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Physical Review B

Decoherence dynamics of a single spin versus spin ensemble

V. V. Dobrovitski, A. E. Feiguin, D. D. Awschalom, Ronald Hanson

Published Jun 26, 2008• 81 citations
Publisher

Abstract

We study decoherence of central spins by a spin bath, focusing on the difference between measurement of a single central spin and measurement of a large number of central spins (as found in typical spin-resonance experiments). For a dilute spin bath, the single spin demonstrates Gaussian free-induction decay, in contrast to exponential decay characteristic of spin ensembles. A strong difference between a single spin and a spin ensemble also exists for the Rabi oscillation decay: for a repeated Rabi oscillation experiment, suppression of decoherence happens for a single spin while acceleration takes place for a spin ensemble. The mathematical origin of such behavior is similar to quantum Zeno/anti-Zeno effects.

DOI
10.1103/physrevb.77.245212

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We study the dynamics of a single spin 1∕21∕21∕2 coupled to a bath of spins 1∕21∕21∕2 by inhomogeneous Heisenberg couplings including a central magnetic field. This central-spin model describes decoherence in quantum bit systems. An exact formula for the dynamics of the central spin is presented, based on the Bethe ansatz. For initially completely polarized bath spins and small magnetic field, we find persistent oscillations of the central spin about a nonzero mean value. For a large number of bath spins Nb{N}_{b}Nb​, the oscillation frequency is proportional to Nb{N}_{b}Nb​, whereas the amplitude behaves as 1∕Nb1∕{N}_{b}1∕Nb​, to leading order. No asymptotic decay of the oscillations due to the nonuniform couplings is observed, in contrast to some recent studies.
We numerically investigate decoherence of a two-spin system (central system) by a bath of many spins 1/2. By carefully adjusting parameters, the dynamical regime of the bath has been varied from quantum chaos to regular, while all other dynamical characteristics have been kept practically intact. We explicitly demonstrate that for a many-body quantum bath, the onset of quantum chaos leads to significantly faster and stronger decoherence compared to an equivalent non-chaotic bath. Moreover, the non-diagonal elements of the system's density matrix, the linear entropy, and the fidelity of the central system decay differently for chaotic and non-chaotic baths. Therefore, knowledge of the basic parameters of the bath (strength of the system-bath interaction, and the bath's spectral density of states) is not always sufficient, and much finer details of the bath's dynamics can strongly affect the decoherence process.
We develop a mathematical description of the decoherence caused by "spin baths", such as nuclear spins or magnetic impurities. In contrast to the usual oscillator bath models of quantum environments, decoherence in the spin bath can occur without any dissipation. Given the almost ubiquitous presence of nuclear spins in nature, our results have important consequences for quantum measurement theory, particularly as the decoherence mechanisms in spin baths work very differently from those in oscillator baths.
The quantum dynamics of mesoscopic or macroscopic systems is always complicated by their coupling to many `environmental' modes. At low T these environmental effects are dominated by localized modes, such as nuclear and paramagnetic spins, and defects (which also dominate the entropy and specific heat). This environment, at low energies, maps onto a `spin bath' model. This contrasts with `oscillator bath' models (originated by Feynman and Vernon) which describe delocalized environmental modes such as electrons, phonons, photons, magnons, etc. The couplings to N spin bath modes are independent of N (rather than the ~O(1/( N ) 1/2 ) dependence typical of oscillator baths), and often strong. One cannot in general map a spin bath to an oscillator bath (or vice versa); they constitute distinct `universality classes' of quantum environment. We show how the mapping to spin bath models is made, and then discuss several examples in detail, including moving particles, magnetic solitons, nanomagnets, and SQUIDs, coupled to nuclear and paramagnetic spin environments. We then focus on the `central spin' model, which couples a central two-level system to a background spin bath. It is the spin bath analogue of the famous `spin-boson' oscillator model, and describes, e.g., the tunnelling dynamics of nanoscopic and mesoscopic magnets and superconductors. We show how to average over (or `integrate out') spin bath modes, using an operator instanton technique, to find the central spin dynamics. The formal manouevres involve four separate averages - each average corresponds physically to a different `decoherence' mechanism acting on the central spin dynamics. Each environmental spin has its own topological `spin phase', which by interacting with the phase of the central system, decoheres it - this can happen even without dissipation. We give analytic results for the central spin correlation functions, under various conditions. We then describe the application of this theory to magnetic and superconducting systems. Particular attention is given to recent work on tunnelling magnetic macromolecules, where the role of the nuclear spin bath in controlling the tunnelling is very clear; we also discuss other magnetic systems in the quantum regime, and the influence of nuclear and paramagnetic spins on flux dynamics in SQUIDs. Finally, we discuss decoherence mechanisms and coherence experiments in superconductors and magnets. We show that a spin bath environment causes decoherence even in the T 0 limit. Control of this decoherence will be essential in the effort to construct `qubits' for quantum computers.
We systematically investigate the universal spin decoherence dynamics of a localized electron in an arbitrary nuclear spin bath, which can even be far away from equilibrium due to the weak nuclear-lattice interaction. We show that the electron spin relaxation dynamics (as well as spin pure dephasing and Hahn echo decay) can always have a universal behavior as long as the initial state is composed of a sufficiently large amount of spin eigenstates. For a given system, the pattern of the universal dynamics depends on the complicated initial condition only via a single parameter, which measures the amount of phase coherence between different spin eigenstates in the initial state. Our results apply even when the number of the involved nuclei is not large and, therefore, provide a solid foundation in the comparison of the theoretical/numerical results to the experimental measurement. As an example, we also show the numerical results for systems of noninteracting spin bath in a zero magnetic field regime and discuss the features of universal decoherent dynamics.