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Physical Review B

Diffusion Monte Carlo calculation of rate of elastic transmission of a helium vapor beam through a slab of superfluid helium

Y. Lutsyshyn, J. W. Halleý

Published Jan 12, 2011• 3 citations
Publisher

Abstract

We present the results of diffusion Monte Carlo calculations of the elastic transmission of a low-energy beam of helium atoms through a suspended slab of superfluid helium. These calculations represent a significant improvement on variational Monte Carlo methods which were previously used to study this problem. The results are consistent with the existence of a condensate-mediated transmission mechanism, which would result in very fast transmission of pulses through a slab.

DOI
10.1103/physrevb.83.014504

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We present the results of diffusion Monte Carlo calculations of the elastic transmission of a low-energy beam of helium atoms through a suspended slab of superfluid helium. These calculations represent a significant improvement on variational Monte Carlo methods which were previously used to study this problem. The results are consistent with the existence of a condensate-mediated transmission mechanism, which would result in very fast transmission of pulses through a slab.
We report variational Monte Carlo calculations which give amplitudes and phases of the reflected and transmitted components of states representing scattering of helium atoms normally incident on a superfluid 4He{}^{4}\mathrm{He}4He slab. The wave function describes a previously postulated condensate mediated process [J. W. Halley et al., Phys. Rev. Lett. 71, 2429 (1993)] and the results are consistent with uncertainty principle arguments suggesting that the transmission time for thin (but macroscopic) samples will be independent of slab thickness.
In previous work on the interaction of single helium atoms with a slab of superfluid helium the authors found a large amplitude, dependent on the condensate fraction, for transmission with re-emission of a helium atom at the other side of the slab. Here they report a variational formulation of the problem which permits a time dependent calculation and which does not require any perturbation expansion. The variational principle involves a minimization of the expectation value of the square of the difference H-E. They will present preliminary results of a variational Monte Carlo calculation using a simple variational form for the wave function.
We describe a measurement of the transmission probability of 4He atoms through a freely suspended slab of superfluid 4He at low temperatures. In our experiment the slab is realized by using an array of parallel cylindrical holes of diameter 51 microm in a glass disc of thickness 190 microm. By controlling the chemical potential, the holes can be made to fill or empty with liquid, and the surface curvature varied. We have measured the transmission of atom beams, generated by a thin-film heater and detected with a sensitive bolometer, through this structure. The results show that the dominant transmission channel is atom-R+ roton-atom with a probability p approximately 0.12 and that R+ rotons can undergo total internal reflection at the free liquid surfaces.
We show that very low velocity droplets can be used to carry out an experiment to test whether condensate mediated transmission processes can occur in a superfluid droplet of 4He^{4}\mathrm{He}4He. By appropriately choosing the droplet radius and temperature, we can eliminate the competing roton, phonon, and ripplon mediated elastic transmission events. Then a calculation shows that if a few percent or more of the incident atoms experience anomalous condensate mediated transmission, the effects should be detectable in the droplet trajectories. We consider two forms of the experiment, involving a freely falling droplet in ambient vapor in the first instance and an oscillating droplet in a magnetic trap in the second.
Below Tλ = 2.17 K, bulk 4He is a superfluid and has a non-zero Bose-Einstein condensate fraction. This work will focus primarily on how phenomena such as superfluidity, Bose condensation and superfluid vortices are manifested in microscopic, inhomogeneous helium systems. Path Integral Monte Carlo is a powerful method for calculating the equilibrium properties of quantum systems at finite temperature. We have achieved linear scaling of computer time with number of particles through the use of neighbor lists, allowing us to simulate systems of several thousand atoms. We have derived a local superfluid estimator and used it to examine the microscopic superfluid response around a molecule rotating in a helium nanodroplet. We found that the first solvation layer is well-described by a two dimensional superfluid, with thermal excitations occuring at a lower temperature than in bulk helium. The effective moment of inertia of a linear impurity in a helium droplet is calculated, and compared with experimental scattering results. In addition, we calculated the vortex formation energy for both pure droplets and droplets doped with linear impurities, and found that the linear impurities had a negligible impact on the formation energy. A possible spectroscopic signature of vortices in doped helium droplets was suggested. After deriving a local estimator, we calculated the condensate fraction throughout the free helium surface of a semi-infinite slab. These results, along with densitydensity correlation functions, were used to characterize the surface excitations and calculate the extent to which ripplons are present. In addition, the ripplon dispersion relation was calculated using imaginary-time correlation functions, and found to be lll in good agreement with experimental results. Finally, we have calculated the Dey be-Waller factor in solid helium for a range of temperatures and densities, and compared the scaling behavior with the predictions of harmonic theory. The first non-Gaussian contribution to the density distribution was calculated.
We present a phenomenological analysis of an experiment to observe the condensate fraction of helium-4 by firing low-energy pulses of helium atoms at suspended droplets of the superfluid and observing the resulting emission of helium atoms from the fluid. Emission occurs through a conventional process in which rotons are produced and propagate to the other side of the droplet, and through a second process depending on the existence of the condensate. If A is the area of the incoming beam, the cross section scales with A2{\mathit{A}}^{2}A2 (first process) and A4{\mathit{A}}^{4}A4 (second process), respectively, for small A. Aspects of a fully many body calculation and the performance of such an experiment are briefly discussed.