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Physical Review A

Photon Correlations in the Parametric Frequency Splitting of Light

B. R. Mollow

Published Nov 1, 1973• 109 citations
Publisher

Abstract

Correlation effects in parametric photon-pair production are studied within the framework of a physically realistic model. The analysis, which is fully quantum mechanical, takes into account the finite sizes of the target and the beam cross section, and allows for dispersion and anisotropy in the linear susceptibility. The correlations in position and time at which the two members of a parametrically generated pair may be detected are carefully evaluated. These correlations, which have been measured experimentally, are intrinsically quantum mechanical; i.e., they can be explained by no theory in which the subharmonic fields are described purely by $c$-number functions. A complete solution, from which field correlation functions of arbitrarily high order may be evaluated, is obtained by a method which at the same time allows for an arbitrary degree of parametric gain. The solution is expressed entirely in terms of a particular two-point field-correlation-function, as evaluated in lowest order in the incident field strength, at points distant from the target. The function in question is found by directly examining the fluctuating currents in the material medium, rather than by eliminating the matter variables at the outset through the introduction of a nonlinear electomagnetic susceptibility.

DOI
10.1103/physreva.8.2684

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Correlation effects in parametric photon-pair production are studied within the framework of a physically realistic model. The analysis, which is fully quantum mechanical, takes into account the finite sizes of the target and the beam cross section, and allows for dispersion and anisotropy in the linear susceptibility. The correlations in position and time at which the two members of a parametrically generated pair may be detected are carefully evaluated. These correlations, which have been measured experimentally, are intrinsically quantum mechanical; i.e., they can be explained by no theory in which the subharmonic fields are described purely by ccc-number functions. A complete solution, from which field correlation functions of arbitrarily high order may be evaluated, is obtained by a method which at the same time allows for an arbitrary degree of parametric gain. The solution is expressed entirely in terms of a particular two-point field-correlation-function, as evaluated in lowest order in the incident field strength, at points distant from the target. The function in question is found by directly examining the fluctuating currents in the material medium, rather than by eliminating the matter variables at the outset through the introduction of a nonlinear electomagnetic susceptibility.
Introduction In the preceding chapters we have been largely concerned with the simplest coherence effects of optical fields, namely those which depend on the correlation of the field variable at two space-time points ( r 1 , t 1 ) and ( r 2 , t 2 ). As we have seen, these effects include the most elementary coherence phenomena involving interference, diffraction and radiation from fluctuating sources. In this chapter we present an extension of the theory to cover more complicated situations, which have to be described by correlations of higher order, i.e. by correlations of the field variables at more than two space-time points or the expectation values involving various powers and products of the field variables. Situations of this kind have become of considerable importance since the development of the laser and of nonlinear optics. The basic difference between the statistical properties of thermal light and laser light can, in fact, only be understood by going beyond the elementary second-order correlation theory. Many of the higher-order coherence phenomena are most clearly manifest in the photoelectric detection process, which can only be adequately described by the quantum theory of detection or by taking into account the quantum features of the field, both of which will be studied in the succeeding chapters. However, because the field is still described classically in the semi-classical theory of light detection, and also because the classical field description provides a natural stepping stone to the quantum description of field correlations, we will now discuss the general description of field correlations of all orders on the basis of the classical theory of the fluctuating wavefield.
A theoretical treatment is given of the situation in which two photons produced in the parametric frequency splitting of light in a nonlinear medium are allowed to interfere. It is shown that there is no interference pattern in the usual sense of quantities that are of the second order in the field, but that fourth-order interference effects are present. These could be demonstrated by placing two photodetectors at positions x,x′ in the interference plane and measuring the joint probability of two detections as a function of x – x′. The probability is predicted to exhibit a cosine modulation with separation x – x′ of close to 100% visibility, even when the integration time in the experiment greatly exceeds the reciprocal bandwidth of the accepted photons. As a result two photons cannot be detected at two points separated by a distance corresponding to an odd number of half-interference fringes. This is an interference effect that violates the laws of classical probability.
One 01 the main objectives of quantum optiCS is to prepare quantum light sources 'Nith the characteristics required lor various quantum optica ppllcallons. Pure single photons and entangled paired photons are two of the most 'Nidely used types of quantum tight. Single photons In a pure, well ellned quantum state may prove to be the building blocks lor future quantum technologies. These technologies promise enormous improvements ove heir ctasslcal counterparts In terms of speed or security. For eICample, in quantum inlormation processing, single photons may be used in quanturT ogic gales, playing the role of electrons in current electric circuits. Although light is all around us In all possible colors, polarizations and intensities, it I ICtremely difficult to get a single photon In a pure quantum state. On the other hand, 11 is relallvely easy to produce pairs of photons, and pure singl horons can be obtained from a two-photon source in a heralded way. Thus, generatlng paired photons with desired photonic properties becomes o'nE pf the cruciattasks in the research area 01 quantum optics and related applications. rrhe process of spontaneous parametric down-conversion (SPDC) is one 01 the most convenient ways to produce pairs 01 photons. In SPDC, a strons ump laser beam Is shone on a nonlinear crystal. Occasionally, a pump photon disappears and two new photons with lower energy are create imultaneously. The production of photon paIrs In the nonlinear crystal is probabilistic and the fact that the two photons are produced simultaneously I n advantage. The two photons can be taken apart and one 01 them can be used as a trigger 10 indicate (herald) the presence of the olher, thereb elllng us when a photon is ready to be used. These pairs of photons have special types 01 correlation In their color (frequency), in theIr spatial shape ndIor In Iheir polarization. For many applications, such as quantum cryptography, these types of correlation may be useful, but at the moment 0 enerating pure Single photons they are detrimental since they diminish the purity of the single photon. In this thesis, we are interested in the frequency properties 01 SPDC pairs of photons. and our main goal Is 10 demonstrate new methods 10 contre hese properties. The frequency properties ollhe photon pairs are described by its joint spectrum, which contains the information of the bandwidth, th wavalorm and the type of frequency correlation possessed by the two photons. n the first part of our work, two new toolklts are added to the current toolbox to manipulate the joint spectrum of photon pairs. One tool is called pulse ronHill' technique. This technique is based on the appropriate Introduction of angular dispersion into the interacting waves. The feasibitity of thi method is demonstrated by observing a sevenfold increase of the band;dth of photon pairs. The corresponding experiment has been accomplished b dding angular dispersion into a coItinear SPDC geometry, where the interacting waves propagate at the same direction. Also, we discuss Ih mplicalion 01 this method lor the generation 01 narrow temporal Fourier transform limited btphotons, and paired photons 'Nith high degree 0 ntangtement. The second tool is called spatial-to·spectral' mapping technique. This technique takes eHec! in a noncoUinear geomelry, in which caSE he pump beam and the down-<:onverted paired photons propagate at different directions. With this situatton, the spatial features of the pump beam 'Nil ~ Imprinted inlo the lrequency distribution 01 the new created photon pairs. We eICperimenlalty prove this method by shaping the waveform, and tunin he types ollrequency correlation 01 the dO'M'l-converted two photons. n addition, we propose a new scheme to fully control the Joint spectrum ollhe pholon pairs by combining the above two discussed techniques. In thi proposal, angular dispersion is introduced into a noncollinear SPDC geometry. This opens a new way to obtain pure single photons 'Nith tunabl band'Nidth. Another topic discussed in this thesis is the exploration of more compact quantum light sources 'Nith versatile characteristics. We describe an SPDC !WO-photon source by using Brag9 reflection wavegulde (BAW) in AI .Gah. As material as down-converting material. Here, the nonlinear proces happens between a pump beam in 8 Bragg refleclion wavegulde mode, and down-converted photon pairs in total internal rellection (TtA) mode. Th ~aveguide dispersion properties can be largely modified by implementing different ridge sizes. and this allows the described monolithic source 10 oHe Ignificant control over the process band'Nidth. We numerically demonstrate the possibility 01 tuning the bandwidth 01 the photon pairs between 1 n~ nd 450 nm with the same waler structure. The results presented in this part have been obtained as a result 01 the collaboration ;th Prol. Amr S. Helmy and his PhD student Payam Abolghasem from University of Toronto. In particular, the programs used lor the presented simulations have bee developed by the University of Toronto leam. o summarize, In this thesis, we add new elements to the current ways 01 engineering quantum light sources. Two readily be used methods to enginee he spectrum of the photon pairs are presented. Particularly, new routes are provided to get pure heralded single photons and narrow tempora biphoton. In addil!on, a compact monolithic two-photon source ;th tunable bandwidth control Is Investigated, which could be very promIsing for furthe pOrlormance of various quantum applications towards reality. Uoc I data Barcelona, 2009·11-16 Signature
Verifying entanglement with experimental measurements requires that we take the limitations of experimental techniques into account, while still proving that the data obtained could not have been generated from a classical source. In the energy-time degree of freedom, this challenge is exacerbated because realistic high-resolution frequency measurements are obtained as a function of light passing through arbitrary filters positioned at uneven intervals. In this work, we show how the data gathered from these kinds of measurements can be used to fully certify the degree of energy and timing correlations needed to certify energy-time entanglement without having to make special assumptions about the state or the measurement device. We accomplish this by showing how to construct a continuous-variable probability density from the data that can closely estimate, but never overestimate the correlations (and entanglement) actually present in the system, and note that these methods are applicable to all continuous-variable degrees of freedom (e.g., spatial, field quadratures, etc.). We illustrate the feasibility of these methods using frequency and timing correlations obtainable from photon pairs in spontaneous parametric down-conversion.