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Physica B+C

Dynamical correlation functions for linear spin chains

Gerhard Müller, H. Beck

Published Jan 1, 1977• 1 citation
Publisher
DOI
10.1016/0378-4363(77)90808-7

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Dynamical spin correlation functions in (q, omega )-space are calculated numerically for linear quantum-mechanical Heisenberg systems containing up to ten spins with s= 1 / 2 and s=1. The authors consider ferro- and antiferromagnets including single-site and exchange anisotropies. They compare their results with various other theoretical treatments and draw conclusions for the dynamics of infinite chains. In the case of the s=1 planar Heisenberg ferromagnet direct comparison is made with inelastic neutron scattering cross sections of CsNiF 3 . The theoretical and experimental results are in good agreement.
We present the exact solution for the full dynamics of a nonequilibrium spin chain and its dual reaction-diffusion model, for arbitrary initial conditions. The spin chain is driven out of equilibrium by coupling alternating spins to two thermal baths at different temperatures. In the reaction-diffusion model, this translates into spatially alternating rates for particle creation and annihilation, and even negative "temperatures" have a perfectly natural interpretation. Observables of interest include the magnetization, the particle density, and all correlation functions for both models. Two generic types of time dependence are found: if both temperatures are positive, the magnetization, density, and correlation functions decay exponentially to their steady-state values. In contrast, if one of the temperatures is negative, damped oscillations are observed in all quantities. They can be traced to a subtle competition of pair creation and annihilation on the two sublattices. We comment on the limitations of mean-field theory and propose an experimental realization of our model in certain conjugated polymers and linear chain compounds.