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Photonics and Micro- and Nano-structured Materials

Quantum optics with atomic polaritons

Evgeny S. Sedov, Igor Yu. Chestnov, Igor O. Barinov, A. P. Alodjants, Sergei M Arakelyan

Published Jan 20, 2012• 0 citations
Publisher

Abstract

The interaction of a two-level atomic ensemble with a quantized single mode electromagnetic field in the presence of optical collisions is theoretically investigated. The main accent is made on achieving thermal equilibrium for coupled atom-light states (in particular dressed states). We propose a model of atomic dressed state thermalization that accounts for the evolution of the pseudo-spin Bloch vector components and characterize the essential role of the spontaneous emission rate in the thermalization process. Our model shows that the time of thermalization of the coupled atom-light states strictly depends on the ratio of the detuning and the resonant Rabi frequency. The predicted time of thermalization is in the nanosecond domain and about ten times shorter than the natural lifetime of rubidium D-lines.

DOI
10.1117/12.923617

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The interaction of a two-level atomic ensemble with a quantized single mode electromagnetic field in the presence of optical collisions is theoretically investigated. The main accent is made on achieving thermal equilibrium for coupled atom-light states (in particular dressed states). We propose a model of atomic dressed state thermalization that accounts for the evolution of the pseudo-spin Bloch vector components and characterize the essential role of the spontaneous emission rate in the thermalization process. Our model shows that the time of thermalization of the coupled atom-light states strictly depends on the ratio of the detuning and the resonant Rabi frequency. The predicted time of thermalization is in the nanosecond domain and about ten times shorter than the natural lifetime of rubidium D-lines.
The interaction of a two-level atomic ensemble with a quantized single-mode electromagnetic field in the presence of optical collisions is investigated both theoretically and experimentally. The main focus is on achieving thermal equilibrium for coupled atom-light states (in particular dressed states). We propose a model of atomic dressed-state thermalization that accounts for the evolution of the pseudo-spin Bloch vector components and characterize the essential role of the spontaneous emission rate in the thermalization process. Our model shows that the time of thermalization of the coupled atom-light states depends strictly on the ratio of the detuning to the resonant Rabi frequency. The predicted time of thermalization is in the nanosecond domain at full optical power and about 10 times shorter than the natural lifetime in our experiment. Experimentally we investigate the interaction of the optical field with rubidium atoms in an ultrahigh-pressure buffer gas cell under the conditions of large atom-field detuning comparable to the thermal energy in frequency units. In particular, an observed asymmetry of the saturated lineshape is interpreted as evidence of thermal equilibrium of coupled atom-light states.
We consider the fundamental problem of high-temperature phase transitions in the system of high-density two-level atoms off-resonantly interacting with a pump field in the presence of optical collisions (OCs) and placed in the cavity. OCs are considered in the framework of thermalization of atomic dressed-state (DS) population. For the case of a strong atom-field coupling condition, we analyze the problem of a thermodynamically equilibrium superradiant phase transition for the order parameter representing a real amplitude of cavity mode and taking place as a result of the atomic DSs thermalization process. Such a transition is also connected with condensed (coherent) properties of low branch DS polaritons occurring in the cavity. For describing nonequilibrium phase transitions we derive Maxwell-Bloch--like equations which account for cavity decay rate, collisional decay rate, and spontaneous emission. Various aspects of transitions to laser field formation by using atomic DS levels for both positive and negative detuning of a pump field from atomic transition frequency are studied in detail. It is revealed that for positive atom-light detuning DS lasing can be obtained in the presence of quasiequilibrium DS population that corresponds to a true two-level atomic system with the inversion in a nonresonant limit.
The problem of photonic phase transition for the system of a two-level atomic ensemble interacting with a quantized single-mode electromagnetic field in the presence of optical collisions (OCs) is considered. We have shown that for large and negative atom-field detuning a photonic field exhibits high-temperature second-order phase transition to superradiant state under thermalization condition for coupled atom-light states. Such a transition can be connected with superfluid (coherent) properties of photonlike low branch (LB) polaritons. We discuss the application of metallic cylindrical waveguide for observing predicted effects.
The problem of phase transitions in the system of high-density gas of two-level atoms non-resonantly interacting with a pump field in the presence of optical collisions (OCs) and placed in the cavity is studied. The OCs are considered in the framework of thermalization of atomic dressed state (DS) population. For the case of a strong atom-field coupling condition we analyze the problem of thermodynamic equilibrium superradiant phase transition for the order parameter representing real amplitude of cavity mode and taking place as a result of the atomic DS thermalization process. At the same time such a transition can be connected with condensed (coherent) properties of low branch DS-polaritons occurring in the cavity. Various aspects of non-equilibrium phase transition to laser field generation by using atomic DS levels are studied in detail. It is important that for positive atom-light detuning DS lasing can be obtained in the presence of quasi-equilibrium DS population that corresponds to a true two-level atomic system with inversion in perturbative limit.
Abstract We investigate a hybrid quantum system consisting of two coupled optical cavities, each containing an ensemble of coherently pumped artificial or real two-level atoms. The system is modelled within the dressed-state formalism, accounting for coherent driving and dissipative interactions with independent electromagnetic reservoirs. Focusing on the regime where the Rabi frequency greatly exceeds the collective spontaneous emission and cavity decay rates, respectively, we derive the equations of motion characterizing the system and analyse its steady-state behaviours. Special attention is given to the scenario in which only one cavity contains a pumped multi-atom ensemble, and as a consequence, coherent excitation transfer to the second cavity occurs via cavity–cavity coupling. In this case, the mean photon number in the second cavity mode scales proportional to the squared number of atoms, i.e., N2 from the first cavity. The proposed model offers insight into light–matter interaction in composite systems and suggests viable mechanisms for engineering collective interactions and non-local excitation transport in quantum optical platforms.