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Physical Review A

Quantum limits to all-optical phase shifts in a Kerr nonlinear medium

Barry C. Sanders, Gerard J Milburn

Published Feb 1, 1992• 67 citations
Publisher

Abstract

We consider two copropagating fields in a nonlinear Kerr medium, each with a particular phase and intensity. The Kerr medium possesses an intensity-dependent refractive index and the phase shift of each field thus depends on the intensities of the fields. Classically it is possible to induce an arbitrary phase shift of one field (the signal field) by either increasing the intensity of the other field (the control field) or by increasing the interaction legnth. We show that if the intensity of the control field is low, the phase shift on the signal is limited by the discrete nature of the photon-number distribution in the control field and cannot be increased simply by increasing the interaction length. In general the maximum phase shift of the signal field is \ensuremath{\varphi} if the control field possesses \ensuremath{\varphi} photons. This limit arises as a consequence of quantum recurrence effects.

DOI
10.1103/physreva.45.1919

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We consider two copropagating fields in a nonlinear Kerr medium, each with a particular phase and intensity. The Kerr medium possesses an intensity-dependent refractive index and the phase shift of each field thus depends on the intensities of the fields. Classically it is possible to induce an arbitrary phase shift of one field (the signal field) by either increasing the intensity of the other field (the control field) or by increasing the interaction legnth. We show that if the intensity of the control field is low, the phase shift on the signal is limited by the discrete nature of the photon-number distribution in the control field and cannot be increased simply by increasing the interaction length. In general the maximum phase shift of the signal field is \ensuremath{\varphi} if the control field possesses \ensuremath{\varphi} photons. This limit arises as a consequence of quantum recurrence effects.
A cross-Kerr interaction produces a phase shift on two modes of light proportional to the number of photons in both modes and is sometimes called cross-phase modulation. Cross-Kerr nonlinearities have many applications in classical and quantum nonlinear optics, including the possibility of a deterministic and all-optical controlled-phase gate. We calculate the one- and two-photon SSS matrices for fields propagating in a medium where the cross-Kerr interaction is spatially distributed at discrete interaction sites comprised of atoms. For the interactions considered, we analyze the cases where the photons copropagate and counterpropagate through the medium and give a physical interpretation to the differences between the two cases. Finally, we obtain the SSS matrix in the limit of infinitely long chains, showing that it corresponds to a perfect controlled-phase operation.
The self-Kerr interaction is an optical nonlinearity that produces a phase shift proportional to the square of the number of photons in the field. At present, many proposals use nonlinearities to generate photon-photon interactions. For propagating fields these interactions result in undesirable features such as spectral correlation between the photons. Here we engineer a discrete network composed of cross-Kerr interaction regions to simulate a self-Kerr medium. The medium has effective long-range interactions implemented in a physically local way. We compute the one- and two-photon SSS matrices for fields propagating in this medium. From these scattering matrices we show that our proposal leads to a high-fidelity photon-photon gate. In the limit where the number of nodes in the network tends to infinity, the medium approximates a perfect self-Kerr interaction in the one- and two-photon regime.
The influence of quantum fluctuations of the electromagnetic field on the propagation of a polarized light wave in a nonlinear dielectric is investigated. It is shown that in some cases the fluctuations couple to the optical nonlinearities of the medium and make its refractive index dependent on the polarization of the propagating wave. As a consequence, two light waves propagating in the same direction but with different polarizations will have different speeds, so there will be a Kerr-effect birefringence induced by quantum fluctuations. We consider the case of the electromagnetic field in a squeezed vacuum state, where there are regions where the mean squared electric field can be negative and the birefringence effect has the opposite sign to the Kerr effect in classical physics. We give some estimates for the magnitude of these effects, and discuss their possible observability.
Intense light beams propagating in a lossless, dispersionless, single-mode optical fiber are subject to the Kerr effect, i.e., to the intensity-dependent refractive index of the fiber’s fused-silica core. Classically, Kerr-effect-induced self-phase modulation (SPM) can be used for spectral broadening of a picosecond pulse for grating-pair pulse compression down to femtosecond duration. Quantum mechanically, Kerr-effect-induced four-wave mixing (FWM) has been used to produce squeezed-state light. We present a quantum propagation theory for a lossless, dispersionless fiber with the Kerr nonlinearity. The theory includes classical SPM and quantum FWM within their regions of validity. It introduces a material time constant for the Kerr interaction, limiting the quantum phase shifts caused by the broadband zero-point fluctuations that accompany any input field, to develop a coarse-grained time multitemporal mode field analysis. Explicit expressions are obtained for the first and the second output-field moments when the fiber’s input field is in an arbitrary Gaussian state. These results are used to obtain homodyne-detection noise spectra, which are employed, in turn, to seek experimentally accessible manifestations of the Kerr time constant.
Summary form only given.Nonlinear optical effects are normally limited to high-intensity fields containing a large number of photons because the electric field associated with a single photon is usually very weak. Nonlinear phase shifts at the two-photon level previously have been observed using high-Q cavities and atomic beams. The authors recently predicted that nonlocal effects involving pairs of atoms in a medium could enhance the nonlinear interaction between two photons to the point that nonlinear phase shifts could be obtained in an ordinary medium without the use of resonant cavities.