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Physica Scripta

Dynamics of spontaneous emission

P. L. Knight

Published Jan 1, 1997• 5 citations
Publisher

Abstract

A number of interpretations of the origins of spontaneous emission are examined. In particular, the idea of quantum jumps in the recorded fluorescence from excited atoms and their theoretical treatment is reviewed using recent Monte-Carlo simulation approaches to spontaneous emission. These are illustrated for pure spontaneous emission and for the telegraphic quantum jump signal in the fluorescence from three-level atoms.

DOI
10.1088/0031-8949/1997/t70/014

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A number of interpretations of the origins of spontaneous emission are examined. In particular, the idea of quantum jumps in the recorded fluorescence from excited atoms and their theoretical treatment is reviewed using recent Monte-Carlo simulation approaches to spontaneous emission. These are illustrated for pure spontaneous emission and for the telegraphic quantum jump signal in the fluorescence from three-level atoms.
A Monte Carlo simulation of the atomic master equation for spontaneous emission in terms of atomic wave functions is developed. Realizations of the time evolution of atomic wave functions are constructed that correspond to an ensemble of atoms driven by laser light undergoing a sequence of spontaneous emissions. The atomic decay times are drawn according to the photon count distribution of the driven atom. Each quantum jump of the atomic electron projects the atomic wave function to the ground state of the atom. Our theory is based on a stochastic interpretation and generalization of Mollow's pure-state analysis of resonant light scattering, and the Srinivas-Davies theory of continuous measurements in photodetection. An extension of the theory to include mechanical light effects and a generalization to atomic systems with Zeeman substructure are given. We illustrate the method by simulating the solutions of the optical Bloch equations for two-level systems, and laser cooling of a two-level atom in an ion trap where the center-of-mass motion of the atom is described quantum mechanically.
The spontaneous decay of an excited atom by photon emission is one of the most common and elementary physical process present in nature and in laboratories. The decay is random in time with constant probability density, as it can be inferred by the exponential law observed experimentally. Despite the simplicity of the process, in Quantum Mechanics the decay itself is considered a law of nature which is not further analyzed or explained. However it is legitimate to ask for the reason of its randomness and for the dynamics of the atom around the decay. The decay process of an isolated atom is usually assumed to be instantaneous, the so called Quantum jumps. Particular experimental arrangements can widen the duration of the transition from an excited state to the ground state to a finite time. In general this is due to the quantum back action of the detector. The development of Quantum Optics has enormously enriched the possibilities to study in detail the process, and new illuminating insights have been obtained, but the question is still valid and its answer is still elusive. In this paper we analyze the spontaneous decay within the new prospect introduced by a recent model that complete standard Quantum Mechanics in a formalism which is able to describe the dynamics of measurement and of spontaneous decay. Comparison is made with more phenomenological theories, the Quantum Mechanics of open system and the Stochastic wave function model. In the new model the stochastic photon emission by an excited atom is triggered by the vacuum fluctuations. It is suggested how to re-analyze three types of experiments, already realized in many laboratories, in order to reveal the presence and the effect of these fluctuations.
We consider a three-level atomic system driven strongly on one transition and weakly on the other. The excited state on the weak transition is assumed to be metastable. We give an analysis of the fluorescence from the strong transition in terms of the elementary probability density p[0{p}_{[0}p[0​,t)(t1{\mathrm{t}}_{1}t1​,t2{t}_{2}t2​,..., tn{t}_{n}tn​) which gives us the probability density that exactly n photons are emitted at times t1{t}_{1}t1​,t2{t}_{2}t2​,...,tn{t}_{n}tn​ by the atom in the time interval [0,t). We show that p[0{p}_{[0}p[0​,t) essentially factorizes into products of conditional densities c\ifmmode \tilde{}\else \~{}\fi{}(\ensuremath{\tau}) that, given a photon is emitted at time zero, the next photon emission occurs at time \ensuremath{\tau}. This enables a simulation of the individual photon emissions to be given which shows directly the existence of prolonged dark windows in the fluorescence corresponding to the shelving of the electron in the metastable state or ``quantum jumps.''
The statistics of spontaneous photon emission times in single atom resonance fluorescence are investigated through the radiative cascade of the dressed atom. The delay function which gives the distribution of the delays between two successive emissions is calculated for a coherent as well as an incoherent laser excitation. For a two-level atom, various signals that reflect the fluorescence intensity (average value, photon counting, fluctuation spectrum, etc.) are reviewed by this method. For a three-level atom, this approach is applied to the analysis of the recently observed phenomenon of intermittent fluorescence and quantum jumps.>