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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Progress towards atomic vapor photonic microcells: atomic polarization decoherence of Zeeman levels in rubidium filled HC-PCF

Ekaterina Ilinova, Thomas D. Bradley, Fetah Benabid

Published Feb 21, 2014• 0 citations
Publisher

Abstract

We report a study on de-phasing mechanisms in Rb-filled hypocycloidal core shape Kagome hollowcore photonic crystal fibers. We experimentally measure the atomic polarization relaxation rates in Rb loaded bare silica Kagome hollow-core photonic crystal fibers at six different geometries. The measurements show a polarization relaxation time ranging from from ~ 16 μs for a 30 μm core inner-diameter HC-PCF to ~34 μs for a 96 μm core inner-diameter HC-PCF. The measured polarization lifetimes are much longer than the typical transit time for the atomic vapor at room temperature. We perform the theoretical analysis of the mechanisms of atomic de-coherence taking to account the fiber geometries and further experimental parameters. The analysis demonstrates that at given experimental conditions the main contribution to the polarization rotation signal comes from the transversally slow atoms. The effective temperature of the polarized atoms is than lower than the room temperature. We perform the Monte-Carlo simulations to calculate the atomic polarization relaxation rate in fibers with different inner core radius and negative curvature parameters. The calculated values are in a good agreement with the experimental results.

DOI
10.1117/12.2047537

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We report a study on de-phasing mechanisms in Rb-filled hypocycloidal core shape Kagome hollowcore photonic crystal fibers. We experimentally measure the atomic polarization relaxation rates in Rb loaded bare silica Kagome hollow-core photonic crystal fibers at six different geometries. The measurements show a polarization relaxation time ranging from from ~ 16 μs for a 30 μm core inner-diameter HC-PCF to ~34 μs for a 96 μm core inner-diameter HC-PCF. The measured polarization lifetimes are much longer than the typical transit time for the atomic vapor at room temperature. We perform the theoretical analysis of the mechanisms of atomic de-coherence taking to account the fiber geometries and further experimental parameters. The analysis demonstrates that at given experimental conditions the main contribution to the polarization rotation signal comes from the transversally slow atoms. The effective temperature of the polarized atoms is than lower than the room temperature. We perform the Monte-Carlo simulations to calculate the atomic polarization relaxation rate in fibers with different inner core radius and negative curvature parameters. The calculated values are in a good agreement with the experimental results.
We report a comparative study on dephasing mechanisms between inner core coated and uncoated sections of the same Kagome hypocycloid-shaped core hollow core photonic crystal fibers (HC-PCF) filled with rubidium vapor. The comparison is performed by measuring the atomic polarization relaxation and electromagnetically induced transparency (EIT) linewidth in Rb loaded polydimethylsiloxane (PDMS) inner wall coated and bare silica core Kagome HC-PCF. The measurements show a polarization relaxation time of 32μs in a PDMS coated Kagome HC-PCF and 24μs in uncoated Kagome HC-PCF. A minimum EIT linewidth of 6.2±0.8MHz is achieved in PDMS coated Kagome HC-PCF, and 8.3±0.9 MHz for the uncoated Kagome HC-PCF.
Abstract We report on the measurement of ground-state atomic polarization relaxation time of Rb vapor confined in five different hypocycloidal core-shape Kagome hollow-core photonic crystal fibers made with uncoated silica glass. We are able to distinguish between wall-collision and transit-time effects in an optical waveguide and deduce the contribution of the atom’s dwell time at the core wall surface. In contrast with conventional macroscopic atomic cell configuration, and in agreement with Monte Carlo simulations, the measured relaxation times were found to be at least one order of magnitude longer than the limit set by atom-wall collisional from thermal atoms. This extended relaxation time is explained by the combination of a stronger contribution of the slow atoms in the atomic polarization build-up, and of the relatively significant contribution of dwell time to the relaxation process of the ground state polarization.
We report on progress in different hollow core photonic crystal fiber (HC-PCF) design and fabrication for atomic vapor based applications. We have fabricated a Photonic bandgap (PBG) guiding HC-PCF with a record loss of 107dB/km at 785nm in this class of fiber. A double photonic bandgap (DPBG) guiding HC-PCF with guidance bands centred at 780nm and 1064nm is reported. A 7-cell 3-ring Kagome HC-PCF with hypocycloid core is reported, the optical loss at 780nm has been reduced to 70dB/km which to the best of our knowledge is the lowest optical loss reported at this wavelength using HC-PCF. Details on experimental loading of alkali metal vapours using a far off red detuned laser are reported. This optical loading has been shown to decrease the necessary loading time for Rb into the hollow core of a fiber. The quantity of Rb within the fiber core has been enhanced by a maximum of 14% through this loading procedure.
This thesis reported on atomic spectroscopy for the development of alkaline atomic vapor photonic microcell (PMC). The work is motivated by reproducing the outstanding laboratory environment based performances achieved in the fields of frequency standard and coherent optics in highly compact and stand-alone devices that can be accessible to a wider scientific community or to a commercial market. In our case these future devices will be based a Hollow-core photonic crystal fiber (HC-PCF) filled with a gas phase material to form a PMC, and outstands with an ultra-long long interaction length and micrometric modal area. However, the micrometric scale of the fiber core harboring the atoms raises several technical and scientific challenges. Among the technical challenges, we list the development of efficient process for atom loading inside long hollow fiber with small core diameter, the suppression or mitigation of physio-chemical reactivity of the atoms (i.e. Rubidium) with the fiber core inner-surface silica etc. In parallel, the large surface-to-volume ratio of the fiber-core raises questions like the coherence relaxation dynamics and the nature and effect of the atom-surface interaction. The thesis reports on fiber-core inner surface coating with different materials to mitigate the physio-chemical reactions of the confined atoms with the surface, on tapering large core inhibited coupling Kagome HC-PCF, and splicing technique that ensures low splice loss and no atomic reactivity during the splicing process. In parallel, the thesis reports on a set of spectroscopy experiments to assess the relaxation dynamics of atoms inside HC-PCF and to report on novel sub-Doppler transparencies.