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Journal of the Optical Society of America B

Giant Kerr nonlinearity induced by tunneling in triple quantum dot molecules

Si-Cong Tian, Ren-Gang Wan, Cunzhu Tong, Yongqiang Ning, Qin Li, Yun Liu

Published Jun 3, 2014• 43 citations
Publisher

Abstract

A scheme for giant enhancement of the Kerr nonlinearity in linear triple quantum dot molecules is proposed. In such a system, the tunneling-induced transparency window obtained in double quantum dot molecules splits into two windows, due to the coupling with the third quantum dot. And most important, the Kerr nonlinearity can be enhanced by several orders of magnitude, compared with that generated in double quantum dot molecules. With proper detuning of the tunneling, giant Kerr nonlinearity accompanied by vanishing absorption can be realized, which opens the possibility to enhance self-phase modulation in tunneling controllable semiconductor nanostructures under conditions of low light levels. Quantitative analysis shows that the giant Kerr nonlinearity is attributed to the interacting double dark resonances induced by the tunneling between the triple quantum dots, therefore no extra laser fields are required.

DOI
10.1364/josab.31.001436

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A scheme for giant enhancement of the Kerr nonlinearity in linear triple quantum dot molecules is proposed. In such a system, the tunneling-induced transparency window obtained in double quantum dot molecules splits into two windows, due to the coupling with the third quantum dot. And most important, the Kerr nonlinearity can be enhanced by several orders of magnitude, compared with that generated in double quantum dot molecules. With proper detuning of the tunneling, giant Kerr nonlinearity accompanied by vanishing absorption can be realized, which opens the possibility to enhance self-phase modulation in tunneling controllable semiconductor nanostructures under conditions of low light levels. Quantitative analysis shows that the giant Kerr nonlinearity is attributed to the interacting double dark resonances induced by the tunneling between the triple quantum dots, therefore no extra laser fields are required.
A scheme for giant Kerr nonlinearity via tunneling in triangular triple quantum dot molecules is proposed. In such a system, the linear absorption and the Kerr nonlinearity depend critically on the energy splitting of the excited states and the tunneling intensity. With proper parameters, giant Kerr nonlinearity accompanied by vanishing absorption can be realized. The enhancement of Kerr nonlinearity is attributed to the interacting double dark resonances induced by the tunneling between the quantum dots, requiring no extra coupling laser fields.
The coherent coupling between three quantum dots via tunneling fields leads to double tunneling-induced transparency and giant Kerr nonlinearity with vanishing absorption. This creates the possibility to achieve self-phase modulation in semiconductor nanostructures via controllable tunneling under the conditions of low light levels. As a result, a considerably high refractive index can be obtained. We suggest an intracavity medium which consists of triple quantum dot molecules to control the Goos–Hänchen (GH) shifts in the reflected light. For a suitable design of a triple quantum dot system, our results show that relatively large positive and negative GH shifts are achievable, without significant distortion, using partially coherent incident light fields.
A theoretical investigation was carried out into the program for enhancing the Kerr nonlinearity by interacting double dark states resonances.Using density-matrix equations and perturbative iterative method,the dependence of the real part of the third-order susceptibility on the variation of the additional coherent driving field detuning was derived.It is found that the maximal Kerr nonlinearity induced by interacting dark resonances increases with increment of the detuning and enters gradually the electromagnetically induced transparency window,in which the corresponding linear absorption vanishes,moreover,by utilizing the dressed state theory,physical mechanisms for the results were presented.The realization of the giant Kerr nonlinearity with vanishing absorption is possible in a generic four-level system with double dark resonances.
The nonlinearity of semiconductor quantum dots under the condition of low light levels has many important applications. In this study, linear absorption, self-Kerr nonlinearity, fifth-order nonlinearity and cross-Kerr nonlinearity of multiple quantum dots, which are coupled by multiple tunneling, are investigated by using the probability amplitude method. It is found that the linear and nonlinear properties of multiple quantum dots can be modified by the tunneling intensity and energy splitting of the system. Most importantly, it is possible to realize enhanced self-Kerr nonlinearity, fifth-order nonlinearity and cross-Kerr nonlinearity with low linear absorption by choosing suitable parameters for the multiple quantum dots. These results have many potential applications in nonlinear optics and quantum information devices using semiconductor quantum dots.
A model of the dynamical equations of the density matrix describes double tunnelling between double quantum dot (QD) system states, this is to study Kerr nonlinearity in QD structure. Inhomogeneity in the QD system is included which is not included in earlier studies of Kerr nonlinearity in QDs. Possibilities of subluminal and superluminal light propagation and switching between them are examined. Double tunnelling is shown to obtain giant Kerr dispersion compared with single tunnelling. High conduction- and low valence-band tunnelling components are required to obtain high Kerr dispersion. Working with one tunnel component reduced Kerr dispersion and switching between subluminal and superluminal can be obtained and the EIT window can be removed.
In the present work, the linear and nonlinear optical properties of quantum dot molecules composed of two quantum dots as well as three quantum dots molecules, respectively known as double quantum dot (DQD) molecule and triple quantum dot (TQD) molecules are studied using the probability amplitude method, and the obtained results are discussed and compared. By solving the state equations of these systems in the interaction picture, under the rotating wave approximation and the dipole approximation, the first and third-order susceptibilities for DQD and TQD molecules are calculated. A phenomenon called tunneling-induced transparency (TIT) which is similar to electromagnetically induced transparency (EIT) is studied in these types of quantum dot molecules. The effect of key system parameters such as tunneling couplings between quantum dots and the tunneling intensity on the linear and nonlinear optical response of multiple quantum dot molecules DQD and TQD is investigated. It was shown that the position and the width of the TIT window created in these quantum dot molecules can be tuned by changing the physical parameters.