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Applied Physics B

Effects of inert gases on the degenerate four-wave-mixing spectrum of NO2

A. P. Smith, Ged Hall, Benjamin J. Whitaker, A. G. Astill, David W. Neyer, Paul A. Delve

Published Jan 1, 1995• 20 citations
Publisher
DOI
10.1007/bf01082067

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We report an experimental investigation of degenerate four-wave mixing spectrum of SO2.A novel beam-split technique is used to compensate the beam drift caused by the laser itself and disturbance from the environment.Degenerate four-wave mixing spectra of the transition B 1 B1 ← X 1 A11 for SO2 are obtained.The degenerate four-wave mixing signal intensity as a function of the total input laser energy is measured.The effects of the laser field intensity on the degenerate four-wave mixing spectrum are analyzed.Our results show that the degenerate four-wave mixing signal intensity rises with laser intensity and tends to saturate.Then, a dip begins to appear at resonance in the profile with increase in laser field.The existence of saturation for degenerate four-wave mixing signal intensity and spectrum profile confirms the prediction of previous theoretical work.