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Physical review. B, Condensed matter

Two-magnon states of the alternating-bond ferrimagnetic chain

A. J. M. Medved, B. W. Southern, David A. Lavis

Published Jan 1, 1991• 5 citations
Publisher

Abstract

In this paper we examine the nature of two-magnon excitations in the alternating-bond ferrimagnetic spin chain for general values S and S' of the two species of spin. Both a direct analytic approach as well as a method based on a scaling transformation are used to study the bound-state branches and their relationship to the two-magnon continuum.

DOI
10.1103/physrevb.43.816

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In this paper we examine the nature of two-magnon excitations in the alternating-bond ferrimagnetic spin chain for general values S and S' of the two species of spin. Both a direct analytic approach as well as a method based on a scaling transformation are used to study the bound-state branches and their relationship to the two-magnon continuum.
In this thesis we examine the nature of three magnon excitations in alternating spin/bond ferromagnetic chains. We study a Hamiltonian that describes a chain (composed of two non-identical one-dimensional uniform and homogeneous sublattices) with alternating spin magnitudes, S and SspprimeS\\sp\\primeSspprime, and alternating nearest neighbor interactions, Jsb1J\\sb1Jsb1 and Jsb2.J\\sb2.Jsb2. The Recursion Method is used to locate the bound states and their relationship to the three-magnon continuum. The specific cases studied are the S = SspprimeS\\sp\\primeSspprime = 1/2, S = 2Sspprime2S\\sp\\prime2Sspprime = 1, and S = SspprimeS\\sp\\primeSspprime = 1 alternating spin chains. We consider not only the effects of spin alternation but also of varying strengths. For each case, we studied different bond sets, more exactly, Jsb1J\\sb1Jsb1 = 1 and Jsb2J\\sb2Jsb2 equal to 0, 1/4, 1/2 and 1.
The nature of multimagnon excitations in alternating spin/bond ferromagnetic chains are studied using a combination of scaling methods and the recursion method. Two-magnon excitations for a Heisenberg chain with either alternating spin magnitudes, SSS and ${S}^{\ensuremath{'}},$ or alternating nearest-neighbor couplings, J1{J}_{1}J1​ and J2{J}_{2}J2​ can be studied using real-space rescaling techniques. These results are then used to investigate three-magnon excitations using the recursion method.
We numerically investigate elementary excitations of the Heisenberg alternating-spin chains with two kinds of spins, 1 and 1/2,1/2,1/2, antiferromagnetically coupled to each other. Employing a recently developed efficient Monte Carlo technique as well as an exact-diagonalization method, we verify the spin-wave argument that the model exhibits two distinct excitations from the ground state which are gapless and gapped. The gapless branch shows a quadratic dispersion in the small-momentum region, which is of the ferromagnetic type. With the intention of elucidating the physical mechanism of both excitations, we make a perturbation approach from the decoupled-dimer limit. The gapless branch is directly related to spin 1's, while the gapped branch originates from cooperation of the two kinds of spins.
The spectra of both two- and three-magnon excitations in Heisenberg spin chains with next-nearest-neighbour (NNN) interactions are studied using scaling methods and the recursion method respectively. Both two-spin and three-spin couplings are considered for general spin S. In the three-magnon case, the asymptotic behaviour of the recursion coefficients can be used to directly identify the presence of bound states in the spectrum. Both integrable and non-integrable models can be studied, and the integrable models display special features in the bound-state spectra. Our results for the three-magnon bound states of S = 1 chains differ appreciably from those obtained in previous studies based upon an integral equation approach.
Motivated by recent measurements on CuGeO3{\mathrm{O}}_{3}O3​, the spectrum of magnetic excitations of an antiferromagnetic S=12S=\frac{1}{2}S=21​ chain with alternating coupling strength is investigated. Wave-vector-dependent magnons and a continuum with square-root behavior at the band edges are found. The spectral density of the continua is calculated. Spin-rotation symmetry fixes the gap of the continuum to be twice the elementary magnon gap. This is in excellent agreement with experimental results. The existence of (anti)bound states of two magnons is predicted: below the continuum a singlet and a triplet, above the continuum a quintuplet.