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Theory of cold dipolar and toroidal gases

D. Baillie

Published Jan 1, 2012• 0 citations
OpenAlex

Abstract

We develop and apply meanfield methods to two systems of significant interest in cold atom physics. The first system, and the main subject of this thesis, is a gas of polarized dipoles, in which the particles have a long range anisotropic interaction. The second system is a toroidally trapped gas that interacts via short range interactions. \n \nDipolar gases: We develop accurate techniques for dipolar Bose and Fermi gases accounting for both direct and exchange interactions. We detail an efficient numerical implementation of the meanfield treatment. \n \nWe study the thermodynamic and the first and second order correlation properties of the system. We find that exchange interactions cause the correlation functions to be anisotropic in the low temperature regime. We also find that many uniform gas thermodynamic predictions, for which direct interaction effects vanish, are qualitatively unreliable for trapped systems, most notably for oblate traps. \n \nUsing Hartree-Fock theory and analytic approximations, we examine the magnetostrictive position and momentum space distortions that occur in harmonically confined dipolar Bose and Fermi gases. The Bose gas momentum distribution distorts in the opposite sense to that of the Fermi gas. By relating exchange effects to short range correlations between the particles we discuss the energetic origin of this difference. \n \nIntroducing local momentum distortion fields, we develop a practical Hartree-Fock theory in which exchange effects are described by a local effective potential. This theory is applicable at zero and finite temperature, and is in excellent agreement with full Hartree-Fock calculations. \n \nContact gases: We show how considerable simplification of numerical results and analytical derivations can be achieved in the local density approximation using a variety of density of states techniques. \n \nWe examine the process of isentropic loading of a Bose or Fermi gas from a harmonic trap into the scale invariant toroidal regime that exhibits a high degree of system invariance when increasing the radius of the toroid. For bosons a regime of cooling is identified and we find that the Fermi gas is subjected to irreducible heating during loading, caused by the loss of one degree of freedom for thermalization.

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We develop and apply meanfield methods to two systems of significant interest in cold atom physics. The first system, and the main subject of this thesis, is a gas of polarized dipoles, in which the particles have a long range anisotropic interaction. The second system is a toroidally trapped gas that interacts via short range interactions. \n \nDipolar gases: We develop accurate techniques for dipolar Bose and Fermi gases accounting for both direct and exchange interactions. We detail an efficient numerical implementation of the meanfield treatment. \n \nWe study the thermodynamic and the first and second order correlation properties of the system. We find that exchange interactions cause the correlation functions to be anisotropic in the low temperature regime. We also find that many uniform gas thermodynamic predictions, for which direct interaction effects vanish, are qualitatively unreliable for trapped systems, most notably for oblate traps. \n \nUsing Hartree-Fock theory and analytic approximations, we examine the magnetostrictive position and momentum space distortions that occur in harmonically confined dipolar Bose and Fermi gases. The Bose gas momentum distribution distorts in the opposite sense to that of the Fermi gas. By relating exchange effects to short range correlations between the particles we discuss the energetic origin of this difference. \n \nIntroducing local momentum distortion fields, we develop a practical Hartree-Fock theory in which exchange effects are described by a local effective potential. This theory is applicable at zero and finite temperature, and is in excellent agreement with full Hartree-Fock calculations. \n \nContact gases: We show how considerable simplification of numerical results and analytical derivations can be achieved in the local density approximation using a variety of density of states techniques. \n \nWe examine the process of isentropic loading of a Bose or Fermi gas from a harmonic trap into the scale invariant toroidal regime that exhibits a high degree of system invariance when increasing the radius of the toroid. For bosons a regime of cooling is identified and we find that the Fermi gas is subjected to irreducible heating during loading, caused by the loss of one degree of freedom for thermalization.
The work of this thesis concerns the properties of a Bose gas of polarised dipoles that have long-range and anisotropic interactions. Our work is divided into two parts. First, the stability of a dipolar Bose gas at finite temperature (both above and below the critical Bose-Einstein condensation (BEC) temperature Tc). Second, the fluctuations of a dipolar BEC at zero and small finite temperature (T ≪ Tc) in a regime where rotonic excitations emerge. \n \nPart I: Stability of a Trapped Finite Temperature Dipolar Bose Gas: Above Tc we implement a semiclassical Hartree-Fock theory and characterise the dependence of the stability boundary on temperature, trap geometry and the strength of the dipole-dipole interaction and contact interaction. We find that stability is greatly enhanced above Tc and that trap geometry continues to play a key role. Furthermore, we find that for oblate traps a novel double instability feature emerges. \nTo extend our stability analysis to the low temperature regime, T < Tc, we develop a beyond semiclassical Hartree theory. We use this to characterise the stability boundary as a function of geometry. Interestingly, we find large beyond semiclassical effects above Tc for prolate trapping geometries. We characterise thermal effects on biconcave condensate states. \n \nPart II: Rotons and Fluctuations in a Trapped Dipolar Condensate: To study density fluctuations we implement a numerical scheme to solve the Gross-Pitaevskii equation and the Bogoliubov de Gennes equations. We find that the phonon and roton gases spatially separate and we characterise the role of the anomalous density on the density fluctuations of the thermally activated rotons. We develop a numerical scheme that calculates number fluctuations within cells of various shapes and sizes, and find a strong peak in the fluctuations when the cell size is around half the roton wavelength, which should be detectable by current experiments. By tailoring the cell shape we predict that experiments should be able to detect the effects of individual roton modes. \nFor the study of zero temperature fluctuations we deploy the Gross-Pitaevskii and Bogoliubov de Gennes equations to calculate the dynamic and static structure factors for a highly oblate BEC. We find a clear signature of the roton gas dispersion relation within the structure factors. This signature should be detectible in current experiments using Bragg spectroscopy.
We develop a mean-field treatment of a polarized trapped Fermi gas with dipole-dipole interactions. Our approach is based on self-consistent semiclassical Hartree-Fock theory that accounts for direct and exchange interactions. We discuss our procedure for numerically implementing the calculation. We study the thermodynamic and the first- and second-order correlation properties of the system. We find that the system entropy depends on the trap geometry, allowing the system to be cooled as the trap aspect ratio is increased, and that exchange interactions cause the correlation functions to be anisotropic in the low-temperature regime. We also find that many uniform gas thermodynamic predictions, for which direct interaction effects vanish, are qualitatively unreliable for trapped systems, most notably for oblate traps. We develop a simplified Hartree formalism that is applicable to anisotropic harmonic traps.
We examine the magnetostrictive position and momentum space distortions that occur in harmonically confined dipolar Bose and Fermi gases. Direct interactions give rise to position space magnetostriction and exchange interactions give rise to momentum space magnetostriction. While the position space magnetostriction is similar in Bose and Fermi systems, the momentum space magnetostriction is markedly different: The Bose gas momentum distribution distorts in the opposite sense to that of the Fermi gas. By relating exchange effects to short-range correlations between the particles we discuss the energetic origin of this difference. Our main calculations are based on Hartree-Fock theory, but we also provide analytic approximations for the magnetostriction effects at zero and finite temperature. Our predictions should be verifiable in current experiments with ultracold polar molecules.
In this thesis we study the effects of the dipole-dipole interaction on the physics of ultracold quantum gases, both bosonic and fermionic, within the theoretical framework provided by the mean-field regime. This kind of interaction takes place in ultracold atomic gases (for instance 52Cr or 164Dy) due to their atomic magnetic dipole moment, and in ultracold molecular gases due to the magnetic or electric dipole moment. \n \nIn the case of quantum gases of bosonic atoms, or Bose-Einstein condensates, the dipole-dipole interaction can be studied within mean-field approximation using the Gross-Pitaevskii equation, which now contains a new non-linear term due to the dipole-dipole interaction. We investigate, on the one hand dipolar condensates confined in harmonic traps, and on the other dipolar condensates confined in toroidal traps. In the harmonic geometry, our focus is on the study of the ground state and the quantized vortex state, where the density profile is characterized as well as some properties leading to the process of vortex formation, such as the critical frequency and the energy barrier that has to be overcome to bring the vortex from the surface to the centre of the gas. We finish the study of dipolar condensates in harmonic traps by dynamically simulating the precession frequency of an off-center vortex in a non-rotating condensate. \n \nIn the toroidal geometry the dipolar effects are strongly magnified when the polarization axis of the dipoles is perpendicular to the trap symmetry axis. In this case, the anisotropic structure of the density can be understood as the response of the system to the double-well effective potential along the ring. We have studied the dynamics of this system when the initial number of atoms in the left and right wells is imbalanced, predicting Josephson and self-trapping oscillations depending on the initial condition. This has led us to name this new system as Self-induced Josephson Junction. We have studied in detail the self-trapping regime and we have seen that the particle flux inversion is closely related to the crossing of vortices across the Josephson junctions. This result opens the door to establishing a more direct connection between the phase-slip regime, widely addressed in superfluid helium, and the self-trapping regime of condensates. \n \nIn the case of quantum gases of fermionic dipolar particles, we have studied how the radial quadrupole mode allows one to distinguish between hydrodynamic and collisionless regimes. We have analytically calculated the frequency of this mode in the mean-field approximation, generalizing the results from the Thomas-Fermi approximation for trapped ideal Fermi gases. On the one hand, we observe that the frequency in the hydrodynamic regime is smaller than in non-dipolar Fermi gases, while in the collisionless regime the frequency is larger or smaller than that corresponding to the non-interacting system depending on the geometry of the harmonic trap. On the other hand, we predict that reducing the trap deformation (aspect ratio) an observable jump in the frequency of the radial quadrupole mode would take place, which would correspond to the transition between the collisionless and hydrodynamic regimes, for instance when the gas undergoes the transition to the superfluid state.
The quest for quantum degenerate Fermi gases interacting through the anisotropic and long-range dipole-dipole interaction is an exciting and fast developing branch within the cold-atom research program. Recent experimental progress in trapping, cooling, and controlling polar molecules with large electric dipole moments has, therefore, motivated much theoretical effort. In a recent letter, we have briefly discussed the application of a variational time-dependent Hartree-Fock approach to study theoretically both the static and the dynamic properties of such a system in a cylinder-symmetric harmonic trap. We focused on the hydrodynamic regime, where collisions ensure the equilibrium locally. Here we present a detailed theory extended to encompass the general case of a harmonic trap geometry without any symmetry. After deriving the equations of motion for the gas, we explore their static solutions to investigate key properties like the aspect ratios in both real and momentum space as well as the stability diagram. We find that, despite the lack of symmetry of the trap, the momentum distribution remains cylinder symmetric. The equations of motion are then used to study the low-lying hydrodynamic excitations, where, apart from the quadrupole and monopole modes, the radial quadrupole mode is also investigated. Furthermore, we study the time-of-flight dynamics as it represents an important diagnostic tool for quantum gases. We find that the real-space aspect ratios are inverted during the expansion, while that in momentum space becomes asymptotically unity. In addition, anisotropic features of the dipole-dipole interaction are discussed in detail. These results could be particularly useful for future investigations of strongly dipolar heteronuclear polar molecules deep in the quantum degenerate regime.