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The Rochester Conferences on Coherence and Quantum Optics and the Quantum Information and Measurement meeting

A short history of Cavity Quantum Electrodynamics

S. Haroche

Published Jan 1, 2007• 9 citations
Publisher

Abstract

Starting with early experiments about lifetimes of excited atoms near metallic boundaries, I review the evolution of Cavity Quantum Electrodynamics in the microwave and in the optical domains. The coherent coupling of single atoms with photons in high-Q cavities has led to the demonstration of fundamental quantum effects in light-matter interaction processes and to the generation of micromasers and microlasers emitting radiation with non-classical properties. It has made possible the development of single photon light sources and efficient detectors of single atoms as well as the implementation of quantum information and communication procedures in which atoms and photons play the roles of quantum bits. Mesoscopic superpositions of field states have been generated by entangling single atoms to fields made of many photons and the decoherence of these states has been studied, shedding new light on the quantum to classical boundary. Cavity Quantum Electrodynamics has also led recently to the quantum non-demolition counting of photons in a cavity, opening new perspectives for studying non-classical states of radiation. These atomic physics experiments are now extended - with promising applications in perspective - to the study of solid-state devices with microcavities built on substrates and coupled to artificial atoms such as quantum dots or superconducting junctions.

DOI
10.1364/cqo.2007.ctuf2

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arXiv:1412.0335•Dec 1, 2014•0 citations
Starting with early experiments about lifetimes of excited atoms near metallic boundaries, I review the evolution of Cavity Quantum Electrodynamics in the microwave and in the optical domains. The coherent coupling of single atoms with photons in high-Q cavities has led to the demonstration of fundamental quantum effects in light-matter interaction processes and to the generation of micromasers and microlasers emitting radiation with non-classical properties. It has made possible the development of single photon light sources and efficient detectors of single atoms as well as the implementation of quantum information and communication procedures in which atoms and photons play the roles of quantum bits. Mesoscopic superpositions of field states have been generated by entangling single atoms to fields made of many photons and the decoherence of these states has been studied, shedding new light on the quantum to classical boundary. Cavity Quantum Electrodynamics has also led recently to the quantum non-demolition counting of photons in a cavity, opening new perspectives for studying non-classical states of radiation. These atomic physics experiments are now extended - with promising applications in perspective - to the study of solid-state devices with microcavities built on substrates and coupled to artificial atoms such as quantum dots or superconducting junctions.
This paper reviews the work on cavity quantum electrodynamics of free atoms. In recent years, cavity experiments have also been conducted on a variety of solid-state systems resulting in many interesting applications, of which microlasers, photon bandgap structures and quantum dot structures in cavities are outstanding examples. Although these phenomena and systems are very interesting, discussion is limited here to free atoms and mostly single atoms because these systems exhibit clean quantum phenomena and are not disturbed by a variety of other effects. At the centre of our review is the work on the one-atom maser, but we also give a survey of the entire field, using free atoms in order to show the large variety of problems dealt with. The cavity interaction can be separated into two main regimes: the weak coupling in cavity or cavity-like structures with low quality factors Q and the strong coupling when high- Q cavities are involved. The weak coupling leads to modification of spontaneous transitions and level shifts, whereas the strong coupling enables one to observe a periodic exchange of photons between atoms and the radiation field. In this case, atoms and photons are entangled, this being the basis for a variety of phenomena observed, some of them leading to interesting applications in quantum information processing. The cavity experiments with free atoms reached a new domain with the advent of experiments in the visible spectral region. A review on recent achievements in this area is also given.
The physics of strong light-matter coupling has been addressed in different scientific communities over the last three decades. Since the early eighties, atoms coupled to optical and microwave cavities have led to pioneering demonstrations of cavity quantum electrodynamics, Gedanken experiments, and building blocks for quantum information processing, for which the Nobel Prize in Physics was awarded in 2012. In the framework of semiconducting devices, strong coupling has allowed investigations into the physics of Bose gases in solid-state environments, and the latter holds promise for exploiting light-matter interaction at the single-photon level in scalable architectures. More recently, impressive developments in the so-called superconducting circuit QED have opened another fundamental playground to revisit cavity quantum electrodynamics for practical and fundamental purposes. This book aims at developing the necessary interface between these communities, by providing future researchers with a robust conceptual, theoretical and experimental basis on strong light-matter coupling, both in the classical and in the quantum regimes. In addition, the emphasis is on new forefront research topics currently developed around the physics of strong light-matter interaction in the atomic and solid-state scenarios.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
In cavity-quantum-electrodynamics experiments, two-level Rydberg atoms and single-photon microwave fields can be seen as qubits. Quantum gates based on resonant and dispersive atom-field effects have been realized, which implement various kinds of conditional dynamics between these qubits. We have also studied the interaction between a single atom and coherent fields stored in the cavity. By progressively increasing the number of photons in these fields, we have explored various aspects of the quantum-classical boundary. We have realized a complementarity experiment demonstrating the continuous evolution of an apparatus from a quantum to a classical behaviour. We have also prepared 'Schrödinger-cat'-like states of the field made of a few photons, and observed their decoherence. We present a brief review of these experiments along with a proposal to study larger systems, i.e. coherent fields with more photons. Fundamental limits to the size of mesoscopic superpositions of field states in a cavity will be briefly discussed.
After they have interacted, quantum particles generally behave as a single nonseparable entangled system. The concept of entanglement plays an essential role in quantum physics. We have performed entanglement experiments with Rydberg atoms and microwave photons in a cavity and tested quantum mechanics in situations of increasing complexity. Entanglement resulted either from a resonant exchange of energy between atoms and the cavity field or from dispersive energy shifts affecting atoms and photons when they were not resonant. With two entangled particles (two atoms or one atom and a photon), we have realized new versions of the Einstein-Podolsky-Rosen situation. The detection of one particle projected the other, at a distance, in a correlated state. This process could be viewed as an elementary measurement, one particle being a ‘‘meter’’ measuring the other. We have performed a ‘‘quantum nondemolition’’ measurement of a single photon, which we detected repeatedly without destroying it. Entanglement is also essential to understand decoherence, the process accounting for the classical appearance of the macroscopic world. A mesoscopic superposition of states (‘‘Schrodinger cat’’) gets rapidly entangled with its environment, losing its quantum coherence. We have prepared a Schrodinger cat made of a few photons and studied the dynamics of its decoherence, in an experiment which constitutes a glimpse at the quantum/classical boundary. We have also investigated entanglement as a resource for the processing of quantum information. By using quantum two-state systems (qubits) instead of classical bits of information, one can perform logical operations exploiting quantum interferences and taking advantage of the properties of entanglement. Manipulating as qubits atoms and photons in a cavity, we have operated a quantum gate and applied it to the generation of a complex three-particle entangled state. We finally discuss the perspectives opened by these experiments for further fundamental studies.
Since the photon box gedanken experiments of several of the founding fathers of modern physics, considerable progress has been made in differentiating the quantum and classical worlds. In this pursuit, the cavity as an open quantum system has been indispensable. From the quantization of the atom and field within a superconducting cavity, a unique realm of EPR type entanglement has emerged. In this way, dynamical evolution of the system in the strong coupling regime is intimately tied with the coupling of an atom with a single resonant or non-resonant mode within the cavity. More specifically, the cavity can be prepared so that the atom is detected in a desired state. Here, the essentials of the strong coupling regime of Cavity Quantum Electrodynamics (QED) are reviewed for cavities tuned with a single atomic transition. A brief introduction of the systems is followed by an approach of the more striking effects, leading towards Ramsey Interferometry and Quantum Non-Demolition measurements as means for quantum gate protocol. Because the integrity of the atom and photon states is important for the advancement of quantum computation, a brief discussion of the decoherence problems is also presented. This document is meant to introduce the topic in a way that makes it easily accessible to those working in closely related areas of physics, and to highlight key applications and some basic questions concerning decoherence and the measurement problem.