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Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC)

Evidence of macroscopic coherence at room temperature: Rabi oscillation induced pulse break-up in a quantum dot amplifier

Mirco Kolarczik, Nina Owschimikow, Yücel Kaptan, U. Woggon, Julian Korn, Benjamin Lingnau, Eckehard Schöll, Kathy Lüdge

Published May 1, 2013• 1 citation
Publisher

Abstract

We study experimentally and numerically the changes in pulse shape a Gaussian laser pulse undergoes when propagating through an electrically pumped quantum dot semiconductor optical amplifier (QD-SOA). The pulse energy is set to be resonant to the quantum dot ground state transition, and the pulse shape is analyzed in phase and amplitude in a heterodyne cross-correlation experiment. For the case of an inverted system, we observe the appearance of a periodic modulation of the temporal pulse profile above a critical pulse power. Similar signatures of pulse break-up have been observed at low temperature in quantum dot ensembles without electrical pumping and were linked to optically induced Rabi oscillations imprinting the coherent switching between absorption and stimulated emission of photons by the material system.

DOI
10.1109/cleoe-iqec.2013.6801879

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We study experimentally and numerically the changes in pulse shape a Gaussian laser pulse undergoes when propagating through an electrically pumped quantum dot semiconductor optical amplifier (QD-SOA). The pulse energy is set to be resonant to the quantum dot ground state transition, and the pulse shape is analyzed in phase and amplitude in a heterodyne cross-correlation experiment. For the case of an inverted system, we observe the appearance of a periodic modulation of the temporal pulse profile above a critical pulse power. Similar signatures of pulse break-up have been observed at low temperature in quantum dot ensembles without electrical pumping and were linked to optically induced Rabi oscillations imprinting the coherent switching between absorption and stimulated emission of photons by the material system.
We demonstrate the ability to control quantum coherent Rabi-oscillations in a room-temperature quantum dot semiconductor optical amplifier (SOA) by shaping the light pulses that trigger them. The experiments described here show that when the excitation is resonant with the short wavelength slope of the SOA gain spectrum, a linear frequency chirp affects its ability to trigger Rabi-oscillations within the SOA: A negative chirp inhibits Rabi-oscillations whereas a positive chirp can enhance them, relative to the interaction of a transform limited pulse. The experiments are confirmed by a numerical calculation that models the propagation of the experimentally shaped pulses through the SOA.
Coherence in light–matter interaction is a necessary ingredient if light is used to control the quantum state of a material system. Coherent effects are firmly associated with isolated systems kept at low temperature. The exceedingly fast dephasing in condensed matter environments, in particular at elevated temperatures, may well erase all coherent information in the material at timescales shorter than a laser excitation pulse. Here we show for an ensemble of semiconductor quantum dots that even in the presence of ultrafast dephasing, for suitably designed condensed matter systems quantum-coherent effects are robust enough to be observable at room temperature. Our conclusions are based on an analysis of the reshaping an ultrafast laser pulse undergoes on propagation through a semiconductor quantum dot amplifier. We show that this pulse modification contains the signature of coherent light–matter interaction and can be controlled by adjusting the population of the quantum dots via electrical injection. Quantum coherence effects are often only visible at low temperatures, where dephasing times are not too short. Here Kolarczik et al. show that quantum coherence effects can appear in the reshaping of ultrafast laser pulses passing through quantum dots even at room temperature.
We present a numerical study of coherent control in a room temperature InAs/InP quantum dot (QD) semiconductor optical amplifier (SOA) using shaped ultra-short pulses. Both the gain and absorption regimes were analyzed for pulses with central wavelengths lying on either side of the inhomogeneously broadened gain spectrum. The numerical experiments predict that in the gain regime the coherent interactions between a QD SOA and a pulse can be controlled by incorporating a quadratic spectral phase (QSP) in the pulse profile. The sequential interaction with the gain medium of different spectral components of the pulse results in either suppression or enhancement of the coherent signatures on the pulse profile depending upon their proximity to the gain spectrum peak. In the absorption regime, positive QSP induces a negative chirp that adds up to that of a two photon absorption induced Kerr-like effect resulting in pulse compression while negative QSP enhances dispersive broadening of the pulse.
Squeezed light is usually generated using passive nonlinear materials. Semiconductor lasers and optical amplifiers (SOAs) also offer nonlinearities but they differ in that they add amplified spontaneous emission (ASE). Squeezing to below the vacuum level has been demonstrated in a semiconductor laser, and gain saturation in SOAs can likewise reduce photon-number fluctuations to, and in some cases below, the vacuum limit. Here, we demonstrate that Rabi oscillations in room-temperature quantum-dot SOAs, induced by short resonant pulses, cause cyclical noise modification that repeat with every change of 2pi in pulse area, corresponding to a fourfold increase in excitation pulse energy. Homodyne measurements reveal in those cases elliptical Wigner functions corresponding to squeezed thermal states and in certain regimes, the state is squeezed to below the vacuum level. At other pulse areas, the Wigner functions are circular representing thermal coherent states. This periodic behavior persists over two orders of magnitude in input pulse energy, spanning several 2pi cycles. Under specific bias and excitation conditions, we further observe a non-Gaussian Wigner function featuring two bright lobes. Although its precise nature remains unresolved, this structure may be consistent with a Schrodinger cat - like state whose accompanying negativity is suppressed due to an approximately 10 dB optical output loss. Notably, the emergence of this non-Gaussian state is itself periodic in excitation pulse energy.