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Chemical Physics Letters

Optimal quantum control with multi-polarization fields

Rong Wu, Ignacio R. Solá, HERSCHEL A. RABITZ

Published Dec 1, 2004• 8 citations
Publisher
DOI
10.1016/j.cplett.2004.10.151

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Quantum algorithms can afford greater computational efficiency compared to their classical counterparts when addressing specific computing tasks. We describe here the implementation, using a polar molecule in an external electric field, of the single-qudit cyclic permutation identification algorithm proposed by Gedik et al. [ Sci. Rep. 5 , 14671 ( 2015 ). 10.1038/srep10995 ]. A molecular ququart is realized through the field-dressed states generated as the pendular modes of BaI. By employing multi-target optimal control theory, we design microwave pulses for ququart-based operations such as the Fourier transformation and its inverse, as well as the oracle U f operation. Specifically, we design an optimized pulse sequence that realizes a quantum algorithm on a single BaI molecule identifying the parity of a member of a set of cyclic permutations with high fidelity. This demonstrates the applicability of optimal control theory to polar molecules for quantum computation.