On the propagation of coherent radiation in gases

T.E. Kishimoto, Hiroshi Takahashi, Atsushi Hasegawa +1 more

D. V. Kosachev, Boris G. Matisov

F. A. Vorob'ev, R. I. Sokolovskiǐ

A. Ben‐Reuven

General expressions are derived for the spectral line shapes of resonance absorption and scattering of coherent radiation in collision-broadened gases, taking into account effects of coherent excitation of two or more atoms (or molecules), as steady-state solutions of a hierarchy of master equations described in a previous publication (paper I). Coupling between the coherent motions of the atoms, provided by a Bethe-Salpeter---type effective interaction, in the binary-collision approximation, forms the essential mechanism for introducing cooperative coherent effects into the steady-state spectra. Explicit expressions are given for the effects of two-atom coherence in the binary-collision approximation, in which the Bloch-type dressed-atom self-energy superoperator is modified by the presence of collisions in which both atoms retain memory of their coherent propagation before the collision. The self-energies include the effects of resonance exchange symmetrization in self-broadening, and are renormalized by the coincidence of radiative transitions during the collisions. The impact (near-resonance) and the quasistatic (line-wing) limits of the applied-frequency detunings are discussed. In the quasistatic limit, coherent many-atom excitations become irrelevant; however, interactions of both collision partners with the radiation during the collision accounts for such phenomena as collision-induced absorption or radiative collisions. In the impact limit, the inclusion of the Bethe-Salpeter interactions allows for the appearance of two-atom resonances. Magnitude estimates of these effects are discussed. Effects of higher-rank (many-body) coherences are formally discussed with the help of a diagrammatic method, leading into implicit bootstrap equations that can be solved by iterative or other procedures.

C. K. Rhodes

Stephen E. Harris

Electromagnetically induced transparency is a technique for eliminating the effect of a medium on a propagating beam of electromagnetic radiation. EIT may also be used, but under more limited conditions, to eliminate optical self-focusing and defocusing and to improve the transmission of laser beams through inhomogeneous refracting gases and metal vapors, as figure 1 illustrates. The technique may be used to create large populations of coherently driven uniformly phased atoms, thereby making possible new types of optoelectronic devices.