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Physical Review A

Light-narrowed optically pumped Mx magnetometer with a miniaturized Cs cell

Theo Scholtes, V. Schultze, R.P.J. IJsselsteijn, Stefan Woetzel, H.‐G. Meyer

Published Oct 12, 2011• 120 citations
Publisher

Abstract

We demonstrate a way of operating an optically pumped magnetometer with miniaturized cesium cell using the light-narrowing effect. The magnetometer setup shows improvement of shot-noise-limited sensitivity ($42\phantom{\rule{0.16em}{0ex}}\mathrm{fT}/\sqrt{\mathrm{Hz}}$ in a cell of only $9.3\phantom{\rule{0.16em}{0ex}}{\mathrm{mm}}^{3}$ volume) due to the suppression of spin-exchange relaxation to a large extent and the use of a strikingly increased fraction of alkali-metal atoms for signal generation, working even in $\ensuremath{\mu}\mathrm{T}$ magnetic fields, by using only a single high-intensity laser beam both for pumping and probing of atomic spins.

DOI
10.1103/physreva.84.043416

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We demonstrate a way of operating an optically pumped magnetometer with miniaturized cesium cell using the light-narrowing effect. The magnetometer setup shows improvement of shot-noise-limited sensitivity (42fT/Hz42\phantom{\rule{0.16em}{0ex}}\mathrm{fT}/\sqrt{\mathrm{Hz}}42fT/Hz​ in a cell of only 9.3mm39.3\phantom{\rule{0.16em}{0ex}}{\mathrm{mm}}^{3}9.3mm3 volume) due to the suppression of spin-exchange relaxation to a large extent and the use of a strikingly increased fraction of alkali-metal atoms for signal generation, working even in \ensuremathμT\ensuremath{\mu}\mathrm{T}\ensuremathμT magnetic fields, by using only a single high-intensity laser beam both for pumping and probing of atomic spins.
A high-sensitivity optically pumped atomic magnetometer working in the geomagnetic range utilizing the light-narrowing effect and in-phase excitation is described. The setup is based on a simple pump–probe arrangement built around a Cs vapor cell whose active volume is 64 mm3. The transverse oscillating field is applied parallel to the probe beam to drive Zeeman resonance, and the in-phase component of the resonance signal is measured to determine the field. The sensitivity of the magnetometer is improved by pumping most atoms into the stretched state. Consequently, spin-exchange relaxation is suppressed, and a sensitivity of 0.1 pT/Hz1/2 in the range of 10 μT is achieved. This magnetometer has the advantages of large dynamic range, high performance of low-frequency stabilization, high response speed, and compact size. It can be used for many cutting-edge applications such as detection of magnetic anomalies.
Most optically pumped magnetometers based on alkali atom vapor cells and pumped by a single narrow-band laser suffer from a loss of signal since atoms become trapped in the ground hyperfine states that are not coupled to the laser beam. This can be counteracted by additional optical repumping of these ground-state levels. We study hyperfine repumping using cesium vapor cells with partly overlapped ground-state splitting due to their nitrogen buffer-gas filling. We implement two methods of repumping and compare them to the conventional case of F=4 pumping: F=3 repumping with an additional repumper laser and combined pumping/repumping in the light-narrowing mode, where a single high-power laser is tuned near the F=3 transitions. All these modes are investigated for two different methods of spin-phase synchronization: the Mx and intensity modulation methods. For both methods, any kind of repumping results in a clear improvement of the magnetometer sensitivity compared to no repumping, but in the Mx mode it is more pronounced (about 50 versus 200 fT/√Hz for a 50 mm3 Cs vapor cell). The mechanisms responsible for the distinct results in the different working modes are discussed.
An optically pumped atomic magnetometer using a hybrid cell of potassium and rubidium atoms was demonstrated to yield high sensitivity to magnetic fields. We operated the magnetometer with the four possible combinations of optically pumped and optically probed atoms and found that the combination of optically pumped potassium and optically probed rubidium showed the highest sensitivity among the four combinations because the rubidium atoms were denser than those of potassium. Furthermore, we investigated the dependence of the sensitivity on the power densities of the pump and probe beams and the wavelength of the probe beam. The magnetometer using the hybrid cell required higher pump-beam power and had narrower magnetic linewidth than those of the single alkali-metal cell. However, the magnetic linewidth was larger than the theoretical value, ignoring the spin relaxation caused by the spin-exchange collisions. By adjusting the laser conditions, the highest sensitivity approached 30 fTrms/Hz1/2.
We describe a Cs atomic magnetometer operating in the spin-exchange-relaxation-free (SERF) regime. With a vapor cell temperature of $103\text{ }\ifmmode^\circ\else\textdegree\fi{}\text{C}$ we achieve intrinsic magnetic resonance widths $\ensuremath{\Delta}B=17\text{ }\ensuremath{\mu}\text{G}$ corresponding to an electron spin-relaxation rate of $300\text{ }{\text{s}}^{\ensuremath{-}1}$ when the spin-exchange rate is ${\ensuremath{\Gamma}}_{\text{SE}}=14\text{ }000\text{ }{\text{s}}^{\ensuremath{-}1}$. We also observe an interesting narrowing effect due to diffusion. Signal-to-noise measurements yield a sensitivity of about 400 pG/Hz400\text{ }\text{pG}/\sqrt{\text{Hz}}400 pG/Hz​. Based on photon shot noise, we project a sensitivity of 40 pG/Hz40\text{ }\text{pG}/\sqrt{\text{Hz}}40 pG/Hz​. A theoretical optimization of the magnetometer indicates sensitivities on the order of 2 pG/Hz2\text{ }\text{pG}/\sqrt{\text{Hz}}2 pG/Hz​ should be achievable in a 1 cm31\text{ }{\text{cm}}^{3}1 cm3 volume. Because Cs has a higher saturated vapor pressure than other alkali metals, SERF magnetometers using Cs atoms are particularly attractive in applications requiring lower temperatures.
Spin-exchange relaxation free alkali-metal magnetometers typically operate in the regime of high optical density, presenting challenges for simple and efficient optical pumping and detection. We describe a high-sensitivity Rb magnetometer using a single elliptically polarized off-resonant laser beam. Circular component of the light creates relatively uniform spin polarization while the linear component is used to measure optical rotation generated by the atoms. Modulation of the atomic spin direction with an oscillating magnetic field shifts the detected signal to high frequencies. Using a fiber-coupled distributed feedback laser, we achieve magnetic field sensitivity of 7 fT/Hz7\text{ }\text{fT}/\sqrt{\text{Hz}}7 fT/Hz​ with a miniature $5\ifmmode\times\else\texttimes\fi{}5\ifmmode\times\else\texttimes\fi{}5\text{ }\text{mm}\text{ }\text{Rb}$ vapor cell.
The magnetic-resonance lines of alkali atoms are broadened considerably by the spin-exchange collisions for a radio-frequency magnetometer operating at high temperature. The resonance linewidths of cesium atoms are derived by solving the relaxation equations. When spin-exchange relaxation dominates, a light narrowing effect is predicted. For the cesium atomic radio-frequency magnetometer operates at high temperature, a remarkable narrowing of the cesium magnetic-resonance lines are observed by increasing the pump power. The Cs-Cs spin-exchange relaxation is partially suppressed by light narrowing. This study helps to expand the applications of radio-frequency magnetometers in the high-sensitivity radio-frequency magnetic-field detection.