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Journal of the Optical Society of America B

Squeezing and entanglement in doubly resonant, type II, second-harmonic generation

Ulrik L. Andersen, Preben Buchhave

Published Sep 1, 2003• 14 citations
Publisher

Abstract

We investigate, theoretically, the generation of bright and vacuum-squeezed light as well as entanglement in intracavity, type II, phase-matched second-harmonic generation. The cavity in which the crystal is embedded is resonant at the fundamental frequency but not at the second-harmonic frequency. A simple model for the process using semiclassical theory is derived, and quadrature-squeezing spectra of the involved fundamental fields are deduced. The analysis shows that vacuum squeezing reminiscent of subthreshold optical parametric oscillator squeezing is present and, in the ideal case, perfect. Under slight modifications of the operational conditions, the system is shown to produce efficient bright, squeezed light. Furthermore, we investigate the degree of polarization squeezing and find that three Stokes parameters can be squeezed simultaneously. Finally, we gauge the process for possible entanglement.

DOI
10.1364/josab.20.001947

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Physical Review A•Jun 1, 1994•19 citations
We investigate, theoretically, the generation of bright and vacuum-squeezed light as well as entanglement in intracavity, type II, phase-matched second-harmonic generation. The cavity in which the crystal is embedded is resonant at the fundamental frequency but not at the second-harmonic frequency. A simple model for the process using semiclassical theory is derived, and quadrature-squeezing spectra of the involved fundamental fields are deduced. The analysis shows that vacuum squeezing reminiscent of subthreshold optical parametric oscillator squeezing is present and, in the ideal case, perfect. Under slight modifications of the operational conditions, the system is shown to produce efficient bright, squeezed light. Furthermore, we investigate the degree of polarization squeezing and find that three Stokes parameters can be squeezed simultaneously. Finally, we gauge the process for possible entanglement.
We discuss quantum-fluctuation characteristics of a second-harmonic generation system that uses an optical resonator to confine only the fundamental field. It was predicted that the available amount of squeezing is limited to 1.76 dB for the fundamental output and 9.54 dB for the second-harmonic output, respectively, irrespective of system parameters. However, these predictions are based on low-order perturbation theory and are unavailable if the nonlinear coupling between the fundamental and the second harmonic becomes large. We consider the spatial evolution of the fields and reveal that the maximum amount of squeezing depends on the cavity loss: Even an arbitrary amount of squeezing is possible for both the fundamental output and the second-harmonic output. We also consider the possibility of parametric oscillation of empty cavity modes pumped by the generated second harmonic and derive the following prediction: In a system that uses a type I phase-matched crystal, the oscillation of the side mode hardly occurs because of sum-frequency generation with the fundamental and scarcely imposes any limitations on squeezing. On the other hand, a system with a type II phase-matched crystal suffers from the oscillation of the polarization mode orthogonal to that of the fundamental input, and squeezing of the second-harmonic output is limited to 3 dB.
We have generated squeezed states of light by the process of second harmonic conversion within an optical cavity resonant at both fundamental and harmonic frequencies. The experiment consists of a standing-wave cavity containing a crystal of lithium niobate doped with magnesium oxide and driven by the field from a frequency-stabilized Nd:YAG laser (incident power, ~10 mW). The total field reflected from the cavity illuminates a pair of high quantum efficiency photodiodes, whose individual photocurrents are summed. Observations of squeezing are made by analyzing the spectral density of fluctuations for this sum photo-current while the cavity detuning is scanned through resonance. An intensity regulator holds the reflected light intensity constant during the scan by control of the incident light level. Reductions in photocurrent fluctuations of 12% relative to the vacuum-state or shot-noise level are achieved for frequency offsets near 4 MHz. Since significantly higher degrees of squeezing are predicted by our theoretical analysis, we discuss those processes that currently limit the observed noise reduction, including phase noise produced by the intracavity crystal in the absence of nonlinear conversion.
Squeezed states of light represent a manifestation of the nonclassical character of the electromagnetic field and hence are of great intrinsic interest in quantum optics. There are as well a number of applications in measurement science and optical communication associated with the possibility of sensitivity beyond the standard quan­tum limit. The experiments that we have undertaken attempt to explore the degree of achievable and detectable squeezing in three distinct physical systems. From a conceptual point of view each is in some sense ideal and should provide a large degree of squeezing. However, in practice each offers a potential set of advantages and disadvantages associated with technological constraints and with a lack of precise correspondence between experiment and existing theoretical models. The three experiments that we describe are as follows: (1) degenerate parametric oscillation in a doubly resonant cavity pumped by the frequency-doubled light from a Nd:YAG laser at 1.06 μm, (2) intracavity second harmonic generation in a doubly resonant cavity pumped at a fundamental wave­length of 515 nm with an Ar+ laser, and (3) optical bistability for a collection of two-level atoms within a high finesse interferometer of decay rate comparable to the inverse atomic lifetime.
We analyze squeezing of both the fundamental and harmonic fields undergoing traveling-wave, second-harmonic generation (SHG) in second-order (${\mathrm{\ensuremath{\chi}}}^{(2)}$) nonlinear media. We take into account depletion of the fundamental field as well as the phase mismatch between the fundamental and harmonic fields. The behavior of the quantum noises on the propagating fields is studied by linearizing the nonlinear operator equations around the mean-field values. We first consider the degenerate case that is applicable to type-I phase-matching geometries, obtaining expressions for squeezing in both the fundamental and harmonic fields under the conditions of perfect phase matching and large phase mismatch. We show that in the case of a large phase mismatch, the intensity-dependent self-phase shift of the fundamental field, arising due to cascading of the ${\mathrm{\ensuremath{\chi}}}^{(2)}$ nonlinearity, is responsible for the squeezing generation. We also numerically solve the linearized quadrature-operator equations together with the nonlinear mean-field equations. We find that in the case of a finite phase mismatch the harmonic field can be highly squeezed. This is in contrast to the perfectly phase-matched case where the maximum squeezing is limited to 50%. Finally, we analyze the nondegenerate case that applies to type-II phase-matching geometries. Here we show that the commonly used type-II phase-matched SHG process with the input harmonic field in the vacuum state is equivalent to a type-I SHG process in parallel with a degenerate optical-parametric process. The latter causes squeezing in the mode that is polarized orthogonal to the fundamental beam. In the perfect phase-matching case, the squeezing in the orthogonally polarized mode follows the simple expression S=1-\ensuremath{\gamma}, where \ensuremath{\gamma} is the harmonic conversion frequency.
Classical and quantum fluctuations are analyzed in the system of type-II harmonic generation where two frequency-degenerate subharmonic fields with orthogonal polarizations are required for the generation of a harmonic field. The two subharmonic fields as well as the harmonic fields are on resonance in a cavity. It is found that there is no self-pulsing behavior as predicted for the type-I case where the intensities of both the subharmonic and the harmonic fields undergo fast oscillation. Instead there exists a threshold that is identified as the onset of an optical parametric oscillator (OPO) formed by a subharmonic mode with its polarization orthogonal to the input polarization (not the original modes). When the loss for the harmonic field is small, most of the input power is converted to the output power of the OPO. Under this circumstance, quantum-nondemolition measurements of the input can be performed at certain frequencies. The spectra of squeezing are calculated for the two subharmonic modes and it is found that both modes are squeezed for a certain range of frequency. The output of the OPO is found to exhibit phase squeezing.