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The Journal of Chemical Physics

A new quantum control scheme for multilevel systems based on effective decomposition by intense laser fields

Michihiko Sugawara

Published Mar 4, 2009• 4 citations
Publisher

Abstract

A new quantum control scheme for general multilevel systems using intense laser fields is proposed. In the present scheme, the target subspace consisting of several quantum levels is effectively isolated by applying intense cw lasers with specific conditions. The formulation is carried out using the Green function with the help of projection operator method. Dynamics of the isolated target subspace is governed by an effective Hamiltonian. The developed scheme is applied to the quantum control of dissipative four- and five-level systems. It is clarified that the present method makes it possible not only to manipulate the coherent population dynamics but also to suppress the dissipative dynamics.

DOI
10.1063/1.3079327

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A new quantum control scheme for general multilevel systems using intense laser fields is proposed. In the present scheme, the target subspace consisting of several quantum levels is effectively isolated by applying intense cw lasers with specific conditions. The formulation is carried out using the Green function with the help of projection operator method. Dynamics of the isolated target subspace is governed by an effective Hamiltonian. The developed scheme is applied to the quantum control of dissipative four- and five-level systems. It is clarified that the present method makes it possible not only to manipulate the coherent population dynamics but also to suppress the dissipative dynamics.
We propose a new scheme for quantum dynamics control of multilevel system using intense lasers. To do so, we apply intense CW lasers to create a strongly coupled subsystem with which one can make the complementary space effectively isolated, and we apply the established control schemes to the isolated subsystem. We have also obtained an effective Hamiltonian for the target subsystem with the help of the second-order perturbation theory. Numerical demonstrations on model systems show that the present decomposition scheme effectively works for population dynamics control. It is also found that relaxation processes can be suppressed under the proposed scheme.
A quantum control scheme for multilevel systems utilizing effective decomposition is proposed. In this method, a subsystem chosen for control target is effectively isolated by irradiating intense continuous-wave laser fields onto the complimentary space. By choosing the control target space consisting of small number of eigenstates, effective dressed states for the isolated space are analytically given, which makes it possible to express the performance index defined in the target space as an explicit function of laser parameters. Then, designing the control field can be treated as a static parameter optimization. The present scheme makes it possible not only to optimize the laser parameters but also to investigate the parameter search space, which clarifies the physics of the control process.
A scheme to drive and manipulate a finite-dimensional quantum system in decoherence-free subspaces (DFSs) by Lyapunov control is proposed. Control fields are established by the Lyapunov function. This proposal can drive the open quantum system into DFSs and manipulate it to any desired eigenstate of the free Hamiltonian. An example which consists of a four-level system with three long-lived states driven by two lasers is presented to demonstrate the scheme. We have performed numerical simulations of the dynamics of the four-level system, which show that the scheme works well.
Possibility of coherent control of spontaneous emission from four- and five-level systems in the laser radiation field is studied. The four-level system consists of two levels resonantly driven by laser radiation where either of levels may decay to a separate level. For such a system we show that the presence of the second decay channel may deteriorate the destructive interference occurring because of Autler-Townes effect in case of one decay channel. The five-level system represents two two-level resonantly driven systems with the upper levels decaying to a common level. For this case, the interference between the two decay channels is partially or completely destructive or constructive depending on the initial conditions and on the mutual orientation of the transition dipole moments. It is shown that population transfer takes place by the same quantum vacuum via spontaneous emission. The populations are shown to have damping oscillatory nature.
A general local control theory for manipulating quantum system dynamics is developed. Basic concept of the present theory is lying in the realization of monotonous increasing condition of the performance index, which is locally (in time domain) defined to major how the present quantum state satisfies the current objective. The local control field is designed to satisfy the above condition taking into account the equation of motion of the system. It is found, through the formulation, that the monotonous increasing condition can be achieved as long as the performance index is given as a function of expectation values of time-dependent observable operators, whose equation of motion is governed by the field-free system Hamiltonian or Liouvillian. It is also shown that the present theory is a generalization of the local optimization approach which has been successfully applied to many of molecular dynamics control problems. As for the special cases, performance indices for “transition path control,” “population distribution control,” and “wave packet shaping” are proposed. The theory is applied to vibrational control problems of the one-dimensional model system of hydrogen fluoride. The results show that the present method works effectively for the population dynamics control as well as the wave packet shaping.
We present a scheme to drive a finite-dimensional quantum system into the decoherence-free subspaces (DFS) by Lyapunov control. Control fields are established by Lyapunov function. This proposal works well for both closed and open quantum systems, with replacing the DFS by desired subspaces for closed systems. An example which consists of a four-level system with three degenerate states driven by three lasers is presented to gain further insight on the scheme. Numerical simulations for the dynamics of the system are performed and the results are good.