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Physical Review Letters

Atomic Interference in Grazing Incidence Diffraction from an Evanescent Wave Mirror

Laurent Cognet, V. Savalli, G. Horváth, David Holleville, Roberta Marani, Nathalie Westbrook, Christoph Ira Westbrook, Alain Aspect

Published Dec 7, 1998• 24 citations
Publisher

Abstract

We report an experiment showing that atomic diffraction at grazing incidence from an evanescent wave mirror results from polarization gradients in the evanescent wave which induce transitions among atomic internal states. The resulting grating can produce large angle coherent beam splittings. We also demonstrate atomic interference in the form of a St\"uckelberg oscillation in the diffraction efficiency which is very sensitive to the atom wall van der Waals potential.

DOI
10.1103/physrevlett.81.5044

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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•Oct 21, 2004•0 citations
We report an experiment showing that atomic diffraction at grazing incidence from an evanescent wave mirror results from polarization gradients in the evanescent wave which induce transitions among atomic internal states. The resulting grating can produce large angle coherent beam splittings. We also demonstrate atomic interference in the form of a St"uckelberg oscillation in the diffraction efficiency which is very sensitive to the atom wall van der Waals potential.
We show that internal state transitions may induce energy transfer among different directions of motion and lead efficiently to large scattering angles in atomic reflection from evanescent-wave mirrors. The proposed scattering mechanism is reminiscent of the so-called Sisyphus effect of laser cooling. Perturbative calculations are presented and discussed for the diffraction of atomic beams at grazing incidence on evanescent fields with polarization gradients and for the reflection of atoms by a rough mirror.
After a brief introduction to the field of atom optics and to atomic mirrors, we present experimental results obtained in our group during the last two years while studying the reflection of rubidium atoms by an evanescent wave. These involve the first measurement of the van der Waals force between an atom in its ground state and a dielectric wall, as well as the demonstration of a reflection grating for atoms at normal incidence. We also consider the influence of quantum reflection and tunnelling phenomena. Further studies using the atomic mirror as a probe of the van der Waals interaction, and of very small surface roughness are briefly discussed.
We have experimentally demonstrated a material-independent mirror for atomic waves that uses the Fresnel diffraction at an array of parallel ridges. He* (2 (3)S(1)) and Ne* (1s(3)) atomic waves were reflected coherently on a silicon plate with a microfabricated grating structure, consisting of narrow wall-like ridges. We measured the reflectivity at grazing incidence as a function of the incident velocity and angle. Our data show that the reflectivity on this type of mirror depends only on the distance between the ridges, the wavelength, and the incident angle, but is insensitive to the material of the grating structure. The reflectivity is observed to increase by 2 orders of magnitude, compared to that of a flat polished silicon surface, where the reflection is caused by the attractive surface potential. For He* atoms, the measured reflectivity exceeds 10% for normal incident velocities below about 25 cm/s.
We report on the observation of emerging beam resonances, well known as Rayleigh-Wood anomalies and threshold resonances in photon and electron diffraction, respectively, in an atom-optical diffraction experiment. Diffraction of He atom beams reflected from a blazed ruled grating at grazing incidence has been investigated. The total reflectivity of the grating as well as the intensities of the diffracted beams reveal anomalies at the Rayleigh angles of incidence, i.e., when another diffracted beam emerges parallel to the grating surface. The observed anomalies are discussed in terms of the classical wave-optical model of Rayleigh and Fano.
A research project at the “Laboratoire d’électronique quantique” consists in a theoretical study of the reflection and diffraction phenomena via an atomic mirror. This poster presents the principle of an atomic mirror. Many groups in the world have constructed this type of atom optics experiments such as in Paris‐Orsay‐Villetaneuse (France), Stanford‐Gaithersburg (USA), Munich‐Heidelberg (Germany), etc. A laser beam goes into a prism with an incidence bigger than the critical incidence. It undergoes a total reflection on the plane face of the prism and then exits. The transmitted resulting wave out of the prism is evanescent and repulsive as the frequency detuning of the laser beam compared to the atomic transition δ = ωL−ω0 is positive. The cold atomic sample interacts with this evanescent wave and undergoes one or more elastic bounces by passing into backward points in its trajectory because the atoms’ kinetic energy (of the order of the μeV) is less than the maximum of the dipolar potential barrier ℏΩ2/Δ where Ω is the Rabi frequency [1]. In fact, the atoms are cooled and captured in a magneto‐optical trap placed at a distance of the order of the cm above the prism surface. The dipolar potential with which interact the slow atoms is obtained for a two level atom in a case of a dipolar electric transition (D2 Rubidium transition at a wavelength of 780nm delivered by a Titane‐Saphir laser between a fundamental state Jf = l/2 and an excited state Je = 3/2). This potential is corrected by an attractive Van der Waals term which varies as 1/z3 in the Lennard‐Jones approximation (typical atomic distance of the order of λ0/2π where λ0 is the laser wavelength) and in 1/z4 if the distance between the atom and its image in the dielectric is big in front of λ0/2π. This last case is obtained in a quantum electrodynamic calculation by taking into account an orthornormal base [2]. We’ll examine the role of spontaneous emission for which the rate is inversely proportional to the detuning δ and is responsible of the non specular aspect of the atomic reflection (atomic diffusion). In the contrary, we note that the specularity of the reflection preserve the coherence of the atomic wave packet. The atoms will constitute a probe of the rugosity of the prism surface which can be imperfect or super‐polished.
The London-van der Waals potential experienced by an atom under reflection from an atomic mirror is modeled as a quantum dipole-dipole interaction between the atomic dipole induced by the evanescent wave and its image dipole in the dielectric mirror. The quantum dipole-dipole interaction arises from the combined effect of the evanescent field and spontaneous emission. It depends on the electronic structure of the atom and is described by an effective non-Hermitian Hamiltonian that yields dissipative effects under reflection. The analytical expression obtained here preserves the power-law dependence of the static van der Waals interaction at distances close to the wall, but its long-distance behavior reflects that of the evanescent wave.