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Physical Review Letters

Bichromatic laser cooling in a three-level system

R. Gupta, Changjian Xie, Sebastião Pádua, Herman Batelaan, H. Metcalf

Published Nov 8, 1993• 50 citations
Publisher

Abstract

We report a 1D study of optical forces on atoms in a two-frequency laser field. The light couples two ground state hyperfine structure levels to a common excited state of $^{85}\mathrm{Rb}$, thus forming a \ensuremath{\Lambda} system. We observe a new type of sub-Doppler coupling with blue-tuned light that uses neither polarization gradients nor magnetic fields, efficient heating with red tuning, and the spatial phase dependence of these. We observed deflection from a rectified dipole force and determined its velocity dependence and capture range. We report velocity selective resonances associated with Raman transitions. A simplified semiclassical calculation agrees qualitatively with our measurements.

DOI
10.1103/physrevlett.71.3087

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We report a 1D study of optical forces on atoms in a two-frequency laser field. The light couples two ground state hyperfine structure levels to a common excited state of 85Rb^{85}\mathrm{Rb}85Rb, thus forming a \ensuremath{\Lambda} system. We observe a new type of sub-Doppler coupling with blue-tuned light that uses neither polarization gradients nor magnetic fields, efficient heating with red tuning, and the spatial phase dependence of these. We observed deflection from a rectified dipole force and determined its velocity dependence and capture range. We report velocity selective resonances associated with Raman transitions. A simplified semiclassical calculation agrees qualitatively with our measurements.
We have observed a new type of sub-Doppler laser cooling with neither polarization gradients nor magnetic fields. All known sub-Doppler laser cooling methods require one of these two to resdistribute the atomic population among the energy levels. This allows the irreversible processes of optical pumping vels. This allows the irreversible processes of optical pumping (OP) to manipulate the conservative force of light shifts (e.g. resonant exchange between the two beams comprising a standing wave) into a damping force. Our scheme employs stimulated Raman transitions between ground state hyperfine levels of Rb with a bichromatic standing wave, accompanied by a momentum change of {Delta}p = 2{h_bar}k. OP, with {Delta}p = 1{h_bar}k, creates a population imbalance allowing repetition of the Raman process. When the detuning of the light from Raman resonance {delta} is properly chosen, the net momentum exchange damps the atomic motion. Changing {delta} by only {gamma}/6(1 MHz) replaces cooling by heating. This process separates the velocity selective Raman resonance and OP processes differently from others, and helps clarify the role of these different mechanisms.
We study the laser cooling process in a complex lambda system in the presence of force-assisted bichromatic velocity-selective coherent population trapping. Our theoretical model includes atomic transitions based on two ground states, Fg=1 and Fg′=3, and one excited state, Fe=2, excited by a bichromatic laser field tuned in resonance with the Fg=1→Fe=2 and Fg′=3→Fe=2 transitions. The analyzed optical scheme may be useful for alternative transverse cooling in experiments with group III atoms (Al, Ga, In).
Following the bichromatic sub-Doppler cooling scheme on the D1-line of 40K recently demonstrated in (Fernandes et al. 2012), we introduce a similar technique for 7Li atoms and obtain temperatures of 60 uK while capturing all of the 5x10^8 atoms present from the previous stage. We investigate the influence of the detuning between the the two cooling frequencies and observe a threefold decrease of the temperature when the Raman condition is fulfilled. We interpret this effect as arising from extra cooling due to long-lived coherences between hyperfine states. Solving the optical Bloch equations for a simplified, \Lambda-type three-level system we identify the presence of an efficient cooling force near the Raman condition. After transfer into a quadrupole magnetic trap, we measure a phase space density of ~10^-5. This laser cooling offers a promising route for fast evaporation of lithium atoms to quantum degeneracy in optical or magnetic traps.
We examine the laser cooling of three-level (Lambda) -atoms in the field of two standing waves when frequency detunings are considerably greater than natural width of the excited state as well as the Rabi frequencies in the system. It is shown that at the difference of frequency detunings is small when compared to the Rabi frequencies sub-Doppler cooling of the (Lambda) -atom is possible. We present the dependence of the light pressure force on the atoms velocity and dependence of cooled atoms temperature on the parameters of the exciting waves.
We describe several one-dimensional sub-Doppler laser-cooling experiments that cool Rb to finite and zero velocities in a magnetic field and polarization gradients. We then present a physical picture that unifies these measurements in terms of coherent two-photon velocity-selective resonances between atomic ground-state sublevels (including Raman resonances). We propose several sub-Doppler cooling schemes without fields or without polarization gradients, based on VSR between nondegenerate ground states.
A subharmonic resonance occurs on irradiation of a three-level (\ensuremath{\Lambda}) system by two bichromatic fields when an integer multiple of the common frequency difference matches the Raman detuning between the two lower levels. The occurrence of these multiphoton resonances requires saturation of the Raman transition. The three-level model is applied in order to understand recent experimental studies of subharmonic Raman resonances between vibrational states of optically trapped atoms. I explain the difference between these resonances and the well-known velocity-tuned (Doppleron) resonances in two-level atoms by considering a two-state model with the excited state eliminated. I finally point out a Sisyphus cooling mechanism that is entirely dependent on an additional relaxation of the Raman coherence, comparable to collision-induced resonances.