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Physical Review A

Spontaneous emission from an extended wave packet: Field correlations

Ole Steuernagel, Henryk Paul

Published May 1, 1996• 11 citations
Publisher

Abstract

Utilizing a recently found solution to the problem of a spontaneously radiating atom with an extended center-of-mass wave function [K. Rza\ifmmode \mbox{\c{}}\else \c{}\fi{}\ifmmode \dot{z}\else \.{z}\fi{}ewski and W. \ifmmode \dot{Z}\else \.{Z}\fi{}akowicz, J. Phys. B 25, L319 (1992)] it is shown, for nonrelativistic atomic velocities, that the field density matrix is a statistical mixture of parts corresponding to emission from different positions within the wave packet. \textcopyright{} 1996 The American Physical Society.

DOI
10.1103/physreva.53.2983

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Utilizing a recently found solution to the problem of a spontaneously radiating atom with an extended center-of-mass wave function [K. Rza\ifmmode \mbox{\c{}}\else \c{}\fi{}\ifmmode \dot{z}\else .{z}\fi{}ewski and W. \ifmmode \dot{Z}\else .{Z}\fi{}akowicz, J. Phys. B 25, L319 (1992)] it is shown, for nonrelativistic atomic velocities, that the field density matrix is a statistical mixture of parts corresponding to emission from different positions within the wave packet. \textcopyright{} 1996 The American Physical Society.
Spontaneous emission of a photon by an atom is described theoretically in three dimensions with the initial wave function of a finite-mass atom taken in the form of a finite-size wave packet. Recoil and wave-packet spreading are taken into account. The total atom-photon wave function is found in the momentum and coordinate representations as the solution of an initial-value problem. The atom-photon entanglement arising in such a process is shown to be closely related to the structure of atom and photon wave packets which can be measured in the coincidence and single-particle schemes of measurements. Two predicted effects, arising under the conditions of high entanglement, are anomalous narrowing of the coincidence wave packets and, under different conditions, anomalous broadening of the single-particle wave packets. Fundamental symmetry relations between the photon and atom single-particle and coincidence wave-packet widths are established. The relationship with the famous scenario of Einstein-Podolsky-Rosen is discussed.
We solve the spontaneous and induced emission problem for an atom coupled to a ring cavity, taking into account the center-of-mass motion. We solve analytically the non-Hermitian Schrodinger equation Tor the spontaneous emission. Then we use this solution to test our quantum Monte Carlo solution for the induced processes. The coherence of atomic center-of-mass wave function combined with a well-defined phase of the field produces noteworthy interference phenomena. They may be understood with the help of the semiclassical solution.
Spontaneous emission from a system of NNN identical two-level atoms is considered using a master equation recently derived by the author. The master equation describing the time evolution of the phase-space distribution function associated with the reduced density operator of the atomic system is obtained. This master equation, which is of the type of a Fokker-Planck equation, is used to derive the equation of motion for the mean values of various atomic operators characterizing the physical properties of the system. This leads to a hierarchy of equations, which is decoupled by making a suitable approximation. The intensity of the spontaneously emitted radiation is then calculated. Next, the spontaneous emission from geometrically small systems is considered. For this case, the master equation is solved exactly, and an exact expression for the radiation rate is obtained. The exact solution of the master equation is also used to calculate the normally ordered correlation functions for the electric field. Section V deals with the spontaneous emission from a system of harmonic oscillators, the size of the system being small compared to a wavelength. The master equation for this problem is also solved exactly, and it is shown that this system also leads to superradiant emission in some cases, e.g., if all the oscillstors are excited initially to some coherent state ∣z0〉|{z}_{0}〉∣z0​〉.
A general theory of spontaneous emission was developed in Papers I and II of this series. In the present paper, the mastre equation describing spontaneous emission from NNN identical two-level atoms is investigated further. It is shown that the equation of motion for the p(<N)p(<N)p(<N)-atom density matrix is coupled to the (p+1p+1p+1)-atom density matrix. We first consider the initial excitation of the system to state $|{\ensuremath{\theta}}_{0},{\ensuremath{\phi}}_{0}〉$ (${\ensuremath{\theta}}_{0}<\ensuremath{\pi}$) and solve the hierarchy of equations so obtained in the "uncorrelated approximation." It is found that the presence of other atoms is equivalent to an external field which is determined from a self-consistent analysis. It is also found that in this approximation the state of the atom at time ttt can be described by a single parameter $\ensuremath{\theta}(t)$ ($\ensuremath{\theta}<\ensuremath{\pi}$), with ${sin}^{2}\frac{1}{2}\ensuremath{\theta}$ giving the probability that the atom is to be found in the excited state. Next, some improvements over the uncorrelated approximation are given. This is done by decoupling the equation of motion for higher-order mean values. It is found that the fluctuation $〈({S}_{i}^{Z}\ensuremath{-}〈{S}_{i}^{Z}〉)({S}_{j}^{Z}\ensuremath{-}〈{S}_{j}^{Z}〉)〉$ for any pair of atoms is of the order of 1N\frac{1}{N}N1​. The case when ${\ensuremath{\theta}}_{0}=\ensuremath{\pi}$ is considered separately and we obtain an expression for the radiation rate by making a "Hartree-Fock" type of approximation on the two-particle mean values. In this case, the behavior of the radiation rate is found to differ markedly from the "sech" behavior. It is then shown that the entire dynamics of two-level atoms emitting spontaneously can be described by a set of 2N2N2N coupled first-order equations which clearly exhibit the type of nonlinearity (which is the analog of the van der Pol type of nonlinearity) for this problem and provide a better understanding of spontaneous emission. Finally in Sec. V, the theory is extended to include the effects of inhomogeneous broadening, and the functional dependence of the radiation rate on the atomic-line-shape factor is obtained.