The collective decay effects between the dipole-active three-level subsystems in the nonlinear interaction with dipole-forbidden transitions, like 2 S − 1 S of hydrogen-like radiators, are proposed, taking into consideration the cooperative exchanges between two species of atoms through the vacuum field in the scattering and the two-photon resonance processes. One of them corresponds to the situation when the total energy of the emitted two photons by the three-level radiator in the cascade configuration enters into the two-photon resonance with another type of dipole-forbidden transitions of hydrogen-like (or helium-like) atoms. The similar situation appears in the cooperative scattering between two species of quantum emitters when the difference of the excited energies of the two dipole-active transitions of the three-level radiators is in the resonance with the dipole-forbidden transitions of the Hydrogen-like radiators. These effects are accompanied by the interference between single- and two-quantum collective transitions of the inverted radiators from the ensemble. The two-particle collective decay rate is defined in the description of the atomic correlation functions taking into consideration the phase retardation between them. The kinetic equations which describe the cooperative processes as the function of time and correlation are obtained. The behavior of the system of radiators at short and long time intervals in comparison with the retardation time between them is studied.
Using the formalism developed earlier, we treat spontaneous emission from a pair of identical two-level atoms
A1,
A2, whose separation
r21 can be comparable to the wavelength $\ensuremath{\lambda}$. We obtain expressions for time-dependent intensities and damping rates with the initial conditions (a) both atoms inverted, (b) prior excitation by a short $\frac{1}{2}\ensuremath{\pi}$ pulse, and (c) only
A1 inverted. The results in (a) are compared with those obtained for a model consisting of two initially excited harmonic oscillators
O1,
O2. The atoms exhibit superradiant behavior, whereas
O1,
O2 tend to trap radiation. In (a), the intensity pattern $\mathcal{R}(\ensuremath{\theta},t)$ develops lobes in different directions at different times, so that the spatial distribution of photons at time $t\ensuremath{\rightarrow}\ensuremath{\infty}$ is the same as in the independent-atom case ${r}_{21}\ensuremath{\gg}\ensuremath{\lambda}$. For the oscillators, the lobes of $\mathcal{R}(\ensuremath{\theta},t)$ do not change direction, but only become more pronounced as time increases. In (b) and (c), the lobes oscillate back and forth at frequency $2{\ensuremath{\Omega}}_{12}$ corresponding to the shifts $\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$ of the triplet and singlet states due to the ${A}_{1}\ensuremath{-}{A}_{2}$ interaction. The intensity can therefore have a sinusoidal component. Field correlation functions calculated for (a) and (c) show that
A2 and
A2 radiate simultaneously around the frequencies $\ensuremath{\epsilon}\ifmmode\pm\else\textpm\fi{}{\ensuremath{\Omega}}_{12}$, where $\ensuremath{\epsilon}$ is the single-atom resonant frequency. The spectrum is calculated for case (c), and shows the effects of coherent linewidth enhancement in addition to the frequency shifts.
An analysis is made of the deexcitation kinetics of strongly excited extended systems of initially uncorrelated two-level radiators. The possibility of partially cooperative states of the system is predicted when the radiation intensity acquires values intermediate between the spontaneous decay intensity and the Dicke superradiance intensity. The conditions for the onset of cooperative processes are obtained. The threshold for the oscillatory emission conditions is determined and the oscillation frequency is found. Modulation of the emission intensity is predicted with different modulation frequencies before and after the superradiant pulse. The modulation frequencies are determined. Formulas are derived for the superradiant pulse delay times and intensities. The possibility of weakly anisotropic cooperative emission is predicted.
Through studying the interaction between a two_level atom and a single mode emission field in rotating_wave approximations of Jaynes_Cummings Model, the atom and the field are in a coupled superposition state_entangled state is obtained. The expectation value of atom dipole moment is always zero, but the fluctuation of dipole moment is a constant, but not zero. Therefore it is concluded that the spontaneous emission of atoms is caused by the fluctuation of dipole moment, not by the dipole moment oscillation of the atomic system. The property of the entanglement is also studied and it is obtained that information entropy and the amount of entanglement are oscillating with time_evolution periodically and are related with the coupling coefficient and detuning. The quantum state changes between disentangled state and entangled state. The quantum state will be entangled state for a long time when the detuning is small.
Abstract. We discuss the creation of entanglement between two two-level atoms in the dissipative process of spontaneous emission. It is shown that spontaneous emission can lead to a transient entanglement between the atoms even if the atoms were prepared initially in an unentangled state. The amount of entanglement created in the system is quantified by using two different measures: concurrence and negativity. We find analytical formulas for the evolution of concurrence and negativity in the system. We also find the analytical relation between the two measures of entanglement. The system consists of two two-level atoms which are separated by an arbitrary distance r12 and interact with each other via the dipole-dipole interaction, and the antisymmetric state of the system is included throughout, even for small inter-atomic separations, in contrast to the small sample model. It is shown that for sufficiently large values of the dipole-dipole interaction initially the entanglement exhibits oscillatory behaviour with considerable entanglement in the peaks. For longer times the amount of entanglement is directly related to the population of the slowly decaying antisymmetric state.
We discuss the creation of entanglement between two two-level atoms in the dissipative process of spontaneous emission. It is shown that spontaneous emission can lead to a transient entanglement between the atoms even if the atoms were prepared initially in an unentangled state. The amount of entanglement created in the system is quantified by using two different measures: concurrence and negativity. We find analytical formulae for the evolution of concurrence and negativity in the system. We also find the analytical relation between the two measures of entanglement. The system consists of two two-level atoms which are separated by an arbitrary distance r 12 and interact with each other via the dipole–dipole interaction, and the antisymmetric state of the system is included throughout, even for small interatomic separations, in contrast to the small-sample model. It is shown that for sufficiently large values of the dipole–dipole interaction initially the entanglement exhibits oscillatory behaviour with considerable entanglement in the peaks. For longer times the amount of entanglement is directly related to the population of the slowly decaying antisymmetric state.