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Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE

Robust control of quantum systems and in the presence of field fluctuations

HERSCHEL A. RABITZ

Published May 9, 2003• 0 citations
Publisher

Abstract

The impact of control field fluctuations on the optimal manipulation of quantum dynamics phenomena is investigated. The presence of significant field fluctuations is shown to break down the evolution into a sequence of partially coherent robust steps. Robustness occurs because the optimization process reduces sensitivity to noise-driven quantum system fluctuations. This process takes advantage of the observable expectation value being bilinear in the evolution operator and its adjoint. The consequences of this inherent robustness bodes well for the future success of closed loop quantum optimal control experiments.

DOI
10.1117/12.498522

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The impact of control field fluctuations on the optimal manipulation of quantum dynamics phenomena is investigated. The presence of significant field fluctuations is shown to break down the evolution into a sequence of partially coherent robust steps. Robustness occurs because the optimization process reduces sensitivity to noise-driven quantum system fluctuations. This process takes advantage of the observable expectation value being bilinear in the evolution operator and its adjoint. The consequences of this inherent robustness bodes well for the future success of closed loop quantum optimal control experiments.
The impact of control field fluctuations on the optimal manipulation of quantum dynamics phenomena is investigated. The quantum system is driven by an optimal control field, with the physical focus on the evolving expectation value of an observable operator. A relationship is shown to exist between the system dynamics and the control field fluctuations, wherein the process of seeking optimal performance assures an inherent degree of system robustness to such fluctuations. The presence of significant field fluctuations breaks down the evolution of the observable expectation value into a sequence of partially coherent robust steps. Robustness occurs because the optimization process reduces sensitivity to noise-driven quantum system fluctuations by taking advantage of the observable expectation value being bilinear in the evolution operator and its adjoint. The consequences of this inherent robustness are discussed in the light of recent experiments and numerical simulations on the optimal control of quantum phenomena. The analysis in this paper bodes well for the future success of closed-loop quantum optimal control experiments, even in the presence of reasonable levels of field fluctuations.
A relationship is shown to exist between optimally controlled quantum dynamics and field fluctuations, wherein the process of seeking optimal performance assures an inherent degree of system robustness to such fluctuations. Robustness occurs because the optimization process reduces sensitivity to noise-driven quantum system fluctuations by taking advantage of the observable expectation value being bilinear in the evolution operator and its adjoint. The consequences of this inherent robustness are discussed in light of recent experiments and numerical simulations on optimal control of quantum phenomena.
Abstract In recent work, we introduced the asymptotic theory of quantum robust control, which enables control of moments of quantum observables and gates in the presence of Hamiltonian uncertainty or field noise. In this paper, we extend this theory of quantum robust control to encompass two of the most important generalizations: robust control of arbitrary quantum observables and robust control of quantum systems sustaining environmental decoherence. In addition, we present deterministic Pareto optimization algorithms that can be applied in conjunction with either asymptotic or leading order measures of robustness. This enables robust control of any observable in quantum systems with any initial density matrix, and for which the entropy can change arbitrarily during the time evolution. Methods for robust optimal control of open quantum systems are presented that maximize the expected value of a quantum control objective while minimizing the expected environmentally induced decoherence.
This paper investigates the impact of control field noise on the optimal manipulation of quantum dynamics. Simulations are performed on several multilevel quantum systems with the goal of population transfer in the presence of significant control noise. The noise enters as run-to-run variations in the control amplitude and phase with the observation being an ensemble average over many runs as is commonly done in the laboratory. A genetic algorithm with an improved elitism operator is used to find the optimal field that either fights against or cooperates with control field noise. When seeking a high control yield it is possible to find fields that successfully fight with the noise while attaining good quality stable results. When seeking modest control yields, fields can be found which are optimally shaped to cooperate with the noise and thereby drive the dynamics more efficiently. In general, noise reduces the coherence of the dynamics, but the results indicate that population transfer objectives can be met by appropriately either fighting or cooperating with noise, even when it is intense.
Advances in quantum control theory and optimization techniques have made possible a new phenomena of quantum engineering. Chemical reactions can now be dynamically manipulated using first-principles quantum chemical models, in which a laser field, rather than a catalyst, serve as photonic reagents to selectively break a chemical bond and yield products via intramolecular rearrangement. A field pulse may also be designed to perform ultrasensitive spectroscopy, where compounds with very similar chemical properties are differentiated through their unique interaction with resonant and off-resonant photons. Despite significant progress in theoretical and laboratory quantum control, however, quantum engineering remains principally challenging due to manifestation of noise and uncertainties associated with the input and system parameters. Specifically, a small magnitude of variation in the field and Hamiltonian parameters would cause an otherwise optimal field to deviate from controlling desired quantum state transitions and reaching a particular objective. Thus, an accurate analysis of robustness of controlled quantum dynamics followed by a robust control framework is essential in achieving quantum control in a practical setting. In this work, theoretical foundations for quantum control robustness analysis are presented from both a distributional perspective - in terms of moments of the transition amplitude, interferences, and transition probability - and a worst-case perspective. In addition, an evolutionary control strategy for achieving robust control via open- and closed-loop approach are described with its mechanism of convergence elucidated using the robustness analysis method.
Optimal control operates in the presence of noise. Enhancement of the signal to noise ratio through optimized control is demonstrated for two condensed phase systems: the concept was demonstrated for second harmonic generation (SHG) in a nonlinear optical crystal and stimulated emission pumping (SEP) in a dye solution. Management of inherent control noise in the manipulation of quantum system is a subject of basic concern in virtually all applications of manipulating quantum dynamics phenomena. The cases of SHG and SEP in this work serve as illustrations of this capability. For control lasers operating at a kHz repetition rate, readily available electronics can handle this data stream.