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Physical Review A

Resonance fluorescence of a two-level atom driven by phase-modulated laser light

Maciej Janowicz

Published Sep 1, 1991• 11 citations
Publisher

Abstract

The spectral distribution of light scattered by a two-level atom in a laser beam with phase modulation has been calculated. The spectrum has been obtained via numerical solution of the optical Bloch equations using the algorithm of Wilkens and Rza\ifmmode \mbox{\c{}}\else \c{}\fi{}\ifmmode \dot{z}\else \.{z}\fi{}ewski [Phys. Rev. A 40, 3164 (1989)]. The modulation produces additional sidebands in both coherent and incoherent parts of the spectrum; the location of the added components depends on the modulation depth. In the case of two-frequency phase modulation with incommensurate frequencies, wild, ``chaotic'' behavior of the spectrum has been observed, similar to the case of bichromatic amplitude modulation. The intensity distribution is practically insensitive to the chosen constant value of the phase of modulation.

DOI
10.1103/physreva.44.3144

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Resonance-fluorescence and absorption spectra of a two-level atom driven by a strong bichromatic field

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We examine the radiative properties of a two-level atom driven by a strong bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\delta}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{0}$+${\mathrm{\ensuremath{\delta}}}_{2}$, which can be asymmetrically placed about the atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and can have different Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$. Applying the optical Bloch equations for the bichromatic excitation, we derive an infinite set of equations of motion for the time evolution of the atomic variables. The equations are solved numerically by matrix inversion and Laplace transforms. Using the quantum regression theorem, we then solve for the steady-state total fluorescence intensity, and the resonance-fluorescence and absorption spectra. The spectra are found to depend on the frequency difference 2\ensuremath{\delta}=${\mathrm{\ensuremath{\delta}}}_{1}$+${\mathrm{\ensuremath{\delta}}}_{2}$, the average detuning \ensuremath{\Delta}=${\mathrm{\ensuremath{\omega}}}_{0}$-1/2(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$), and the Rabi frequencies of the driving fields. For ${\mathrm{\ensuremath{\Omega}}}_{1}$=${\mathrm{\ensuremath{\Omega}}}_{2}$=\ensuremath{\Omega}, the total fluorescent intensity displays a series of maxima for \ensuremath{\Delta}=\ifmmode\pm\else\textpm\fi{}n\ensuremath{\delta}\ensuremath{\mp}${\mathrm{\ensuremath{\Omega}}}^{2}$/4\ensuremath{\delta}, where the n are the odd integers. The intensity-dependent shift from the resonances n\ensuremath{\delta} is explained as an analog of the generalized Bloch-Siegert shift. The resonance-fluorescence spectrum for \ensuremath{\Delta}\ensuremath{\ne}0 appears to contain more peaks than that for \ensuremath{\Delta}=0.This is due to the splitting of the central peak and the even sidebands into doublets. The absorption spectrum of a weak-probe beam for \ensuremath{\Delta}=0 and equal Rabi frequencies consists of a symmetric series of dispersionlike sidebands separated from ${\mathrm{\ensuremath{\omega}}}_{0}$ by integer multiples of \ensuremath{\delta}, together with a central absorption peak at ${\mathrm{\ensuremath{\omega}}}_{0}$, whose amplitude oscillates with \ensuremath{\Omega}. For \ensuremath{\Delta}\ensuremath{\ne}0 and/or ${\mathrm{\ensuremath{\Omega}}}_{1}$\ensuremath{\ne}${\mathrm{\ensuremath{\Omega}}}_{2}$, the odd sidebands remain dispersionlike, while the central peak and the even sidebands split into absorption-emission doublets. A simple physical interpretation of the spectral features is given in terms of the dressed-atom model.

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The interaction of a strong bichromatic field with a two-level atom has been the subject of numerous experimental and theoretical investigations. We performed an experimental study of the Interaction of an intense 100% amplitude-modulated (AM) field with an ensemble of homogeneously broadened two-level atoms. An optically pumped sodium atomic beam is used as the atomic medium. The field is created by interfering two intense frequency-stabilized laser fields. The frequency of one field is held fixed while another field of equal amplitude is scanned in frequency. The beat frequency produced by interfering the two laser fields is equal to twice the modulation frequency of a 100% AM field. We monitor the time-averaged fluorescent intensity of the atoms as the frequency separation between the two fields is varied. A similar experiment was done in the past in the rf regime.1 For the first time, we report the observation of multiple, well-resolved resonances in the absorption spectrum of the field in the optical regime. We present data and theory for several values of detuning between the fixed field and atomic resonance. The experimental results are in good agreement with theory.

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Quantum trajectory simulations of the fluorescence intensity from a two-level atom driven by a multichromatic field

S. F. Chien, Mohamed Ridza Wahiddin, Z. Ficek

The quantum trajectories method is illustrated for the resonance fluorescence of a two-level atom driven by a multichromatic field. We discuss the method for the time evolution of the fluorescence intensity in the presence of bichromatic and trichromatic driving fields. We consider the special case wherein one multichromatic field component is strong and resonant with the atomic transition whereas the other components are much weaker and arbitrarily detuned from the atomic resonance. We find that the phase-dependent modulations of the Rabi oscillations, recently observed experimentally [Q. Wu, D. J. Gauthier, and T. W. Mossberg, Phys. Rev. A 49, R1519 (1994)] for the special case when the weaker component of a bichromatic driving field is detuned from the atomic resonance by the strong-field Rabi frequency, appear also for detunings close to the subharmonics of the Rabi frequency. Furthermore, we show that for the atom initially prepared in one of the dressed states of the strong field component the modulations are not sensitive to the phase. We extend the calculations to the case of a trichromatic driving field and find that apart from the modulations of the amplitude there is a modulation of the frequency of the Rabi oscillations. Moreover, the time evolution of the fluorescence intensity depends on the phase regardless of the initial conditions and a phase-dependent suppression of the Rabi oscillations can be observed when the sideband fields are tuned to the subharmonics of the strong-field Rabi frequency.

Physical Review A•Feb 1, 1998•7 citations
The spectral distribution of light scattered by a two-level atom in a laser beam with phase modulation has been calculated. The spectrum has been obtained via numerical solution of the optical Bloch equations using the algorithm of Wilkens and Rza\ifmmode \mbox{\c{}}\else \c{}\fi{}\ifmmode \dot{z}\else .{z}\fi{}ewski [Phys. Rev. A 40, 3164 (1989)]. The modulation produces additional sidebands in both coherent and incoherent parts of the spectrum; the location of the added components depends on the modulation depth. In the case of two-frequency phase modulation with incommensurate frequencies, wild, ``chaotic'' behavior of the spectrum has been observed, similar to the case of bichromatic amplitude modulation. The intensity distribution is practically insensitive to the chosen constant value of the phase of modulation.
We examine the radiative properties of a two-level atom driven by a strong bichromatic field with frequencies ${\mathrm{\ensuremath{\omega}}}_{1}$=${\mathrm{\ensuremath{\omega}}}_{0}$-${\mathrm{\ensuremath{\delta}}}_{1}$ and ${\mathrm{\ensuremath{\omega}}}_{2}$=${\mathrm{\ensuremath{\omega}}}_{0}$+${\mathrm{\ensuremath{\delta}}}_{2}$, which can be asymmetrically placed about the atomic transition frequency ${\mathrm{\ensuremath{\omega}}}_{0}$ and can have different Rabi frequencies ${\mathrm{\ensuremath{\Omega}}}_{1}$ and ${\mathrm{\ensuremath{\Omega}}}_{2}$. Applying the optical Bloch equations for the bichromatic excitation, we derive an infinite set of equations of motion for the time evolution of the atomic variables. The equations are solved numerically by matrix inversion and Laplace transforms. Using the quantum regression theorem, we then solve for the steady-state total fluorescence intensity, and the resonance-fluorescence and absorption spectra. The spectra are found to depend on the frequency difference 2\ensuremath{\delta}=${\mathrm{\ensuremath{\delta}}}_{1}$+${\mathrm{\ensuremath{\delta}}}_{2}$, the average detuning \ensuremath{\Delta}=${\mathrm{\ensuremath{\omega}}}_{0}$-1/2(${\mathrm{\ensuremath{\omega}}}_{1}$+${\mathrm{\ensuremath{\omega}}}_{2}$), and the Rabi frequencies of the driving fields. For ${\mathrm{\ensuremath{\Omega}}}_{1}$=${\mathrm{\ensuremath{\Omega}}}_{2}$=\ensuremath{\Omega}, the total fluorescent intensity displays a series of maxima for \ensuremath{\Delta}=\ifmmode\pm\else\textpm\fi{}n\ensuremath{\delta}\ensuremath{\mp}${\mathrm{\ensuremath{\Omega}}}^{2}$/4\ensuremath{\delta}, where the n are the odd integers. The intensity-dependent shift from the resonances n\ensuremath{\delta} is explained as an analog of the generalized Bloch-Siegert shift. The resonance-fluorescence spectrum for \ensuremath{\Delta}\ensuremath{\ne}0 appears to contain more peaks than that for \ensuremath{\Delta}=0.This is due to the splitting of the central peak and the even sidebands into doublets. The absorption spectrum of a weak-probe beam for \ensuremath{\Delta}=0 and equal Rabi frequencies consists of a symmetric series of dispersionlike sidebands separated from ${\mathrm{\ensuremath{\omega}}}_{0}$ by integer multiples of \ensuremath{\delta}, together with a central absorption peak at ${\mathrm{\ensuremath{\omega}}}_{0}$, whose amplitude oscillates with \ensuremath{\Omega}. For \ensuremath{\Delta}\ensuremath{\ne}0 and/or ${\mathrm{\ensuremath{\Omega}}}_{1}$\ensuremath{\ne}${\mathrm{\ensuremath{\Omega}}}_{2}$, the odd sidebands remain dispersionlike, while the central peak and the even sidebands split into absorption-emission doublets. A simple physical interpretation of the spectral features is given in terms of the dressed-atom model.
The relaxation process and resonance fluorescence of a two-level atom strongly driven by stochastically fluctuating laser light is studied. A laser with small intensity fluctuations about a constant mean value and a diffusing phase is assumed. Depending on the relative time scales of the intensity fluctuations and the atomic response to these fluctuations, the time decay of the atomic population is found to be non-exponential. The broadening of the sidebands in the triplet spectrum of resonance fluorescence is shown to be non-Lorentzian.
We investigate the fluorescence spectrum of a two-level atom driven by a multiple amplitude-modulated field. The driving field is modeled as a polychromatic field composed of a strong central (resonant) component and a large number of symmetrically detuned sideband fields displaced from the central component by integer multiples of a constant detuning. Spectra obtained here differ qualitatively from those observed for a single pair of modulating fields [B. Blind, P.R. Fontana, and P. Thomann, J. Phys. B 13, 2717 (1980)]. In the case of a small number of the modulating fields, a multipeaked spectrum is obtained with the spectral features located at fixed frequencies that are independent of the number of modulating fields and their Rabi frequencies. As the number of the modulating fields increases, the spectrum ultimately evolves to the well-known Mollow triplet with the sidebands shifted from the central component by an effective Rabi frequency whose magnitude depends on the initial relative phases of the components of the driving field. For equal relative phases, the effective Rabi frequency of the driving field can be reduced to zero resulting in the disappearance of fluorescence spectrum, i.e., the atom can stop interacting with the field. When the central component and the modulating fields are $180\ifmmode^\circ\else\textdegree\fi{}$ out of phase, the spectrum retains its triplet structure with the sidebands located at frequencies equal to the sum of the Rabi frequencies of the component of the driving field. Moreover, we show that the frequency of spontaneous emission can be controlled and switched from one frequency to another when the Rabi frequency or initial phase of the modulating fields are varied.
The interaction of a strong bichromatic field with a two-level atom has been the subject of numerous experimental and theoretical investigations. We performed an experimental study of the Interaction of an intense 100% amplitude-modulated (AM) field with an ensemble of homogeneously broadened two-level atoms. An optically pumped sodium atomic beam is used as the atomic medium. The field is created by interfering two intense frequency-stabilized laser fields. The frequency of one field is held fixed while another field of equal amplitude is scanned in frequency. The beat frequency produced by interfering the two laser fields is equal to twice the modulation frequency of a 100% AM field. We monitor the time-averaged fluorescent intensity of the atoms as the frequency separation between the two fields is varied. A similar experiment was done in the past in the rf regime.1 For the first time, we report the observation of multiple, well-resolved resonances in the absorption spectrum of the field in the optical regime. We present data and theory for several values of detuning between the fixed field and atomic resonance. The experimental results are in good agreement with theory.
The quantum trajectories method is illustrated for the resonance fluorescence of a two-level atom driven by a multichromatic field. We discuss the method for the time evolution of the fluorescence intensity in the presence of bichromatic and trichromatic driving fields. We consider the special case wherein one multichromatic field component is strong and resonant with the atomic transition whereas the other components are much weaker and arbitrarily detuned from the atomic resonance. We find that the phase-dependent modulations of the Rabi oscillations, recently observed experimentally [Q. Wu, D. J. Gauthier, and T. W. Mossberg, Phys. Rev. A 49, R1519 (1994)] for the special case when the weaker component of a bichromatic driving field is detuned from the atomic resonance by the strong-field Rabi frequency, appear also for detunings close to the subharmonics of the Rabi frequency. Furthermore, we show that for the atom initially prepared in one of the dressed states of the strong field component the modulations are not sensitive to the phase. We extend the calculations to the case of a trichromatic driving field and find that apart from the modulations of the amplitude there is a modulation of the frequency of the Rabi oscillations. Moreover, the time evolution of the fluorescence intensity depends on the phase regardless of the initial conditions and a phase-dependent suppression of the Rabi oscillations can be observed when the sideband fields are tuned to the subharmonics of the strong-field Rabi frequency.