A new method of acquiring two-dimensional correlation spectra in a single-shot is presented. As a demonstration of the functionality of this spectrometer, the two-dimensional correlation spectrum of atomic rubidium is measured.
We observed the spectral coherence structure of twin beam states generated by spontaneous parametric down-conversion by using a simple fiber spectrometer synchronized with a pulsed laser source. The recorded single-shot spectra exhibit a well-defined peak structure, where the peak wavelengths change values from shot to shot. We studied the number and the width of the peaks as a function of the different parameters in the experimental setup (pump power, iris size, iris distance from the BBO crystal). Moreover, we evaluated the number of modes in the intensity distribution of the light in different portions of the spectrum. The experimental results indicate that the number of modes from statistics and the number and width of the peaks evolve differently with the parameters.
We report an experimental demonstration of optical two-dimensional coherent spectroscopy (2DCS) in cold atoms. The experiment integrates a collinear 2DCS setup with a magneto-optical trap (MOT), in which cold rubidium (Rb) atoms are prepared at a temperature of approximately 200 µK and a number density of 10 10 cm −3 . With a sequence of femtosecond laser pulses, we first obtain one-dimensional second- and fourth-order nonlinear signals and then acquire both one-quantum and zero-quantum 2D spectra of cold Rb atoms. The capability of performing optical 2DCS in cold atoms is an important step toward optical 2DCS study of many-body physics in cold atoms and ultimately in atom arrays and trapped ions. Optical 2DCS in cold atoms/molecules can also be a new avenue to probe chemical reaction dynamics in cold molecules.