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Nuclear Physics B - Proceedings Supplements

Microscopic and macroscopic quantum models of high T (YBCO) superconductors

A. Widom, C. Vittoria, Tianjian Yuan, Hai Jiang

Published Nov 1, 1993• 0 citations
Publisher
DOI
10.1016/0920-5632(93)90382-g

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We successfully fabricated and studied planar superconductor-normal-superconductor (SNS) Josephson junctions made of ${\mathrm{YBa}}_{2}{\mathrm{Cu}}_{3}{\mathrm{O}}_{7\ensuremath{-}\ensuremath{\delta}}$ (YBCO) high-TC{\mathrm{T}}_{C}TC​ superconductor (S) and Au normal metal (N). The crucial step in fabrication was done by using a Pt/Au bilayer encapsulation of the patterned YBCO nanogap. This procedure preserves the YBCO nanogap from the degradation due to the contact with resists, water, and chemicals involved in further processing for hybrid devices. The junctions exhibit Fraunhofer-like modulation patterns and Shapiro steps when they are irradiated by a rf field. Furthermore, we analyzed the IC(T){I}_{C}(T)IC​(T) characteristics of our hybrid junctions employing a ${\mathrm{SINI}}^{\ensuremath{'}}\mathrm{S}$ (superconductor--insulator--normal conductor--insulator--superconductor) model.
We report on the nonlinear optical signatures of quantum phase transitions in the high-temperature superconductor YBCO, observed through high harmonic generation. While the linear optical response of the material is largely unchanged when cooling across the phase transitions, the nonlinear optical response sensitively imprints two critical points, one at the critical temperature of the cuprate with the exponential growth of the surface harmonic yield in the superconducting phase and another critical point, which marks the transition from strange metal to pseudogap phase. To reveal the underlying microscopic quantum dynamics, a strong-field quasi-Hubbard model was developed, which describes the measured optical response dependent on the formation of Cooper pairs. Further, the theory provides insight into the carrier scattering dynamics and allows us to differentiate between the superconducting, pseudogap, and strange metal phases. The direct connection between nonlinear optical response and microscopic dynamics provides a powerful methodology to study quantum phase transitions in correlated materials. Further implications are light wave control over intricate quantum phases, light-matter hybrids, and application for optical quantum computing.