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Physical Review Letters

Superradiance and Subradiance in an Inhomogeneously Broadened Ensemble of Two-Level Systems Coupled to a Low- Q Cavity

Vasily V. Temnov, U. Woggon

Published Dec 6, 2005• 170 citations
Publisher

Abstract

The collective spontaneous emission of a fully inverted inhomogeneously broadened ensemble of N two-level systems coupled to a single-mode low-Q cavity is investigated numerically using Monte Carlo wave function technique. An intrinsically bi-exponential emission dynamics is found when the time scales of superradiance tau(sr) and inhomogeneous dephasing T2* approximately 1/Deltaomega(inh) become comparable: a fast superradiant is followed by a slow subradiant decay. Experimental configurations using ensembles of quantum dots coupled to optical microcavities are proposed as possible candidates to observe the combined superradiant and subradiant energy relaxation.

DOI
10.1103/physrevlett.95.243602

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The collective spontaneous emission of a fully inverted inhomogeneously broadened ensemble of N two-level systems coupled to a single-mode low-Q cavity is investigated numerically using Monte Carlo wave function technique. An intrinsically bi-exponential emission dynamics is found when the time scales of superradiance tau(sr) and inhomogeneous dephasing T2* approximately 1/Deltaomega(inh) become comparable: a fast superradiant is followed by a slow subradiant decay. Experimental configurations using ensembles of quantum dots coupled to optical microcavities are proposed as possible candidates to observe the combined superradiant and subradiant energy relaxation.
We study the spontaneous emission from a regular lateral array or a randomly distributed ensemble of quantum dots under strong excitation (full inversion) conditions.We focus on the similarities and dierences between the cases of random and regular arrangement of the dots and show that there is very little dierence between the evolution of luminescence in these two cases, both for identical dots and for a realistically inhomogeneously broadened ensemble.This means that the enhanced emission or superradiance eect is not due to accidental clustering of pairs of dots.Moreover, we point out that observation of an enhanced emission under weak excitation does not prove that true superradiance will develop in a fully inverted system.
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Cooperative effects such as super(or sub)radiance in quantum systems arise from the interplay among quantum emitters. While bright superradiant states have been extensively studied and have yielded important insights into cooperative phenomena, subradiant states remain less explored due to their inherently dark state nature. However, subradiance holds significant potential as a valuable quantum resource exploiting long-lived and large-scale entanglement, which is a key for advancing quantum information technologies. Here, we demonstrate strong collective emission from a cavity-mediated steady-state subradiant state. In a tailored photonic environment with balanced cavity dissipation, emitter-field coupling strength, and incoherent pumping, two quantum dots coupled to a low-Q cavity exhibit a steady-state population in a subradiant state with a highly negative cooperativity parameter among the emitters. As a key signature of steady-state subradiance, the system shows strong photon bunching ( g(2)(0)>8{{{\rm{g}}}}^{\left(2\right)}\left(0\right) > 8g(2)(0)>8 ) and suppressed single-photon decay (36 ns). Furthermore, we investigate that such collective interactions can be manipulated by controlling various system parameters, such as detuning and dephasing, supported by numerical simulations. Our approach to inducing cavity-mediated subradiance paves the way for generating and harnessing quantum correlations among quantum emitters via controlled dissipation. Subradiance is a cooperative effect in systems of quantum emitters, which is the opposite of superradiance, or enhanced emission, but has been less explored. Here, the authors demonstrate a steady-state subradiant state in a system of two InAs quantum dots coupled to a low-Q nanophotonic cavity.
Emission spectra of quantum dot arrays in zero-dimensional microcavities are studied theoretically. It is shown that their form is determined by the competition between collective superradiant mode formation and inhomogeneous broadening. A random sources method is used to calculate the photoluminescence spectra from an nonresonant pumped microcavity, and a standard diagram technique is used to provide a microscopic justification for the random sources method. The emission spectra of a microcavity are analyzed taking into account the spread of exciton energy due to inhomogeneous distribution of quantum dots and tunneling between them. It is demonstrated that the luminescence spectra of strongly tunnel-coupled quantum dots are sensitive to the dot positions, and the collective mode can (under certain conditions) be stabilized by random tunneling links.
We study the collective decay of an initially inverted ensemble of two-level emitters in two distinct scenarios: when coupled to a squeezed photonic reservoir and when interacting with a one-dimensional waveguide. Using a quantum-state diffusion approach to unravel the emission process, we investigate entanglement and classical correlations along individual quantum trajectories over time. This numerical analysis shows that despite an initial buildup of entanglement and a significant amount of entanglement due to either spin squeezing or dark states at late times, the essential features of the superradiant burst are well described by averages over fully factorizable states. We explain this observation in terms of an almost complete factorization of all 2-local observables, which we identify as a generic property of superradiant decay. Based on this insight, we provide a purely classical theory for the burst in squeezed superradiance, which is both intuitive and exact for a large number of emitters. Moreover, we find that our numerical approach also performs well in the presence of subradiant states, which dominate the slow residual decay of nonuniform ensembles at late times.