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Physical Review A

Intrinsic optical bistability for coated spheroidal particles

Nauzer Kalyaniwalla, Joseph W. Haus, R. Inguva, Meyer H. Birnboim

Published Nov 1, 1990• 81 citations
Publisher

Abstract

We present results on the nonlinear-optical response for a series of dielectric particles having nanometer sizes that are coated with a metallic shell. Using the freedom of changing particle shapes and coating thicknesses, we optimize the threshold intensity for intrinsic optical bistability. The metallic shell creates an enhanced local field in the nonlinear core. We report threshold intensities for silver-coated CdS as low as 12 W/${\mathrm{cm}}^{2}$.

DOI
10.1103/physreva.42.5613

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We present results on the nonlinear-optical response for a series of dielectric particles having nanometer sizes that are coated with a metallic shell. Using the freedom of changing particle shapes and coating thicknesses, we optimize the threshold intensity for intrinsic optical bistability. The metallic shell creates an enhanced local field in the nonlinear core. We report threshold intensities for silver-coated CdS as low as 12 W/cm2{\mathrm{cm}}^{2}cm2.
We provide a self-consistent mean field approximation in the framework of Mie scattering theory to study the optical bistability of a metallic nanoparticle coated with a nonlinear shell. We demonstrate that the nanoparticle coated with a weakly nonlinear shell exhibits optical bistability in a broad range of incident optical intensity. This optical bistability critically relies on the geometry of the shell-coated nanoparticle, especially the fractional volume of the metallic core. The incident wavelength can also affect the optical bistability. Through an optimization-like process, we find a design with broader bistable region and lower threshold field by adjusting the size of the nonlinear shell, the fractional volume of the metallic core, and the incident wavelength. These results may find potential applications in optical bistable devices such as all-optical switches, optical transistors and optical memories.
We study the nonlinear optical response of graphene in nanostructures. The spherical nanoparticle coated with a monolayer of graphene displays enhanced optical Kerr nonlinearity and, consequently, optical bistability and multistability in a broad range of incident optical intensity. This optical bistability significantly appertains on the geometry of the shell-coated nanoparticle, the fractional volume of the metallic core, as well as the core genre and Fermi energy of graphene. In particular, Fermi energy could also affect the optical bistability and induce switching from optical bistability to optical multistability. Due to the importance of core–shell nanoparticles, this model may find potential applications in optical bistable devices such as all-optical switches, optical transistors, and memories.
The intrinsic optical bistability (OB) of graded core-shell granular composites is investigated. The coated particles are made of cores with gradient dielectric function ∊ c (r) = A(r/a) k and nonlinear shells. In view of the exponential distribution of the core dielectric constant, the potential functions of each region are obtained by solving the Maxwell equations, and the mathematical expressions of electric field in the shells and cores are determined. Numerical study reveals that the optical bistable threshold and the threshold width of the composite medium are dependent on the shell thickness, core dielectric exponent, and power function coefficient. The optical bistable width increases with the decreasing shell thickness and the power exponent and with the increasing power function coefficient.
The optical properties of a new class of composite nonlinear materials composed of coated grains, such as cadmium sulfide with a silver coating, are examined. These materials exhibit intrinsic optical bistability and resonantly enhanced conjugate reflectivity. The threshold for intrinsic optical bistability is low enough for practical applications in optical communications and optical computing. Some problems associated with the fabrication of these materials are addressed. Based on preliminary results, switching times are expected to be in the subpicosecond range.
We studied the intrinsic optical bistability(OB) of coated spherical particles with graded dielectric profiles.According to Maxwell equations, we obtained the spatial average of the local field in the core as a function of the external applied field. Numerical results for power-law graded profiles show that the optical bistable behavior is dependent on the shell thickness and the power-laws exponent k. The interval of optical bistability increases with increasing shell thickness or increasing k. In addition, the field-dependent reflectance at normal incidence R in random composites is also investigated, and a hysteretic loop is observed.