The influence of the temporal-coherence properties of the pump and signal waves on the efficiency and the temporal fidelity of the phase-conjugation process associated with degenerate four-wave mixing is examined.
One more promising application of the four-wave mixing process is the correction of arbitrary phase aberrations in an optical beam. In such applications, the fidelity as well as the efficiency of the phase-conjugation process needs to be considered in practice. The process which has received the most extensive attention to date is degenerate four-wave mixing (DFWM). The nonlinear interaction in this case is known to result in a perfect phase-conjugate provided high-quality pump beams are available and competing effects such as local self-focusing (or defocusing) can be neglected.
Degenerate four-wave mixing (DFWM) is a simple method to achieve phase conjugation. It uses the third-order nonlinearity of the electric susceptibility to produce changes in the optical properties of materials. A dynamic grating is then induced. Such gratings might be used as fast optical memories in optical computing. Our aim is to find media with large nonlinear susceptibilities and fast response time. We report phase conjugation of 532-nm laser radiation by DFWM in dye solutions. The time dependence of the conjugated wave is investigated experimentally and compared to theoretical predictions. We have also studied the influence of the solvents, dye concentration, and pump intensity on the phase conjugated signal. The results are compared with those predicted by three nonlinear mechanisms. Thermally induced refractive-index changes, Kerr effect, and saturable absorption are considered.