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International Conference on Atomic Physics (ICAP)

Ultracold three-body recombination of fermionic atoms

Brett D. Esry, Hiroya Suno, Chris H. Greene

Published Apr 1, 2003• 2 citations
Publisher

Abstract

Three-body recombination can play an important role in experiments on ultracold atomic gases because it can produce significant atom loss. Such losses have been seen in Bose-Einstein condensates, but have been thought to play little role for degenerate Fermi gases. We show that under some circumstances, three-body recombination can be just as large in fermi systems as in bose systems. In particular, when there is a two-body resonance near threshold — as is often the case experimentally — the threshold suppression due to the Pauli principle no longer applies. 1

DOI
10.1142/9789812705099_0014

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Three-body recombination can play an important role in experiments on ultracold atomic gases because it can produce significant atom loss. Such losses have been seen in Bose-Einstein condensates, but have been thought to play little role for degenerate Fermi gases. We show that under some circumstances, three-body recombination can be just as large in fermi systems as in bose systems. In particular, when there is a two-body resonance near threshold — as is often the case experimentally — the threshold suppression due to the Pauli principle no longer applies. 1
We study inelastic processes for ultracold three-body systems in which only one interaction is resonant. We show that at ultracold temperatures three-body recombination in such systems leads mainly to the formation of weakly bound molecules. In addition, and perhaps more importantly, we have found that the decay rates for weakly bound molecules due to collisions with other atoms can be suppressed not only without fermionic statistics but also when bosonic statistics applies. These results indicate that recombination in three-component atomic gases can be used as an efficient mechanism for molecular formation, allowing the achievement of high molecular densities.
Achieving precise control of ultracold atomic gases requires a detailed understanding of atom loss mechanisms. Motivated by the anomalous three-body decay in a three-component Fermi gas reported in Ref. [1], this work investigates mechanisms that possibly contribute to the observed loss. The three-body Schrödinger equation is solved in the hyperspherical adiabatic representation with pairwise van der Waals interactions, and the SSS-matrix is obtained via the eigenchannel RRR-matrix method to compute recombination rate coefficients K3K_3K3​ and two-body cross sections. At the magnetic field strength where the anomalous decay occurs, K3K_3K3​ is unitary limited, exhibiting the threshold energy scaling K3(E)∝E−1K_3(E)\propto E^{-1}K3​(E)∝E−1. Consequently, the thermally averaged ⟨K3⟩\langle K_3 \rangle⟨K3​⟩ acquires a temperature dependence. Because the experiment is performed in the degenerate regime, ⟨K3⟩\langle K_3 \rangle⟨K3​⟩ also explicitly depends on the per-spin densities through the per-spin Fermi energies EF(i)∝ni2/3E_{F}^{(i)}\propto n_i^{2/3}EF(i)​∝ni2/3​. As the gas is diluted and degeneracy is reduced, ⟨K3⟩\langle K_3 \rangle⟨K3​⟩ approaches the non-degenerate value and becomes a function of temperature only. Channel-resolved branching ratios and cross sections are folded into a Monte Carlo cascade simulation of secondary collisions and trap escape. The analysis indicates that typical three-body recombination events remove fewer than three atoms on average, and that the atom losses are primarily due to the ejection of secondary collision products, rather than the initial three-body recombination products. Therefore, a significant fraction of the released binding energy remains in the trapped ensemble as kinetic energy. Retained energy drives evaporative loss, offering a plausible, partial explanation for the anomalous decay.
Few-body effects play an important role for the understanding of ultracold quantum gases. We make use of an effective field theory approach to investigate various aspects of universal few-body physics close to a Feshbach resonance. That is the regime where the scattering length is large compared to all other length scales of the system and thus determines the observables. It is also the regime where the Efimov effect whose main characteristic is the occurrence of a sequence of three-body bound states becomes important. At unitarity, i.e., for diverging scattering length, the ratio of binding energies of neighboring states approaches a constant. The existence of those trimers can be captured by a single three-body parameter and influences observables such as recombination rates. Starting from adequate Lagrangians, we derive atom-dimer scattering amplitudes that contain all information of interest about the three-particle systems. With this method, we first investigate the scattering of atoms and dimers at finite temperature in the presence of the Efimov effect. We calculate the dimer relaxation rate and obtain good agreement with available experimental data. Furthermore, heteronuclear mixtures exhibiting large interspecies scattering length are studied in detail. If bosons are the majority species, the Efimov effect occurs in an S-wave channel and we are able to compute three-body recombination and dimer relaxation rates. The results are compared to the outcome of two existing experiments. For mainly fermionic systems, the Efimov effect is only present in an overall P-wave and three-body recombination at threshold vanishes. However, in mixtures of atoms and dimers, scattering cross sections and dimer relaxation show the typical Efimov behavior of log-periodicity. We also consider two-dimensional Bose gases, where the Efimov effect does not occur. For those systems, we derive an equation including the first non-universal corrections and deduce three-body observables such as binding energies and atom-dimer scattering parameters.
We study the properties of strongly interacting Bose gases at the density and temperature regime when the three-body recombination rate is substantially reduced. In this regime, one can have a Bose gas with all particles in scattering states (i.e., the "upper branch") with little loss even at unitarity over the duration of the experiment. We show that because of bosonic enhancement, pair formation is shifted to the atomic side of the original resonance (where scattering length a(s)<0), opposite to the fermionic case. In a trap, a repulsive Bose gas remains mechanically stable when brought across resonance to the atomic side until it reaches a critical scattering length a(s)*<0. For a(s)<a(s)*, the density consists of a core of upper branch bosons surrounded by an outer layer of equilibrium branch. The conditions of low three-body recombination require that the particle number N<1.024(T/ω)(5/2) in a harmonic trap with frequency ω.
In several experiments with ultracold trapped atoms, a narrow loss feature has been observed near an atom-dimer resonance, at which there is an Efimov trimer at the atom-dimer threshold. The conventional interpretation of these loss features is that they are produced by the avalanche mechanism, in which the energetic atom and dimer from three-body recombination undergo secondary elastic collisions that produce additional atoms with sufficient energy to escape from the trapping potential. We use Monte Carlo methods to calculate the average number of atoms lost and the average heat generated by recombination events in a Bose-Einstein condensate and in a thermal gas. We improve on previous models by taking into account the energy dependence of the cross sections, the spatial structure of the atom cloud, and the elastic scattering of the atoms. We show that the avalanche mechanism cannot produce a narrow loss feature near the atom-dimer resonance. The number of atoms lost from a recombination event can be more than twice as large as the three that would be obtained in the absence of secondary collisions. However, the resulting loss feature is broad and its peak is at a scattering length that is larger than the atom-dimer resonance and depends on the trap depth.