and bath polarization and nonlinear Fano interference, we incorporate further the time-dependent light field, which interacts with both the molecular system and the collective bath dipoles directly. Numerical demonstrations are carried out on a two-level system, with comparison between phonon and exciton baths, in both linear and nonlinear Fano interference regimes.
We consider the spin-boson model as a measurement device, with the 1/2-spin system acting as a pointer and the influence of the environment simulated by means of the interaction between the 1/2-spin system and a dissipative oscillator. In accordance with the recent finding of Bonilla and Guinea [L. L. Bonilla and F. Guinea, Phys. Rev. A 45, 7718 (1992)] the assumption that the oscillator is classical results, under specific conditions, in the occurrence of a wave-function collapse. However, our theoretical analysis shows that the wave-function collapse is provoked by the action exerted by the 1/2-spin system on the oscillator (reaction field) and that the reaction field is as intense as the quantum-mechanical fluctuation neglected by the semiclassical approximation. A numerical treatment shows that no collapse occurs within a fully-quantum-mechanical treatment.