Quantum state exchange between light and matter is an important ingredient for future quantum information networks as well as other applications. Photons are the fastest and simplest carriers of information for transmission but in general, it is difficult to localize and store photons, so usually one prefers choosing matter as quantum memory elements. Macroscopic superposition and nonlocal quantum interactions have received considerable interest for this purpose over recent years in fields ranging from quantum computers to cryptography, in addition to providing major insights into physical laws. However, these experiments are generally performed either with equipment or under conditions that are unrealistic for practical applications. Ideally, the two can be combined using conventional equipment and conditions to generate a "quantum teleportation"-like state, particularly with a very small amount of purity existing in an overall highly mixed thermal state (relatively low decoherence at high temperatures). In this study we used an experimental design to demonstrate these principles. We performed optical coherence tomography (OCT) using a thermal source at room temperatures of a specifically designed target in the sample arm. Here, position uncertainty (i.e., dispersion) was induced in the reference arm. In the sample arm (target) we placed two glass plates separated by a different medium while altering position uncertainty in the reference arm. This resulted in a chirped signal between the glass plate reflective surfaces in the combined interferogram. The chirping frequency, as measured by the fast Fourier transform (FFT), varies with the medium between the plates, which is a nonclassical phenomenon. These results are statistically significant and occur from a superposition between the glass surface and the medium with increasing position uncertainty, a true quantum-mechanical phenomenon produced by photon pressure from two-photon interference. The differences in chirping frequency with medium disappears when second-order correlations are removed by dual balanced detection, confirming the proposed mechanism. We demonstrated that increasing position uncertainty at one site leads to position uncertainty (quantum position probability amplitude) nonlocally via second-order correlations (two-photon probability amplitude) from a low coherence thermal source (low purity, high local entropy). The implications, first, are that the phenomenon cannot be explained through classical mechanisms but can be explained within the context of quantum mechanics, particularly relevant to the second-order correlations where controversy exists. More specifically, we provide the theoretical framework that these results indicate a nonlocal macroscopic superposition is occurring through a two-photon probability amplitude-induced increase in the target position probability amplitude uncertainty. In addition, as the experiments were performed with a classical source at room temperature, it supports both the quantum-mechanical properties of second-order correlations and that macroscopic superposition is obtainable in a target not in a single coherent state (mixed state). Future work will focus on generalizing the observations outside the current experimental design and creating embodiments that allow practical application of the phenomenon.
Quantum state exchange between light and matter is an important ingredient for future quantum information networks as well as other applications. Photons are the fastest and simplest carriers of information for transmission but in general, it is difficult to localize and store photons, so usually one prefers choosing matter as quantum memory elements. Macroscopic superposition and nonlocal quantum interactions have received considerable interest for this purpose over recent years in fields ranging from quantum computers to cryptography, in addition to providing major insights into physical laws. However, these experiments are generally performed either with equipment or under conditions that are unrealistic for practical applications. Ideally, the two can be combined using conventional equipment and conditions to generate a "quantum teleportation"-like state, particularly with a very small amount of purity existing in an overall highly mixed thermal state (relatively low decoherence at high temperatures). In this study we used an experimental design to demonstrate these principles. We performed optical coherence tomography (OCT) using a thermal source at room temperatures of a specifically designed target in the sample arm. Here, position uncertainty (i.e., dispersion) was induced in the reference arm. In the sample arm (target) we placed two glass plates separated by a different medium while altering position uncertainty in the reference arm. This resulted in a chirped signal between the glass plate reflective surfaces in the combined interferogram. The chirping frequency, as measured by the fast Fourier transform (FFT), varies with the medium between the plates, which is a nonclassical phenomenon. These results are statistically significant and occur from a superposition between the glass surface and the medium with increasing position uncertainty, a true quantum-mechanical phenomenon produced by photon pressure from two-photon interference. The differences in chirping frequency with medium disappears when second-order correlations are removed by dual balanced detection, confirming the proposed mechanism. We demonstrated that increasing position uncertainty at one site leads to position uncertainty (quantum position probability amplitude) nonlocally via second-order correlations (two-photon probability amplitude) from a low coherence thermal source (low purity, high local entropy). The implications, first, are that the phenomenon cannot be explained through classical mechanisms but can be explained within the context of quantum mechanics, particularly relevant to the second-order correlations where controversy exists. More specifically, we provide the theoretical framework that these results indicate a nonlocal macroscopic superposition is occurring through a two-photon probability amplitude-induced increase in the target position probability amplitude uncertainty. In addition, as the experiments were performed with a classical source at room temperature, it supports both the quantum-mechanical properties of second-order correlations and that macroscopic superposition is obtainable in a target not in a single coherent state (mixed state). Future work will focus on generalizing the observations outside the current experimental design and creating embodiments that allow practical application of the phenomenon.
Why are classical theories often sufficient to describe the physics of our world even though everything around us is entirely composed of microscopic quantum systems? The boundary between these two fundamentally dissimilar theories remains an unsolved problem in modern physics. Position measurements of small objects allow us to probe the area where the classical approximation breaks down. In quantum mechanics, Heisenbergâ s uncertainty principle dictates that any measurement of the position must be accompanied by measurement induced back-action---in this case manifested as an uncertainty in the momentum. In recent years, cavity optomechanics has become a powerful tool to perform precise position measurements and investigate their fundamental limitations. The utilization of optical micro-cavities greatly enhances the interaction between light and state-of-the-art nanomechanical oscillators. Therefore, quantum mechanical phenomena have been successfully observed in systems far beyond the microscopic world. In such a cavity optomechanical system, the fluctuations in the position of the oscillator are transduced onto the phase of the light, while fluctuations in the amplitude of the light disturb the momentum of the oscillator during the measurement. As a consequence, correlations are established between the amplitude and phase quadrature of the probe light. However, so far, observation of quantum effects has been limited exclusively to cryogenic experiments, and access to the quantum regime at room temperature has remained an elusive goal because the overwhelming amount of thermal motion masks the weak quantum effects. This thesis describes the engineering of a high-performance cavity optomechanical device and presents experimental results showing, for the first time, the broadband effects of quantum back-action at room temperature. The device strongly couples mechanical and optical modes of exceptionally high quality factors to provide a measurement sensitivity ∼104 times below the requirement to resolve the zero-point fluctuations of the mechanical oscillator. The quantum back-action is then observed through the correlations created between the probe light and the motion of the nanomechanical oscillator. A so-called â variational measurementâ , which detects the transmitted light in a homodyne detector tuned close to the amplitude quadrature, resolves the quantum noise due to these correlations at the level of 10\% of the thermal noise over more than an octave of Fourier frequencies around mechanical resonance. Moreover, building on this result, an additional experiment demonstrates the ability to achieve quantum enhanced metrology. In this case, the generated quantum correlations are used to cancel quantum noise in the measurement record, which then leads to an improved relative signal-to-noise ratio in measurements of an external force. In conclusion, the successful observation of broadband quantum behavior on a macroscopic object at room temperature is an important milestone in the field of cavity optomechanics. Specifically, this result heralds the rise of optomechanical systems as a platform for quantum physics at room temperature and shows promise for generation of ponderomotive squeezing in room-temperature interferometers.
It has recently been shown that counter-intuitive Franson-like second-order interference can be observed with a pair of classically correlated pseudo thermal light beams and two separate unbalanced interferometers (UIs): the second-order interference visibility remains fixed at 1/3 even though the path length difference in each UI is increased significantly beyond the coherence length of the pseudo thermal light [Phys. Rev. Lett.119, 223603 (2017)PRLTAO0031-900710.1103/PhysRevLett.119.223603]. However, as the pseudo thermal beam itself originated from a long-coherence laser (and by using a rotating ground disk), there exists the possibility of a classical theoretical model to account for second-order interference beyond the coherence time on the long coherence time of the original laser beam. In this work, we experimentally explore this counter-intuitive phenomenon with a true thermal photon source generated via quantum thermalization, i.e., obtaining a mixed state from a pure two-photon entangled state. This experiment not only demonstrates the unique second-order coherence properties of thermal light clearly but may also open up remote sensing applications based on such effects.
With the development of quantum optics, photon correlations acquired a prominent role as a tool to test our understanding of physics, and played a key role in verifying the validity of quantum mechanics. The spatial and temporal correlations in a light field also reveal information about its origin, and allow us to probe the nature of the physical systems interacting with it. Additionally, with the advent of quantum technologies, they have acquired technological relevance, as they are expected to play an important role in quantum communication and quantum information processing. This thesis develops techniques that combine spontaneous Raman scattering with Time Correlated Single Photon Counting, and uses them to study the quantum mechanical nature of high frequency vibrations in crystals and molecules. We demonstrate photon bunching in the Stokes and anti-Stokes fields scattered from two ultrafast laser pulses, and use their cross-correlation to measure the 3.9 ps decay time of the optical phonon in diamond. We then employ this method to measure molecular vibrations in CS2, where we are able to excite the respective vibrational modes of the two isotopic species present in the sample in a coherent superposition, and observe quantum beating between the two signals. Stokes scattering, when combined with a projective measurement, leads to a well defined quantum state. We demonstrate this by measuring the second order correlation function of the anti-Stokes field conditional on detecting one or more photons in the Stokes field, which allows us to observe a phonon modeâ s transition form a thermal state into the first excited Fock state, and measure its decay over the characteristic phonon lifetime. Finally, we use this technique to prepare a highly entangled photon-phonon state, which violates a Bell-type inequality. We measure S = 2.360 ± 0.025, violating the CHSH inequality, compatible with the non-locality of the state. The techniques we developed open the door to the study of a broad range of physical systems, where spectroscopic information is obtained with the preparation of specific quantum states. They also hold potential for future technological use, and promote vibrational Raman scattering to a resource in nonlinear quantum optics -- where it used to be considered as a source of noise instead.
Thermal light, such as sunlight, is usually considered classical light. In a macroscopic picture, classical theory successfully explained the first-order coherence phenomena of thermal light. The macroscopic theory, based on the statistical behavior of light intensity fluctuations, however, can only phenomenologically explain the second- or higher-order coherence phenomena of thermal light. This thesis introduces a microscopic quantum picture, based on the interferences of a large number of randomly distributed and randomly radiated subfields, wavepackets or photons, to the study of high-order coherence of thermal light. This thesis concludes that the second-order intensity fluctuation correlation is caused by nonlocal interference: a pair of wavepackets, which are randomly paired together, interferes with the pair itself at two distant space-time coordinates. This study has the following practical motivations: (1) to simulate N-qbits. Practical quantum computing requires quantum bits(qubits) of N-digit to represent all possible integers from 0 to 2 N -1 simultaneously. A large number of independent particles can be prepared to represent a large set of N orthogonal |0> and |1> bits. In fact, based on our recent experiments of simulating the high-order correlation of entangled photons, thermal radiation is suggested as a promising source for quantum information processing. (2) to achieve sunlight ghost imaging. Ghost imaging has three attractive non-classical features: (a) the ghost camera can see targets that can never be seen by a classic camera; (2) it is turbulence-free; and (3) its spatial resolution is mainly determined by the angular diameter of the light source. For example, a sunlight ghost image of an object on earth may achieve a spatial resolution of 200 micrometer because the angular diameter of sun is 0.53 degree with respect to Earth. Although ghost imaging has been experimental demonstrated by using entangled photon pairs and pseudo-thermal light, we still have difficulties to make sunlight ghost image. From the picture of macroscopic local statistics of intensity fluctuations, we may never find the problem that causes sunlight ghost imaging so difficult comparing with that of pseudo-thermal light. To achieve the goals in both fundamental understanding of physics and practical engineering applications, this thesis aims at studying the high-order quantum coherence of thermal light. The first successful attempt of this study is to invent a novel measurement scheme — Positive-Negative Intensity Fluctation Correlation(PNFC) protocol, to measure the intensity fluctuation correlation(or photon number fluctuation correlation) of thermal light. This new photodetection measurement protocol distinguishes positive and negative intensity fluctuations(or photon number fluctuations) of two or more photodetectors within a sequence of short time windows, and then calculates the statistical correlation between these individual fluctuations. With the help of this invention, an anti-correlation of thermal light in a typical Hanbury Brown and Twiss(HBT) interferometry was discovered, which cannot be understood from the view point of traditional macroscopic classical theory. In the microscopic quantum coherence picture, the observation is successfully explained as a nonlocal two-photon interference phenomenon. We also successfully simulated the behavior of Bell-state with thermal light. By manipulating polarization, a thermal Bell-like state was built from two incoherent and orthogonally polarized thermal radiations. With intensity fluctuation correlation measurement, a sinusoidal function with 100% visibility, which suggests thermal light as a feasible source for preparing qubits. Besides the fundamental significance, PNFC protocol also brings incredibly high contrast for quantum imaging, such as 100% visibility for ghost imaging. Above all, we invented a 100% Intensity Fluctuation Correlation of Chaotic-thermal Light and Turbulence-free Imaging System, which provides high contrast as well as high resolution. Based on the experiments of the simulations of quantum interference in thermal light and the dramatically improvement of the contrast in quantum imaging, this study of the high-order coherence of thermal light has a great significance both for fundamental physics and applications.
The utilization and control of nonlocal quantum interactions is an area of active investigation. This is not limited to subatomic structures but extends to the macroscopic level. Nonlocal interactions can be from either entanglement or path indistinguishability (the path integral for larger systems), with the latter being further subdivided as discussed. These two distinct phenomenon have recently been treated often in the literature as essentially identical, which is problematic when utilizing them for practical applications. The confusion may lie in misunderstanding the physics of the type II spontaneous parameteric downconversion source (SPDS), which is used extensively with entanglement studies. This paper examines the distinction, and why it is important for practical applications, between quantum correlations from path indistinguishability versus entanglement. The path indistinguishability approaches discussed, under ambient conditions, are performed with a thermal source or, a coherent source (single photon wavepacket) when local entanglements in both arm have specific characteristics. The latter we will show has the property that it can surprisingly lead to coherence expansion rather than decoherence under the proper conditions. Nonlocal quantum correlations are a complex topic that extends beyond quantum entanglement.
In the case of mixed states ρAB of the composite system A ⊗ B, the previous relation generalizes to ρAB = ∑ k pkρ A k ⊗ρk , where pk are probabilities and ρk ’s (ρk ’s) are generic density matrix of the system A (B). The entanglement derives from “subtle” nonlocal correlations between the parts of a quantum system and combines three basic structural elements of quantum theory: the superposition principle, the quantum non-separability property and the exponential scaling of the state space with the number of partitions. This unique resource can be used to perform computational and cryptographic tasks otherwise impossible with classical systems. An entangled state shared by two or more separated parties is a valuable resource for fundamental quantum protocols, such as quantum teleportation [2], quantum computing [3] and quantum cryptography. By using entangled states we can deeply investigate the nonlocal properties of the quantum world. In fact, an entangled system exhibits correlations between two (or more) parties, which cannot be reproduced by a classical theory or, in general, by a Local Hidden Variables Theory (LHVT). Quantum optics represents an excellent experimental test bench for various novel concepts introduced within the framework of quantum information theory. Quantum states of photons, generally produced by a probabilistic process, namely spontaneous parametric down conversion (SPDC), may be easily and accurately manipulated using linear and nonlinear optical devices and measured by efficient single-photon detectors. Photonic qubits represent the typical carrier of quantum information and can be distributed over long distances, either in free-space or in low-loss optical fibers. Two-particle experiments correspond to operate with qubits belonging to a (2 × 2) Hilbert space. Many quantum information tasks and fundamental tests of quantum mechanics, such as the simulation of properties of quantum systems, the realization of quantum algorithms of increasing complexity and the investigation of the quantum world at a mesoscopic level, deal with a large number of qubits. In order to take full advantage of the possibilities offered by quantum mechanics, more qubits must be added to a quantum state. Two approaches may be followed to increase the number of qubits. The first one consists of increasing the number of entangled particles. In this way, multi-qubit entangled states are created by distributing the qubits between the particles so that each particle carries one qubit. A second strategy consists of encoding more than one qubit in each particle, by exploiting different degrees of freedom (DOFs) of the photon such as the polarization, the path, the emission time, the orbital angular momentum. This has been used to create two-photon fourand six-qubit states and up to five-photon ten-qubit graph states. The entanglement of two particles in different DOFs corresponds to socalled hyperentanglement. It is worth noting that multi-qubit hyperentanglement allows to achieve higher