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Journal of the Optical Society of America B

Perturbation analysis of Raman echo

Heiki Sõnajalg, Myung K. Kim

Published Jun 1, 1998• 2 citations
Publisher

Abstract

A time-dependent perturbational approach is used to study the Raman echo generated by an inhomogeneous ensemble of three-level atomic systems in the Λ configuration. The sixth-order perturbative solution for coherence between the two lower states contains eight echo terms that are visualized with double Feynman diagrams. The echo is interpreted as a response of the ensemble to six short single-frequency optical pulses whose timing satisfies a special condition. Nonperturbative numerical simulation confirms the predictions of the perturbation analysis about the main characteristics of the echo. When the excitation pulses vary adiabatically with respect to fast optical coherence decay the echo amplitude depends on interference of the eight terms. A computational scheme developed for the higher-order perturbative analysis is also discussed.

DOI
10.1364/josab.15.001780

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A time-dependent perturbational approach is used to study the Raman echo generated by an inhomogeneous ensemble of three-level atomic systems in the Λ configuration. The sixth-order perturbative solution for coherence between the two lower states contains eight echo terms that are visualized with double Feynman diagrams. The echo is interpreted as a response of the ensemble to six short single-frequency optical pulses whose timing satisfies a special condition. Nonperturbative numerical simulation confirms the predictions of the perturbation analysis about the main characteristics of the echo. When the excitation pulses vary adiabatically with respect to fast optical coherence decay the echo amplitude depends on interference of the eight terms. A computational scheme developed for the higher-order perturbative analysis is also discussed.
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The analysis of nonlinear spectroscopy, widely used to study the dynamics and structures of condensed-phase matter, typically employs a perturbative approach noticing the weak interaction between the laser and the matter of interest. However, such perturbative approach is no longer applicable once the interaction between the laser and the matter is strong. We adapt the method of quantum dynamical evolution into the calculation of signal and present the response formalism of the nonlinear spectroscopy in a nonperturbative approach. In this new approach, we demonstrate that in addition to the third-order term in the perturbative method, the higher-order terms have essential contributions to the nonlinear signal of the two-pulse and three-pulse photon echo (2PPE and 3PPE). The detailed calculations are demonstrated with the example of a three-level V-type system, which is widely used in the studies of quantum optics. We consider the effect of the environment via a pure dephasing mechanism with both the localized modes of each molecule and the shared modes between molecules.
The dynamics of an ultracold dilute boson gas in an optical lattice is described in the framework of the Bose-Hubbard model in which the parameters of the system are controlled by light. Within this model, an ensemble of Bose-Einstein condensates trapped in cells of a double optical lattice generates an echo response in the quantum-mechanical probability current. The echo signal is excited by biharmonic radiation pulses under two-photon (Raman) resonance conditions. The time profile of the echo signal and the role played by the inhomogeneous broadening and the interaction of atoms in the formation of the boson echo are discussed.
An analytical study of the photon echoes associated with the three-level system interacting resonantly with optical pulses possessing two different frequencies is performed. It is predicted that photon echoes arise at anomalous times corresponding to the correlation between the inhomogeneous broadenings for the different spectral lines as well as at the normal time expected in a simple two-level system. This new effect is caused by the coupling of the two resonant transitions through the common energy level. Furthermore, if the particle does not have inversion symmetry, the echoes with the sum or difference frequency of the exciting optical pulses can be observed in such a system. The quantitative analysis is also given for intensities, direction of propagation and polarizations of the anomalous echoes which depend upon the exciting pulses with different frequency.
A generalized perturbation theory is developed for an inhomogeneously broadened two-level quantum system interacting with an optical field of arbitrary temporal shape. Solutions of the Liouville equation carried out to nth order in the optical field strength exhibit a rephasing behavior and therefore are interpreted as an n-pulse echo where each pulse corresponds to one power of the field strength. We conclude that at low fields any coherence effect can be interpreted as a generalized stimulated echo phenomenon. Several well-understood coherence effects are explained and a few new ones are predicted, including one example where the light source is incoherent.