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Journal of the Optical Society of America B

Four-wave mixing under conditions when optical Bloch equations fail

Sunita Singh, G. S. Agarwal

Published Feb 1, 1988• 7 citations
Publisher

Abstract

The nonlinear-optical properties of a system whose collisional dynamics are strongly affected by intense pump fields are calculated. The four-wave mixing signals can be affected in a dramatic way if the period of the Rabi oscillation is comparable with the correlation time of the collisional mechanism.
DOI
10.1364/josab.5.000254

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We investigate the influence of the distribution of atom velocities in a hot rubidium sample on the correlation between field-intensity fluctuations of two independently generated four-wave mixing signals and between the transmission signals. The nonlinear process is driven by a single continuous-wave (cw) laser in a pure two-level system due to the forward geometry with circular and parallel polarization of the input fields. The intensity cross correlations of the four-wave mixing signals and the transmission signals present an oscillatory behavior with a clear dependence on the power of the incident fields, which indicates a connection with Rabi oscillations. A two-level theoretical model using stochastic differential equations to account for the mechanism of conversion of phase noise into amplitude noise shows good agreement with our experimental results. Moreover, we show how the response of the system is affected by the different atomic velocity groups.