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Physical Review A

Nonperturbative Analysis of the Resonant Interaction between a Linear and a Nonlinear Oscillator

I. R. Senitzky

Published Jan 1, 1971• 41 citations
Publisher

Abstract

The consideration of the resonant interaction between a linear harmonic oscillator (LO) and a (nonlinear) angular momentum oscillator (NO) is motivated by its relation to the interaction between a field mode and a number of atomic systems, its relation to the interaction between three field modes, and the appearance of qualitatively different results quantum mechanically and classically even in cases that can be regarded as macroscopic. The analysis is carried out both classically and quantum mechanically in the rotating-wave approximation, and the time dependence of the energies of the two oscillators is examined, mainly by means of a nonlinear differential equation for the NO energy. In the classical analysis, the problem turns out to be identical to that of a spherical pendulum, where the NO energy ${L}_{3}$ corresponds to the pendulum potential energy, the LO energy $n$ corresponds to the pendulum kinetic energy, and the coupling energy between the two oscillators $\frac{1}{2}\frac{\ensuremath{\gamma}K}{\ensuremath{\omega}}$ is proportional to the angular momentum $K$ of the pendulum about the vertical axis, all quantities being expressed in suitable units. A solution for ${L}_{3}(t)$ is obtained, and is shown to be described uniquely, apart from a shift in the time origin, by the constants of motion $E(\ensuremath{\equiv}{L}_{3}+n)$ and $K$. ${L}_{3}$ oscillates periodically, except for the "unstable-equilibrium" solution and the "conical-pendulum" solution. The quantum-mechanical problem is solved exactly for the cases in which the NO is a two-level system and a three-level system, and certain aspects of the exact solution are derived in the case of a four-level system. The constants $E$ and $K$ become a complete set of quantum numbers. It is found that unstable equilibrium, in the sense that $〈{L}_{3}〉$ is constant, does not exist, because of spontaneous emission; it is also found that $〈{L}_{3}〉$ oscillates sinusoidally for the two-level system, oscillates periodically but not sinusoidally for the three-level system, and oscillates aperiodically for a four- or higher-level system, conclusions about the higher-level systems coming from general considerations and numerical solutions found in the literature. Approximate solutions for NO' s with arbitrarily large numbers of levels are obtained. One method of approximation displays spontaneous emission but not aperiodicity. Another approximate method, which contains the statistical spread of the initial phase difference between the oscillations of the two oscillators inherent in the uncertainty principle, displays both spontaneous emission and aperiodicity. It is shown that the aperiodicity - a property which does not exist classically for precise initial conditions - does not disappear even in the macroscopic limit and is due to the averaging performed, in taking the quantum-mechanical expectation value, over an ensemble of periodic oscillations with a spread in frequencies.

DOI
10.1103/physreva.3.421

Related papers

Interaction between a Nonlinear Oscillator and a Radiation Field

I. R. Senitzky

The behavior of a nonlinear oscillator (NO) coupled to a radiation field is investigated. The NO considered is an angular momentum oscillator, of energy $\ensuremath{\hbar}\ensuremath{\omega}{L}_{3}$, that describes the collective effect of a number of identical two-level (or spin-\textonehalf{}) systems under given idealized conditions, a large total angular momentum quantum number ${L}_{0}$ corresponding to a large number of two-level systems. The field is described by a set of modes. Free decay---with the NO initially excited and the radiation field in the ground state---and forced oscillation---with the NO subject to a prescribed resonant driving field---are studied. The analysis is performed both classically and quantum mechanically, using the classical and Heisenberg equations of motion, respectively, so as to display explicitly the difference in the results. Interest in the comparison between the two formalisms is motivated by the expectation that for large ${L}_{0}$, the NO should behave essentially classically, except near its highest-energy state in the absence of a driving field. The general equations of motion are reduced to equations for the NO variables only. In the classical analysis of free decay, expressions for the energy and oscillating coordinates are derived. The decay time is shown to approach infinity as ${L}_{3}(0)$ approaches ${L}_{0}$ (the limiting condition being that of unstable equilibrium) and the radiative frequency shift is shown to be approximately proportional to ${L}_{3}(t)$. It is also shown that use of the rotating-wave approximation alters qualitatively the expression for the frequency shift. In the classical analysis of forced oscillation, approximate results are obtained for a weak driving field and a strong driving field, the NO being initially in the ground state. The weakfield results exhibit a monotonic approach of ${L}_{3}(t)$ to a constant (negative) value---or steady state---at which the power absorbed equals the power radiated; in the strong-field case, ${L}_{3}(t)$ oscillates periodically between the limits $\ifmmode\pm\else\textpm\fi{}{L}_{0}$, the coupling to the radiation field having negligible effect on the frequency of this oscillation. In the quantum-mechanical analysis, the equations of motion become simplified for ${L}_{0}=\frac{1}{2}$, and this case is treated first. The free-decay results are essentially similar to those of the Weisskopf-Wigner theory, exhibiting an exponential decay of $〈{L}_{3}(t)〉$ and a radiative frequency shift in the oscillating coordinates. Under forced oscillation, with $〈{L}_{3}(0)〉=\ensuremath{-}{L}_{0}, 〈{L}_{3}(t)〉$ approaches a constant value either monotonically, if the driving field is sufficiently weak, or by means of a damped oscillation, if the driving field is strong. For ${L}_{0}>\frac{1}{2}$, the free decay is treated by a method that involves the derivation of a set of expressions for the $k\mathrm{th}$ derivative of $〈{L}_{3}(t)〉$ as an expectation value of a polynomial in ${L}_{3}$ of order $k+1$. This set, together with the eigenvalue equation for ${L}_{3}$, is shown to lead to a solution for all the moments of ${L}_{3}$. The method is used to obtain complete solutions for several low values of ${L}_{0}$, and also to obtain initial derivatives of $〈{L}_{3}(t)〉$ as polynomials in ${L}_{0}$ for $〈{L}_{3}(0)〉={L}_{0}$. For large ${L}_{0}$, a comparison of classical and quantum-mechanical equations shows that only the condition $〈{L}_{3}(0)〉\ensuremath{\approx}{L}_{0}$ requires quantum-mechanical treatment, and that for a short time only. 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Physical Review A•Sep 1, 1972•41 citations

Quantum-Mechanical Aperiodicity in the Resonant Interaction between a Field Mode and a Spin System

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Physical Review•Jul 25, 1969•6 citations

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A field theoretical formulation of the rather easy problem of N identical, one-dimensional bosons, interacting pairwise via harmonic oscillator potentials of equal force constants is given, in a way similar to the way the nonlinear Schrodinger model provides a field theoretical formulation of a one-dimensional, delta -function Bose gas. The nonlinear integro-differential equation obtained for the complex scalar field of the model is treated classically, and solved in the semiclassical limit of a large number of particles. Working in the centre of mass frame of the field, a sequence of operators that would raise or lower the energy of a state by definite amounts without changing its particle number are constructed from certain bilinear expressions in the field. These operators have, in the limit of a large number of particles, commutation relations similar to those of the Fourier modes of a compact free field, except that the first mode is missing as a result of the fact that the field in the centre of mass frame is subject to the obvious constraint that its centre of mass always coincides with the coordinate origin. The quantum states can be labelled by the total centre of mass momentum, and the quasi-particle numbers in each of the independent oscillator modes. The energy spectrum of the system is calculated, giving the same results as the exact, quantum-mechanical N-body analysis.

Journal of Physics A Mathematical and General•Oct 7, 1993•1 citation

Interaction of a quantum system with a strong oscillating field

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The problem of the interaction of a quantum system having discrete states, with a classical oscillating field, is reexamined as a problem in the solution of the time-dependent Schrodinger equation with a periodic Hamiltonian. A method is presented for approximating the time-dependent Hamiltonian with a time-independent one in the weak oscillating field case. With the aid of Floquet's theorem the problem is exactly converted to one with a time-independent Hamiltonian represented by an infinite matrix. The approximation of only two states then permits finding the resonance line shape by perturbation theory for both single and multiple quantum transitions with equal ease. The simple case of only two states connected by an off diagonal sinusoidal perturbation is studied in detail, and a complete description of the average transition probability is found for the strong oscillating field case. A few more complex cases are discussed. A deeper understanding of the analysis is obtained by examining the theory with the oscillating field quantized. Experimental verification of the theory could best be obtained by the methods of atomic beam spectroscopy at radio frequencies.

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Complete description of the classical and quantum dynamics of a particle in an anisotropic, rotating, harmonic trap is given. The problem is studied in three dimensions and no restrictions on the geometry are imposed. In the generic case, for an arbitrary orientation of the rotation axis, there are two regions of instability with different characteristics. The analysis of the quantum-mechanical problem is made simple due to a direct connection between the classical mode vectors and the quantum-mechanical wave functions. This connection is obtained via the matrix Riccati equation that governs the time evolution of squeezed states of the harmonic oscillator. It is also shown that the inclusion of gravity leads to a resonant behavior -- the particles are expelled from the trap.

arXiv:quant-ph/0409070•Sep 13, 2004•1 citation
The consideration of the resonant interaction between a linear harmonic oscillator (LO) and a (nonlinear) angular momentum oscillator (NO) is motivated by its relation to the interaction between a field mode and a number of atomic systems, its relation to the interaction between three field modes, and the appearance of qualitatively different results quantum mechanically and classically even in cases that can be regarded as macroscopic. The analysis is carried out both classically and quantum mechanically in the rotating-wave approximation, and the time dependence of the energies of the two oscillators is examined, mainly by means of a nonlinear differential equation for the NO energy. In the classical analysis, the problem turns out to be identical to that of a spherical pendulum, where the NO energy L3{L}_{3}L3​ corresponds to the pendulum potential energy, the LO energy nnn corresponds to the pendulum kinetic energy, and the coupling energy between the two oscillators 12\ensuremathγK\ensuremathω\frac{1}{2}\frac{\ensuremath{\gamma}K}{\ensuremath{\omega}}21​\ensuremathω\ensuremathγK​ is proportional to the angular momentum KKK of the pendulum about the vertical axis, all quantities being expressed in suitable units. A solution for L3(t){L}_{3}(t)L3​(t) is obtained, and is shown to be described uniquely, apart from a shift in the time origin, by the constants of motion E(\ensuremath≡L3+n)E(\ensuremath{\equiv}{L}_{3}+n)E(\ensuremath≡L3​+n) and KKK. L3{L}_{3}L3​ oscillates periodically, except for the "unstable-equilibrium" solution and the "conical-pendulum" solution. The quantum-mechanical problem is solved exactly for the cases in which the NO is a two-level system and a three-level system, and certain aspects of the exact solution are derived in the case of a four-level system. The constants EEE and KKK become a complete set of quantum numbers. It is found that unstable equilibrium, in the sense that 〈L3〉〈{L}_{3}〉〈L3​〉 is constant, does not exist, because of spontaneous emission; it is also found that 〈L3〉〈{L}_{3}〉〈L3​〉 oscillates sinusoidally for the two-level system, oscillates periodically but not sinusoidally for the three-level system, and oscillates aperiodically for a four- or higher-level system, conclusions about the higher-level systems coming from general considerations and numerical solutions found in the literature. Approximate solutions for NO' s with arbitrarily large numbers of levels are obtained. One method of approximation displays spontaneous emission but not aperiodicity. Another approximate method, which contains the statistical spread of the initial phase difference between the oscillations of the two oscillators inherent in the uncertainty principle, displays both spontaneous emission and aperiodicity. It is shown that the aperiodicity - a property which does not exist classically for precise initial conditions - does not disappear even in the macroscopic limit and is due to the averaging performed, in taking the quantum-mechanical expectation value, over an ensemble of periodic oscillations with a spread in frequencies.
The behavior of a nonlinear oscillator (NO) coupled to a radiation field is investigated. The NO considered is an angular momentum oscillator, of energy $\ensuremath{\hbar}\ensuremath{\omega}{L}_{3}$, that describes the collective effect of a number of identical two-level (or spin-\textonehalf{}) systems under given idealized conditions, a large total angular momentum quantum number L0{L}_{0}L0​ corresponding to a large number of two-level systems. The field is described by a set of modes. Free decay---with the NO initially excited and the radiation field in the ground state---and forced oscillation---with the NO subject to a prescribed resonant driving field---are studied. The analysis is performed both classically and quantum mechanically, using the classical and Heisenberg equations of motion, respectively, so as to display explicitly the difference in the results. Interest in the comparison between the two formalisms is motivated by the expectation that for large L0{L}_{0}L0​, the NO should behave essentially classically, except near its highest-energy state in the absence of a driving field. The general equations of motion are reduced to equations for the NO variables only. In the classical analysis of free decay, expressions for the energy and oscillating coordinates are derived. The decay time is shown to approach infinity as L3(0){L}_{3}(0)L3​(0) approaches L0{L}_{0}L0​ (the limiting condition being that of unstable equilibrium) and the radiative frequency shift is shown to be approximately proportional to L3(t){L}_{3}(t)L3​(t). It is also shown that use of the rotating-wave approximation alters qualitatively the expression for the frequency shift. In the classical analysis of forced oscillation, approximate results are obtained for a weak driving field and a strong driving field, the NO being initially in the ground state. The weakfield results exhibit a monotonic approach of L3(t){L}_{3}(t)L3​(t) to a constant (negative) value---or steady state---at which the power absorbed equals the power radiated; in the strong-field case, L3(t){L}_{3}(t)L3​(t) oscillates periodically between the limits $\ifmmode\pm\else\textpm\fi{}{L}_{0}$, the coupling to the radiation field having negligible effect on the frequency of this oscillation. In the quantum-mechanical analysis, the equations of motion become simplified for L0=12{L}_{0}=\frac{1}{2}L0​=21​, and this case is treated first. The free-decay results are essentially similar to those of the Weisskopf-Wigner theory, exhibiting an exponential decay of 〈L3(t)〉〈{L}_{3}(t)〉〈L3​(t)〉 and a radiative frequency shift in the oscillating coordinates. Under forced oscillation, with $〈{L}_{3}(0)〉=\ensuremath{-}{L}_{0}, 〈{L}_{3}(t)〉$ approaches a constant value either monotonically, if the driving field is sufficiently weak, or by means of a damped oscillation, if the driving field is strong. For L0>12{L}_{0}>\frac{1}{2}L0​>21​, the free decay is treated by a method that involves the derivation of a set of expressions for the kthk\mathrm{th}kth derivative of 〈L3(t)〉〈{L}_{3}(t)〉〈L3​(t)〉 as an expectation value of a polynomial in L3{L}_{3}L3​ of order k+1k+1k+1. This set, together with the eigenvalue equation for L3{L}_{3}L3​, is shown to lead to a solution for all the moments of L3{L}_{3}L3​. The method is used to obtain complete solutions for several low values of L0{L}_{0}L0​, and also to obtain initial derivatives of 〈L3(t)〉〈{L}_{3}(t)〉〈L3​(t)〉 as polynomials in L0{L}_{0}L0​ for 〈L3(0)〉=L0〈{L}_{3}(0)〉={L}_{0}〈L3​(0)〉=L0​. For large L0{L}_{0}L0​, a comparison of classical and quantum-mechanical equations shows that only the condition $〈{L}_{3}(0)〉\ensuremath{\approx}{L}_{0}$ requires quantum-mechanical treatment, and that for a short time only. The free-decay problem with initial condition 〈L3(0)〉=L0〈{L}_{3}(0)〉={L}_{0}〈L3​(0)〉=L0​ solved quantum mechanically up to such a time t1{t}_{1}t1​ by means of the initial derivatives previously derived, and then this solution if used to provide initial conditions determining a classical solution for $t\ensuremath{\ge}{t}_{1}$. The statistical aspects introduced by the quantum mechanics are preserved in the classical solution, and their significance is discussed, with several examples, comparison is also made with a nonstatistical approximation. In the case of forced oscillation, the behavior of 〈L3(t)〉〈{L}_{3}(t)〉〈L3​(t)〉---for arbitrary L0{L}_{0}L0​---is examined in detail for a strong field, and turns out to be described by a damped oscillation, the existence of the damping being independent of L0{L}_{0}L0​. The apparent inconsistency of this result with the expectation that a large system subject to strong forces should behave classically is discussed, and 〈L23(t)〉〈{L}_{2}^{3}(t)〉〈L23​(t)〉 is examined. It is concluded that in a single experiment, the NO energy oscillates approximately like the classical energy, without damping; quantum mechanics introduces, however, a slight randomness (or unpredictability) in the frequency of this oscillation, because of the coupling with the radiation field. Since 〈L3(t)〉〈{L}_{3}(t)〉〈L3​(t)〉 describes the average over an ensemble of which each member consists of a NO coupled to a radiation field, the random frequency variation among the members accounts for the damping of the average. The usefulness of the combination of classical and quantum-mechanical analyses in achieving and interpreting theoretical results for a class of phenomena involving the collective interaction between a number of atoms and a radiation field is pointed out.
A large number of "molecules," which are taken to be angular momentum oscillators of frequency $\ensuremath{\nu}$, are considered to interact through their dipole moment with two electromagnetic cavity modes of frequencies ${\ensuremath{\omega}}_{1}$ and ${\ensuremath{\omega}}_{2}$, respectively, where $\ensuremath{\nu}={\ensuremath{\omega}}_{1}\ifmmode\pm\else\textpm\fi{}{\ensuremath{\omega}}_{2}$. The behavior of the combined system is analyzed up to fourth order in perturbation theory. Phenomena known as two-photon emission or absorption, parametric amplification, various types of Raman emission, and frequency conversion are exhibited. The analytical method used is applicable to both a quantum-mechanical and a classical description of the modes and molecules; it displays explicitly the resulting differences. Expressions for the rate of energy change of the modes and molecules indicate resonance in second and fourth order. The second-order results are the same for the classical and quantum-mechanical treatments, while the fourth-order results show certain differences, which are examined in detail. The conditions under which each of the above phenomena occurs are discussed in a self-consistent manner, both classically and quantum-mechanically. It is shown that the second-order expression and the most significant part of the fourth-order expression can be derived very simply from a resonance interaction Hamiltonian that consists of a sum of products of three variables---two referring to the two modes, and the third to the molecules. The relationship between this resonance Hamiltonian and the fundamental dipole-moment Hamiltonian is examined, and the approximations by which the resonance Hamiltonian may be derived are considered. Arguments concerning the applicability of perturbation theory to steady-state situations are presented; it is pointed out that the second-order expressions for the energy transfer between molecules and field may be applicable to such a situation, in which case the classical and quantum-mechanical treatments are equivalent.
A field theoretical formulation of the rather easy problem of N identical, one-dimensional bosons, interacting pairwise via harmonic oscillator potentials of equal force constants is given, in a way similar to the way the nonlinear Schrodinger model provides a field theoretical formulation of a one-dimensional, delta -function Bose gas. The nonlinear integro-differential equation obtained for the complex scalar field of the model is treated classically, and solved in the semiclassical limit of a large number of particles. Working in the centre of mass frame of the field, a sequence of operators that would raise or lower the energy of a state by definite amounts without changing its particle number are constructed from certain bilinear expressions in the field. These operators have, in the limit of a large number of particles, commutation relations similar to those of the Fourier modes of a compact free field, except that the first mode is missing as a result of the fact that the field in the centre of mass frame is subject to the obvious constraint that its centre of mass always coincides with the coordinate origin. The quantum states can be labelled by the total centre of mass momentum, and the quasi-particle numbers in each of the independent oscillator modes. The energy spectrum of the system is calculated, giving the same results as the exact, quantum-mechanical N-body analysis.
The problem of the interaction of a quantum system having discrete states, with a classical oscillating field, is reexamined as a problem in the solution of the time-dependent Schrodinger equation with a periodic Hamiltonian. A method is presented for approximating the time-dependent Hamiltonian with a time-independent one in the weak oscillating field case. With the aid of Floquet's theorem the problem is exactly converted to one with a time-independent Hamiltonian represented by an infinite matrix. The approximation of only two states then permits finding the resonance line shape by perturbation theory for both single and multiple quantum transitions with equal ease. The simple case of only two states connected by an off diagonal sinusoidal perturbation is studied in detail, and a complete description of the average transition probability is found for the strong oscillating field case. A few more complex cases are discussed. A deeper understanding of the analysis is obtained by examining the theory with the oscillating field quantized. Experimental verification of the theory could best be obtained by the methods of atomic beam spectroscopy at radio frequencies.
Complete description of the classical and quantum dynamics of a particle in an anisotropic, rotating, harmonic trap is given. The problem is studied in three dimensions and no restrictions on the geometry are imposed. In the generic case, for an arbitrary orientation of the rotation axis, there are two regions of instability with different characteristics. The analysis of the quantum-mechanical problem is made simple due to a direct connection between the classical mode vectors and the quantum-mechanical wave functions. This connection is obtained via the matrix Riccati equation that governs the time evolution of squeezed states of the harmonic oscillator. It is also shown that the inclusion of gravity leads to a resonant behavior -- the particles are expelled from the trap.