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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Self-induced-transparency soliton propagation under the influence of a far-from-resonance transition line

Victor V. Kozlov, Evald E. Fradkin

Published Jun 10, 1997• 0 citations
Publisher

Abstract

The results of theoretical research of the propagation effect of an ultrashort optical pulse under the conditions of coherent interaction with two resonant transitions are presented. One of the transitions is tuned to exact resonance with the pulse carrier frequency; the other is distanced by much more than the pulse spectral width, thus the adiabatic following approximation may be applied to it. The interaction between the pulse and the far-from-resonance transition is described by the wave equation with the nonlinear index of refraction in the form of the Lorentz function of the field amplitude. This wave equation is solved together with the Bloch equations for the exact resonant transition. The solution in the form of the stationary phase-modulated pulse is obtained, and (pi) -pulse of self-induced transparency is the special case of this solution. The obtained solution has the area under the pulse envelope less than (pi) , and with increasing the absorption coefficient of the far-from-resonance transition the pulse area decreases. The effect can be used for reducing the transparency threshold of the resonant medium below (pi) .

DOI
10.1117/12.276183

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Journal of Physics A Mathematical Nuclear and General•Sep 1, 1973•169 citations
The results of theoretical research of the propagation effect of an ultrashort optical pulse under the conditions of coherent interaction with two resonant transitions are presented. One of the transitions is tuned to exact resonance with the pulse carrier frequency; the other is distanced by much more than the pulse spectral width, thus the adiabatic following approximation may be applied to it. The interaction between the pulse and the far-from-resonance transition is described by the wave equation with the nonlinear index of refraction in the form of the Lorentz function of the field amplitude. This wave equation is solved together with the Bloch equations for the exact resonant transition. The solution in the form of the stationary phase-modulated pulse is obtained, and (pi) -pulse of self-induced transparency is the special case of this solution. The obtained solution has the area under the pulse envelope less than (pi) , and with increasing the absorption coefficient of the far-from-resonance transition the pulse area decreases. The effect can be used for reducing the transparency threshold of the resonant medium below (pi) .
Theoretical research of propagation effect of ultrashort optical pulse under conditions of coherent interaction with two resonant transitions simultaneously is presented. One of the transitions is tuned in exact resonance with pulse carrier frequency; the other is distanced much more than spectral pulse width, thus the adiabatic following approximation may be applied. Interaction between the pulse and far-resonant transition is described by wave equation with nonlinear index of refraction in the form of Lorentz function for field amplitude. This wave equation is solved together with Bloch equations for the exact resonant transition. The solution in the form of stationary phase-modulated pulse is obtained, and 2π-pulse of self-induced - transparency is the special case of this solution. The obtained solution has a square under pulse envelope less than 2π, and with increasing of far-resonant transition absorption coefficient the pulse square decreases. The effect can be used for reducing of the transparency threshold of the resonant medium below pi.
Propagation of a pulse of self-induced transparency in a resonance medium is discussed for the case when it is necessary to take into account the direct electric dipole-dipole interaction between atoms. An equation for the envelope of a wave packet—the sine-Gordon equation—is obtained for the case of durations short compared to ω 0 −1 (ω0 is the transition frequency). The dependence of the velocity and the amplitude of the soliton on the magnitude of the dipole-dipole interaction of atoms is examined in the adiabatic approximation.
The self-induced transparency solution of the Bloch-Maxwell equations is found in the case of inhomogeneously broadened resonant atomic lines and a host medium with a Kerr-type nonlinearity in the index of refraction. The characteristic feature of the solution is that the atomic functions are not factorized. The time dependence of the pulse phase is different from that in the case of a sharp atomic line. In addition to the known term quadratic in the pulse envelope, it contains a term increasing in time, attaining a maximum at the trailing edge of the pulse, and rapidly decreasing afterwards. The average carrier frequency is proportional to the square of the spectral width of the atomic line divided by the squared width of the pulse. A satisfactory solution is found by modulation of the center of the Lorentz distribution function of the purely resonant solutions. It is shown that in the presence of the inhomogeneous broadening the problem cannot be solved by a linear perturbation expansion with respect to the Kerr constant. This method leads to divergencies near the trailing edge of the pulse.
The phenomenon of self-induced transparency (SIT) in the exciton range of the spectrum consists of the propagation through the crystal of solitary wave packets of coherent excitons and photons with anomalous small losses. In the running frame of reference at the site occupied by the soliton a single aperiodic transformation of photons into excitons and a reverse motion of the energy into the field takes place. The solutions of the SIT equations have been received in the slowly-varying amplitude approximation. Taking into account the phase modulation, the authors have shown the appearance of the branch of the carrier wave frequency with anomalous dispersion not only at the given pulse width but at the given pulse amplitude. They have also found the exact solution of the above mentioned equations taking into account the effect of saturation of the dipole momentum transition from the crystal ground state to the exciton state. It leads to the increasing of the soliton time width, to the decreasing of its amplitude and worsens the SIT observation.
Above a critical power threshold for a given pulse width, a short pulse of coherent traveling-wave optical radiation is observed to propagate with anomalously low energy loss while at resonance with a two-quantum-level system of absorbers. The line shape of the resonant system is determined by inhomogeneous broadening, and the pulse width is short compared to dissipative relaxation times. A new mechanism of self-induced transparency, which accounts for the low energy loss, is analyzed in the ideal limit of a plane wave which excites a resonant medium with no damping present. The stable condition of transparency results after the traversal of the pulse through a few classical absorption lengths into the medium. This condition exists when the initial pulse has evolved into a symmetric hyperbolic-secant pulse function of time and distance, and has the area characteristic of a "$2\ensuremath{\pi}$ pulse." Ideal transparency then persists when coherent induced absorption of pulse energy during the first half of the pulse is followed by coherent induced emission of the same amount of energy back into the beam direction during the second half of the pulse. The effects of dissipative relaxation times upon pulse energy, pulse area, and pulse delay time are analyzed to first order in the ratio of short pulse width to long damping time. The analysis shows that the $2\ensuremath{\pi}$ pulse condition can be maintained if losses caused by damping are compensated by beam focusing. In an amplifying inhomogeneously broadened medium an analytic "$\ensuremath{\pi}$ pulse area" solution is presented in the limit of a sharp leading edge of the pulse. The dynamics of self-induced transparency are studied for the particular effects of Doppler velocities upon a resonant gas. The analysis of transparency for random orientations of dipole moments associated with degenerate rotational states yields modified forms of self-induced transparency behavior, which indicates a finite pulse energy loss as a function of distance in some cases. The effect of self-induced transparency on the photon echo is considered. Experimental observations of self-induced transparency have been made in a ruby sample at resonance with a pulsed ruby-laser beam. Single and multiple $2\ensuremath{\pi}$ pulse outputs have been observed, and pulse areas measured in the range of $2\ensuremath{\pi}$. The experimental results are compared with the predictions of the ideal-plane-wave theory. Deviations from the ideal-plane-wave theory are discussed. An analysis is made of the effect of a transverse mode of the propagating beam upon the transparency properties of the pulse.
A more accurate description of the 2 pi pulse of self-induced transparency is obtained. This is an exact solution of an approximate form of the Maxwell-Bloch equations in which only backscattering is neglected; the equations are valid at densities less than about 10 18 atoms cm -3 . At such densities the 2 pi sech pulse of McCall and Hahn (1967, 1969) remains a good approximate well into the picosecond range. The more accurate solution is chirped by a factor proportional to the square of the ratio of the spectral width of the pulse to its carrier wave frequency. The stability of this pulse solution and other N soliton solutions of the approximate Maxwell-Bloch equations is demonstrated.