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Physica Scripta

Perspectives on the Fano Resonance Formula

A. R. P. Rau

Published Dec 22, 2003• 80 citations
Publisher

Abstract

The general profile of a resonance, as given by Fano in 1961, is well known throughout physics. This Comment provides some of the simplest derivations of this formula, together with a discussion of subtleties in handling continuum states with regard to their normalization, orthogonality, and completeness. Inadequate appreciation of these subtleties has led to misconceptions and errors in analysis. Recent, novel applications of the Fano formula in condensed matter systems include systems with decoherence and lack of time reversal symmetry which make the resonance profile parameter complex.

DOI
10.1238/physica.regular.069a00c10

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The general profile of a resonance, as given by Fano in 1961, is well known throughout physics. This Comment provides some of the simplest derivations of this formula, together with a discussion of subtleties in handling continuum states with regard to their normalization, orthogonality, and completeness. Inadequate appreciation of these subtleties has led to misconceptions and errors in analysis. Recent, novel applications of the Fano formula in condensed matter systems include systems with decoherence and lack of time reversal symmetry which make the resonance profile parameter complex.
Abstract The Fano resonance has been a familiar and important feature in atomic and molecular physics for more than half a century. Typically, the combination of a discrete state with one or more continua results in an asymmetric peak in the ionization spectrum. The peak-shape, called the Fano profile, can be expressed by a simple formula derived by Fano in 1935. However, the interpretation of its characteristic parameter q , which represents the asymmetry of the peak in the formula, is not necessarily intuitively transparent. The Fano resonance is not necessarily a quantum effect, but it is a manifestation of a certain physical mechanism in various systems, both quantum and classical. Through the derivation of q from the known classical pictures with the classical coupled oscillator, we interpret the q value with a geometrical view. And further, we introduce a complex valued q parameter for the description of the resonance with a damped oscillator.
Fano resonance is a ubiquitous phenomenon, and it is commonly interpreted as a two-channel interference of the discrete and continuous channels. The present work investigates the Fano profile from a perspective of the temporal evolution of the wave function. By exciting the atom with a δ pulse and calculating the evolution of the wave function, the Fano formula is deduced. The results clearly show that the Fano resonance is of a three-channel interference, which is different from the traditional understanding. The three channels are revealed as the ground-continuum, ground-discrete-continuum, and a previously unmentioned third channel, i.e., ground-continuum-discrete-continuum. The present three-channel interpretation can be easily generalized to other physical systems, contributing to a deeper understanding of the Fano profile.
The line shape of resonances in the overlapping regime is studied by using the eigenvalues and eigenfunctions of the effective Hamiltonian of an open quantum system. A generalized expression qk(E){q}_{k}(E)qk​(E) for the Fano parameter of the resonance state k is derived that contains the interaction of the state k with neighbored states $l\ensuremath{\ne}k$ via the continuum. It is energy dependent since the coupling coefficients between the state k and the continuum show a resonancelike behavior at the energies of the neighbored states $l\ensuremath{\ne}k.$ Under certain conditions, the energy dependent qk(E){q}_{k}(E)qk​(E) are equivalent to the generalized complex energy independent Fano parameters that are introduced by Kobayashi et al. in analyzing experimental data. Long-lived states appear mostly isolated from one another in the cross section, also when they are overlapped by short-lived resonance states. The qk(E){q}_{k}(E)qk​(E) of narrow resonances allow therefore to study the complicated interplay between different time scales in the regime of overlapping resonance states by controlling them as a function of an external parameter.
Fano resonance is a well-celebrated weak-coupling phenomenon whereby a small interaction between a discrete and a continuum of excited states leads to an interference between the respective two transition amplitudes, resulting in an asymmetric line shape in the excitation spectra. We present the strong-coupling phase of the Fano's model where the interaction is localized in a region $\ensuremath{\xi}$ that is smaller than the collective coupling between the discrete state and the continuum. We explore the behavior of the excitation probability $\ensuremath{\sigma}$ as a function of $\ensuremath{\xi}$, the ratio of the bare transition amplitudes, and the energy of the discrete state. In the strong-coupling phase, the spectral function of the discrete state splits up and produces up to three complete destructive interferences or zeros of $\ensuremath{\sigma}$ along with ultrasharp features. We also find that the discrete state does not have to lie within the continuum to produce the well-known weak-coupling profiles of $\ensuremath{\sigma}$ as long as the collective coupling is strong enough. In addition, we consider a broadened state instead of a continuum and present a method that exactly treats such cases by explicitly including the source of the broadening---a weak coupling to the continuum of environment states---in the model.