Exact results for the thermodynamic properties of ensembles of magnetic impurities with randomly distributed host-impurity couplings in the quantum antiferromagnetic Heisenberg model are presented. Exact calculations are done for arbitrary values of temperature and external magnetic field. We have shown that for strong disorder the quenching of the impurity moments is absent. For weak disorder the screening persists, but with the critical non-Fermi-liquid behaviors of the magnetic susceptibility and specific heat. A comparison with disordered Kondo effect experiments in dirty metallic alloys is performed.
In the framework of the exactly solvable model, using nonperturbative methods, the temperature and magnetic field behavior of the NMR relaxation rate (and low-energy dynamical structure factor) for the antiferromagnetic Heisenberg spin-1/2 chain with magnetic impurities is calculated. For a single magnetic impurity, totally screened at low temperatures by spinons of the chain, the critical exponents, which determine the low-temperature and magnetic field behavior, get renormalized. For the finite concentration of impurities with the random distribution of the impurity-chain coupling the weak disorder in the distribution does not produce essential changes to the dynamical structure factor. Contrary, the strong disorder yields drastically different behavior of the low-energy dynamical characteristics, comparing to the homogeneous chain. Our results are generic, and they qualitatively agree in limiting cases with the results of perturbative calculations for disordered spin chains and with the data of experiments on quasi-one-dimensional spin compounds.
In this work we consider several exactly solvable models of magnetic impurities in critical quantum antiferromagnetic spin chains and multichannel Kondo impurities. Their ground-state properties are studied, and the finite set of nonlinear integral equations which exactly describe the thermodynamics of the models is constructed. We obtain several analytical low-energy expressions for the temperature, magnetic field, and frequency dependences of important characteristics of exactly solvable disordered quantum spin models and disordered multichannel Kondo impurities with essential many-body interactions. We show that the only low-energy parameter that gets renormalized is the velocity of the low-lying excitations (or the effective crossover scale connected with each impurity); the others appear to be universal. In our study several kinds of strong disorder important for experiments were used. Some of them produce low divergences in certain characteristics of our strongly disordered critical systems (compared with finite values for the homogeneous case or a single impurity). For weak disorder, or for narrow distributions of the local Kondo temperatures, our exact results reveal the presence of Kondo screening of disordered ensembles of magnetic impurities by low-lying excitations of the host. We point out that our results qualitatively coincide with the data of experiments on real disordered quasi-one-dimensional antiferromagnetic systems and with the similar behavior of some heavy metallic alloys.
We present an exact theory that describes how magnetic impurities change the behavior of the thermal conductivity for the integrable Heisenberg antiferromagnetic quantum spin-1/2 chain. Single magnetic impurities and a large concentration of impurities with similar values of the couplings to the host chain (a weak disorder) do not change the linear-in-temperature low-T behavior of the thermal conductivity: Only the slope of that behavior becomes smaller, compared to the homogeneous case. The strong disorder in the distribution of the impurity-host couplings produces more rapid temperature growth of the thermal conductivity, compared to the linear-in-T dependence of the homogeneous chain and the chain with weak disorder. Recent experiments on the thermal conductivity in inhomogeneous quasi-one-dimensional quantum spin systems manifest qualitative agreement with our results.
We study the effect of anisotropy of spin-
S impurities on an antiferromagnetic SU(2) Heisenberg chain. The magnetic impurities are assumed to have an XXZ-type anisotropic exchange with their neighboring sites. First, using density-matrix renormalization group technique, we examine spin-spin correlation function, instability of N\'eel order, and local spin susceptibility in the presence of a single spin-
S impurity. Based on the results, we find that the types of spin-
S impurities are classified into two groups: (i) nonmagnetic and
S=1 impurities enhance only short-range antiferromagnetic correlation and (ii)
S=21 and
S>1 impurities can, in contrast, stabilize a long-range N\'eel order in the disordered SU(2) Heisenberg chain. Then, we focus on the case of
S=21 impurity as a representative of (ii) and investigate the evolution of some experimentally observable quantities such as magnetization, specific heat, and magnetic susceptibility, as a function of concentration and XXZ anisotropy strength of the impurity. We confirm that the N\'eel order is induced in the bulk spin chain in the presence of finite amount of easy-axis XXZ
S=21 impurities. Furthermore, we recover some of the aforementioned features using cluster mean-field theory, which allows us to present results on experimentally accessible quantities at finite temperatures. Interestingly, in the presence of uniform magnetic field, the total magnetization exhibits a pseudogap behavior for low values of applied field. We also discuss the dependence of NMR spectrum on various XXZ impurities and identify that the spin state of Co impurity in
SrCu0.99Co0.01O2 is
S=23.
We investigate the effect of a unidirectional quenched random field on the anisotropic quantum spin-1/2
XY model, which magnetizes spontaneously in the absence of the random field. We adopt a mean-field approach for this analysis. In general, the models considered have Ising symmetry, and as such they exhibit ferromagnetic order in two and three dimensions in the presence of not too large disorder. Even in the special case when the model without disorder has
U(1) symmetry, a small
U(1)-symmetry-breaking random field induces ferromagnetic long-range order in two dimensions. The mean-field approach, consequently, provides a rather good qualitative and even quantitative description when applied not too close to the criticality. We show that spontaneous magnetization persists even in the presence of the random field, but the magnitude of magnetization gets suppressed due to disorder, and the system magnetizes in the directions parallel and transverse to the random field. Our results are obtained via analytical calculations within a perturbative framework and by numerical simulations. Interestingly, we show that it is possible to enhance a component of magnetization in the presence of the disorder field provided that we apply an additional constant field in the
XY plane. Moreover, we derive generalized expressions for the critical temperature and the scalings of the magnetization near the critical point for the
XY spin system with arbitrary fixed quantum spin angular momentum.