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Physical review. B, Condensed matter

Generalized coherent-state derivation of time-dependent density-functional theory equations for superconductors

Oleg L. Berman, Shaul Mukamel

Published Sep 23, 2003• 2 citations
Publisher

Abstract

Equations of motion are derived for the normal and anomalous single-electron density matrices of a Fermi liquid using a time-dependent finite-temperature generalized coherent-state variational ansatz for the many-body density matrix. Self-consistent equations for the order parameter $\ensuremath{\Delta}$ allow us to investigate the interplay of the Coulomb repulsion and pairing attraction in homogeneous and inhomogeneous Fermi liquids with spontaneously broken symmetry such as high-temperature superconductors. The temperature of the Kosterlitz-Thouless transition to the two-dimensional superfluidity is calculated.

DOI
10.1103/physrevb.68.104519

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Equations of motion are derived for the normal and anomalous single-electron density matrices of a Fermi liquid using a time-dependent finite-temperature generalized coherent-state variational ansatz for the many-body density matrix. Self-consistent equations for the order parameter \ensuremathΔ\ensuremath{\Delta}\ensuremathΔ allow us to investigate the interplay of the Coulomb repulsion and pairing attraction in homogeneous and inhomogeneous Fermi liquids with spontaneously broken symmetry such as high-temperature superconductors. The temperature of the Kosterlitz-Thouless transition to the two-dimensional superfluidity is calculated.
The microscopic theory of a superfluid Fermi liquid at finite temperature is developed for the case of a pure system with SSS-wave pairing, and applied to the calculation of the static properties. As a function of $\ensuremath{\theta}\ensuremath{\equiv}\frac{T}{{T}_{c}}$ these properties are determined entirely by the Landau parameters F0{F}_{0}F0​, F1{F}_{1}F1​, Z0{Z}_{0}Z0​, etc., characterizing quasiparticle interactions in the normal phase. In particular the spin susceptibility $\ensuremath{\chi}$ and the density of the normal component ${\ensuremath{\rho}}_{n}$ are given by $\frac{\ensuremath{\chi}(\ensuremath{\theta})}{\ensuremath{\chi}(1)}=(1+\frac{1}{4}{Z}_{0})\frac{f(\ensuremath{\theta})}{[1+\frac{1}{4}{Z}_{0}f(\ensuremath{\theta})]},$ $\frac{{\ensuremath{\rho}}_{n}}{\ensuremath{\rho}}=(1+\frac{1}{3}{F}_{1})\frac{f(\ensuremath{\theta})}{[1+\frac{1}{3}{F}_{1}f(\ensuremath{\theta})]},$ where the universal function $f(\ensuremath{\theta})\ensuremath{\equiv}\ensuremath{-}{[\ensuremath{\nu}(0)]}^{\ensuremath{-}1}{\ensuremath{\Sigma}}_{\mathrm{p}}(\frac{\mathrm{dn}}{d{E}_{\mathrm{p}}})$ is the "effective density of states near the Fermi surface" relative to its value $\ensuremath{\nu}(0)$ in the normal phase. Thus the often-quoted expression ${\ensuremath{\rho}}_{n}=\frac{1}{3}{\ensuremath{\Sigma}}_{\mathrm{p}}{\mathrm{p}}^{2}(\frac{\mathrm{dn}}{d{E}_{\mathrm{p}}})$ is valid for an interacting system only in the limit $T\ensuremath{\rightarrow}0$. In the latter part of the paper a simple phenomenological theory of "Fermi-liquid" effects on $\ensuremath{\chi}$ and ${\ensuremath{\rho}}_{n}$ is developed for arbitrary conditions (including the presence of impurities and pairing with $l\ensuremath{\ne}0$); it is found that under most circumstances explicit expressions for $\ensuremath{\chi}$ and ${\ensuremath{\rho}}_{n}$ may be obtained which involve only the Landau parameters and a suitably generalized effective density of states. The theory should apply to the possible superfluid phase of He3{\mathrm{He}}^{3}He3 and to most superconductors. It is suggested that the Knight shift in nontransition-metal superconductors should display some "Fermi-liquid" effects. The weak-field dc penetration depth $\ensuremath{\lambda}(T)$ is shown to be insensitive to such effects both in the Pippard limit and near Tc{T}_{c}Tc​; however, in a London superconductor at lower temperatures the correction to $\ensuremath{\lambda}(T)$ should be observable and yield a direct estimate of F1{F}_{1}F1​.
The Fermi-liquid approach generalized to superfluid systems is used to derive general formulas for the normal and abnormal distribution functions (DF) for quasiparticles of a superfluid Fermi liquid (SFL) consisting of electrically neutral fermions with spin-triplet pairing (the spin of a pair s=1, the orbital angular momentum l of the pair being an arbitrary odd number) in a static uniform magnetic field, taking into account the Landau spin-exchange Fermi-liquid interaction at temperatures 0<T<Tc (Tc is the temperature of phase transition from the normal to the superfluid state). In deriving the DF, the explicit form of the energy functional (EF) for SFL is not used. A system of coupled equations is obtained for the order parameter, energy of quasiparticles, and effective magnetic field for the SFL under investigation in the case of an EF quadratic in DF. The obtained DF and the system of equations are applicable for describing both unitary and nonunitary phases of superfluid He3 in a magnetic field, e.g., for determining the magnetization and magnetic susceptibility of these phases.
A Fermi-liquid approach to the theory of superfluidity is developed, based on a generalization of the combinatoric expression for the entropy to the case in which the state of the Fermi liquid is described not only by a normal but also by an anomalous distribution function. The energy of the superfluid Fermi liquid is given in the form of a functional of these distribution functions. In the weak-coupling approximation the Fermi-liquid approach is equivalent to the BCS theory. The interaction between the Fermi liquid and an electromagnetic field is gauge invariant. In addition to the singlet-pairing theory the triplet-pairing theory is also developed. A unified variational principle that gives rise to the theory of superfluidity (superconductivity) is used to obtain the London equations and the Ginzburg–Landau equation. Applications of this theory are made to the derivation of an equation for ideal two-component hydrodynamics.
General expressions are obtained in explicit form for the anomalous and normal distribution functions of quasiparticles in nonunitary phases of a superfluid paramagnetic Fermi liquid consisting of electrically neutral fermions with triplet pairing (the pairs have spin s=1 and an arbitrary odd value of the orbital angular momentum l) in a uniform static magnetic field. A generalized Fermi-liquid approach is used which takes into account the exchange Fermi-liquid interaction but does not specify the form of the energy functional of the superfluid Fermi liquid. The results are valid at any temperature in the interval 0⩽T⩽Tc, where Tc is the temperature of the phase transition from the normal to the superfluid state. When an explicit form of the energy functional is specified, the general formulas for the distribution function can be used to describe the various nonunitary phases of a superfluid Fermi liquid of the He3 type in a high magnetic field. In particular, for He3-A1, He3-A2, and the nonunitary two-dimensional phase of He3 in a high magnetic field at 0⩽T⩽Tc, an energy functional quadratic in the distribution function is used to find a system of coupled equations for the order parameter and the effective magnetic field and to obtain an expression is obtained for the nonlinear magnetic susceptibility.
We study the thermodynamics of a superconductor with strongly bound Cooper pairs by solving the self-consistent T-matrix equations for the attractive Hubbard model within a local approximation. We determine the transition temperature as a function of the interaction strength at quarter filling, and compute the temperature dependence of the superconducting order parameter, the specific heat, the spin susceptibility, and the density of local pairs in the normal and superconducting phase. Pronounced deviations from BCS behavior are found already for moderate interactions, where superconductivity sets in at a critical temperature above the coherence temperature for Fermi liquid behavior.
We have developed a semi-analytical framework formulated in the canonical fermion representation to investigate strongly correlated electron systems. We consider the U=∞\infty∞ Hubbard model and used the equation of motion method to calculate the fermion self-energy which has two parts: single and two-boson exchange processes. The emergent bosons here are self-generated local charge and spin-density fluctuations which become strongly time-dependent due to extreme correlations. The computed boson spectral density is a diffusive damped mode with a long tail. The electron self-energy at d=∞d=\inftyd=∞ is computed self-consistently. The corresponding fermionic spectral density displays a pronounced coherence peak at ω=0ω=0ω=0, while its frequency derivative develops a two-peak structure at finite ωωω. The resistivity shows a linear temperature dependence over a broad range, crossing over to coherent Fermi-liquid behavior at extremely low temperatures.