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Physical Review Letters

Electrostatic Trapping of Neutral Atomic Particles

William H. Wing

Published Aug 25, 1980• 113 citations
Publisher

Abstract

Excited neutral atoms having positive Stark energies may be trapped near magnitude minima of electrostatic fields. At moderate field strengths Rydberg atoms have trap depths comparable to ambient $\mathrm{kT}$ and as much as 100 times those of recently proposed optical-field traps. Polar molecules and metastable hydrogen and positronium atoms also can be trapped. A slow nondegenerate atom in a quadrupole field is harmonically bound. Sustained trapping and cooling should be possible, allowing Doppler-free few-atom spectroscopy and novel collision studies.

DOI
10.1103/physrevlett.45.631

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Excited neutral atoms having positive Stark energies may be trapped near magnitude minima of electrostatic fields. At moderate field strengths Rydberg atoms have trap depths comparable to ambient kT\mathrm{kT}kT and as much as 100 times those of recently proposed optical-field traps. Polar molecules and metastable hydrogen and positronium atoms also can be trapped. A slow nondegenerate atom in a quadrupole field is harmonically bound. Sustained trapping and cooling should be possible, allowing Doppler-free few-atom spectroscopy and novel collision studies.
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In order to confine any object, it is necessary to exchange kinetic for potential energy in the trapping field, and in neutral atom traps, the potential energy must be stored as internal atomic energy. Thus practical traps for ground-state neutral atoms are necessarily very shallow compared with thermal energy because the energy level shifts that result from conveniently sized fields are typically considerably smaller than k B T , even for T = 1 K. Neutral atom trapping therefore depends on substantial cooling of a thermal atomic sample, and is often connected with the cooling process. In most practical cases, atoms are loaded from magneto-optical traps, where they have been efficiently accumulated and cooled to mK temperatures (see Sec. 20.3), or from optical molasses, where they have been optically cooled to μK temperatures (see Sec. 19.4). The small depth of typical neutral atom traps dictates stringent vacuum requirements, because an atom cannot remain trapped after a collision with a thermal energy background gas molecule. Since these atoms are vulnerable targets for thermal energy background gas, the mean free time between collisions must exceed the desired trapping time. The cross-section for destructive collisions is quite large because even a gentle collision (i.e. large impact parameter) can impart enough energy to eject an atom from a trap. At pressure P sufficiently low to be of practical interest, the trapping time is ~(10 -8 / P ) s, where P is in torr. This chapter begins with a discussion of ordinary, single-center traps, but also considers arrays of traps. Such “optical lattices” are playing an increasingly important role in research in atomic physics, so discussion of their properties is an appropriate part of the education of a student of the subject. Dipole force optical traps Single-beam optical traps for two-level atoms The simplest imaginable optical trap consists of a single, strongly focused Gaussian laser beam (see Fig. 20.1) [214, 215] whose intensity at the focus varies transversely with r as where is the beam waist size. Such a trap has a well-studied and important macroscopic classical analog in a phenomenon called optical tweezers (see App. 1.C) [216–218].
Hydrogen atoms in supersonic expansions with velocities in the range from 700to800m∕s700\phantom{\rule{0.3em}{0ex}}\text{to}\phantom{\rule{0.3em}{0ex}}800\phantom{\rule{0.3em}{0ex}}\mathrm{m}∕\mathrm{s}700to800m∕s have been excited to Rydberg-Stark states with principal quantum number nnn between 20 and 40, decelerated to zero velocity in the lab frame using time-dependent inhomogeneous electric fields, and trapped in a two-dimensional electrostatic trap with an initial density of $\ensuremath{\approx}5\ifmmode\times\else\texttimes\fi{}{10}^{6}\phantom{\rule{0.3em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$. The motion of the atomic cloud in the trap was observed by measuring the times of flight and images of the H+{\mathrm{H}}^{+}H+ ions produced by pulsed field ionization. The velocity distribution of the trapped atoms can be described by an effective temperature of 350mK350\phantom{\rule{0.3em}{0ex}}\mathrm{mK}350mK. The decay of the population of trapped atoms does not follow a single-exponential behavior and has contributions from radiative and collisional processes.
The interaction between inhomogeneous electric fields and the large electric dipole moments of atoms and molecules in Rydberg states of high principal quantum number can be used to efficiently accelerate and decelerate atoms and molecules in the gas phase. We describe here how hydrogen atoms and molecules initially moving with velocities of ∼600 m/s in supersonic beams can be decelerated to zero velocity and loaded into electric traps. The long observation times that are made possible by the electrostatic trapping enables one to study slow relaxation processes. Experiments are presented in which we have observed photoionization processes and transitions between Rydberg states induced by blackbody radiation at temperatures between 10 K and 300 K on a time scale of several milliseconds. Comparison of these processes in Rydberg states of H and H(2) suggests the importance, in H(2), of collisional processes and of the process of blackbody-radiation-induced predissociation.
Ion–atom interactions are a comparatively recent field of research that has drawn considerable attention due to its applications in areas including quantum chemistry and quantum simulations. In first experiments, atomic ions and neutral atoms have been successfully overlapped by devising hybrid apparatuses combining established trapping methods, Paul traps for ions and optical or magneto-optical traps for neutral atoms, respectively. Since then, the field has seen considerable progress, but the inherent presence of radiofrequency (rf) fields in such hybrid traps was found to have a limiting impact on the achievable collision energies. Recently, it was shown that suitable combinations of optical dipole traps (ODTs) can be used for trapping both atoms and atomic ions alike, allowing to carry out experiments in absence of any rf fields. Here, we show that the expected cooling in such bichromatic traps is highly sensitive to relative position fluctuations between the two optical trapping beams, suggesting that this is the dominant mechanism limiting the currently observed cooling performance. We discuss strategies for mitigating these effects by using optimized setups featuring adapted ODT configurations. This includes proposed schemes that may mitigate three-body losses expected at very low temperatures, allowing to access the quantum dominated regime of interaction.