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American Journal of Physics

Quantum Theory of Interference Effects in the Mixing of Light from Phase-Independent Sources

U. Fano

Published Aug 1, 1961• 172 citations
Publisher

Abstract

Correlations in space and time of the light intensity from extended sources, observed by Brown and Twiss and by Forrester, were analyzed by these authors primarily in terms of field oscillations. This paper discusses an atomic process which brings out the intensity correlations, namely, the photoionization of a pair of atoms following photon emission by another pair of independently excited atoms. The calculated probability of this process depends sinusoidally on the relative positions of the four atoms and also, when the source atoms emit different frequencies, on the time interval between the photoionizations, in agreement with the macroscopic treatment. The oscillations arise from an interference of probability amplitudes which is not affected by the random phases of the source atoms. The calculation follows a standard approach but involves some novel detail.

DOI
10.1119/1.1937827

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Correlations in space and time of the light intensity from extended sources, observed by Brown and Twiss and by Forrester, were analyzed by these authors primarily in terms of field oscillations. This paper discusses an atomic process which brings out the intensity correlations, namely, the photoionization of a pair of atoms following photon emission by another pair of independently excited atoms. The calculated probability of this process depends sinusoidally on the relative positions of the four atoms and also, when the source atoms emit different frequencies, on the time interval between the photoionizations, in agreement with the macroscopic treatment. The oscillations arise from an interference of probability amplitudes which is not affected by the random phases of the source atoms. The calculation follows a standard approach but involves some novel detail.
A comprehensive review is given of investigations, both theoretical and experimental, that demonstrate interference to take place even when the fields involved are produced by independent sources. The physical situation is rather different for coherent and incoherent fields. In the first case, where the sources are lasers, a conventional interference pattern can be observed which is adequately described by the classical theory. In the present paper, special attention is paid to the question of whether this interference persists when the two laser beams become strongly attenuated. In the second case, the sources are individual atoms excited by a pumping mechanism, that emit spontaneously and, hence, independently from each other. In those circumstances, no interference pattern can show up. However, it becomes evident from both the classical and the quantum-mechanical theory that interference effects can still be established by observing intensity correlations rather than the intensity itself. This point is discussed in greater detail. The pioneering experiments of Forrester, Gudmundson and Johnson, and Brown and Twiss are reviewed in this context. Especially interesting from the theoretical point of view is the case of two emitting atoms, since then the classical and the quantum-mechanical description differ significantly, the quantum theory predicting the intensity correlations to be distinctly stronger than those following from classical considerations. This specific quantum-mechanical feature is shown to be intimately connected with the corpuscular aspect of light.
A theory of four-wave mixing is developed using an amplitude approach in the Schr\"odinger picture. It is shown that the four-wave mixing signal produced when three fields are incident on an ensemble of two-level atoms can be viewed as arising from constructive interference of the signals emitted at the various atomic sites. Fourteen distinct amplitudes contribute to the four-wave mixing signal. Some of these amplitudes involve final states in which one or two atoms are excited, and some involve final states in which photons are emitted into modes other than a phase-matched mode of interest. The amplitude approach has the advantage of clearly showing the atom-field correlations. It helps one to understand the underlying physical mechanisms responsible for creation of the four-wave mixing signal, as well as features in the line shape resulting from collisions and effects relating to atomic recoil on the absorption or emission of radiation. These so-called collision- and recoil-induced resonances are calculated explicitly using the amplitude approach, and an interpretation of the results in terms of the interference between different amplitudes is given. Our results, calculated for a finite interaction time between the atoms and the fields, are compared with analogous calculations in which an effective ground-state decay time is assumed. It is shown that the results differ if the atom-field interaction time is not the longest relevant time parameter in the problem.
The interference effects that can be observed in the two output arms of a lossless beam splitter are calculated for incident light in the form of a photon-pair excitation in the two input arms. The output state that occurs when the photon pair is excited in a single input arm resembles that expected for independent classical particles, whereas quantum interference effects occur when the photon pair is divided between the two input arms. Detailed output photocount correlation functions are calculated for two-photon input states produced by a two-atom light source, a degenerate or nondegenerate parametric oscillator in a high-Q cavity, and an atomic cascade emission light source.
In this thesis we discuss an extension of the historical Hanbury Brown and Twiss experiment and investigate spatial intensity correlations of higher-orders in the radiation field of statistically independent light sources. The light sources can be non-classical like single-photon emitters or classical, obeying thermal or coherent statistics. Although the light sources are assumed to emit the photons in an incoherent manner, we find spatial photon correlations in the far field which can be explained by the quantum mechanical concept of multi-photon interferences. We demonstrate that spatial correlation measurements between indistinguishable photons based on linear optical detection techniques can be used to overcome the resolution limit of classical optics (Abbe/Rayleigh limit) and also to manipulate the spatial radiation characteristic of the light sources. Both remarkable properties of higher-order intensity correlations have been experimentally verified using statistically independent pseudothermal light sources. Due to the fact that the reported correlation measurements require neither special quantum tailoring of light nor N-photon absorbing media, they are of particular interest for the field of quantum imaging and quantum information processing. The thesis is divided into three main parts: In the first part (Chapter 2 and 3) we introduce a quantum path formalism which allows to describe multi-photon interferences arising in both classical and nonclassical light fields. This quantum path approach explains the origin of the underlying interference mechanism of the higher-order spatial intensity correlation functions in a transparent and simple manner. Moreover, it enables us to compare the multi-photon interferences obtained by nonclassical single-photon emitters with those generated by classical light sources. In the course of this discussion it appears that Dirac's famous statement “Each photon interferes only with itself. Interference between two different photons never occurs.” should better read “A multi-photon state of independent photons only interferes with itself. Interference between different multi-photon states never occurs.” This general statement summarizes the physics behind all multi-photon interference phenomena investigated in this thesis. In the second part of the thesis (Chapter 4) we investigate particular multi-photon interference measurements of independent light sources in the context of quantum imaging. We demonstrate that the Nth-order spatial intensity correlation functions display at specific ‘magic’ detector positions the ability to filter sub-wavelength information out of the light fields arising from N incoherently radiating light sources. These multi-photon interference patterns achieve a higher resolution for N>2 than the classical Abbe/Rayleigh limit for imaging the light source. In case of N single-photon emitters we theoretically show that the super-resolving interference patterns obtained for the ‘magic’ detector positions are identical to the ones generated by NOON states with N-1 photons. Quite unexpected, the same is true for N thermal light sources, except for a reduced visibility. Experimental results with up to eight independent thermal light sources confirm this approach to improve the spatial resolution in imaging. In the last part of this thesis (Chapter 5) we finally demonstrate that multi-photon detections can lead to a strong angular focussing of incoherent photons emitted again by either uncorrelated single-photon sources or statistically independent classical light sources. For this effect the sources can be far away from each other and do not interact. The mth-order intensity correlation measurement causes source correlations which produce a heralded peaked emission pattern for the initially uncorrelated light sources. In particular, we show that if m-1 photons have been detected in a particular direction, the conditional probability to detect the mth photon in the same direction can be as high as 100 %. Owing to the great flexibility of detector positions for the correlation measurement, a wide variety of additional detection schemes exists which produces similar directional photon emission patterns. This theoretically predicted measurement-induced focussing was experimentally confirmed with up to eight pseudothermal light sources for three particular detection schemes.
The conditions are examined under which interference effects should be observable in the superposition of two light beams derived from independent sources. The quantum-mechanical description of these effects differs from the classical description principally in that it is necessarily based on expectation values of the light intensity at one or more space-time points. It is shown that pure states of the radiation field which are not energy states give rise to interference effects, but in that case the two beams cannot meaningfully be described as statistically independent. For a realistic description mixed states have to be introduced, when the expectation value of the intensity gives no indication of interference effects. On the other hand, the intensity correlation at two space-time points is a periodic function of the separation of the points and indicates the presence of transient interference effects. The effects become readily observable only when the average photon occupation number of each cell of phase space is appreciably greater than 1, and this explains why laser beams were needed for the experimental observations. It is pointed out that, even in these experiments, each photon may be regarded as interfering only with itself.
Excitation and photoionization of Rydberg wave packets are described. Interference of bound-free transitions from many coherently populated Rydberg levels is shown to affect the dependence of the photoionization probability on the duration of interaction. Strong-field interference effects in such a system are described also. The most important of these is the field-induced interference stabilization of Rydberg atoms in a strong ionizing field. The intensity range in which this effect can exist is determined. The results derived are used for a qualitative model describing supercontinuum emission in the process of multiphoton ionization.