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Physical Review A

Low-light-level cross-phase modulation by quantum interference

Hsiang-Yu Lo, Po-Ching Su, Yong‐Fan Chen

Published May 18, 2010• 39 citations
Publisher

Abstract

We report on the direct measurement of low-light-level cross-phase modulation (XPM) based on electromagnetically induced transparency (EIT) in the pulsed regime. A phase shift of 0.02 rad of a probe pulse modulated by a signal pulse with a peak intensity of 3 $\mathrm{\ensuremath{\mu}}\mathrm{W}/{\mathrm{cm}}^{2}$ was observed, which is the lowest intensity ever achieved for the N-type EIT-based XPM system. The experimental data make a quantitative prediction of the single-photon-level XPM phase shift arising from two interacting pulses with unequal group velocities that is consistent with the theoretical predictions proposed by Harris and Hau [Phys. Rev. Lett. 82, 4611 (1999)]. Furthermore, a proof-of-principle experiment demonstrating an enhancement of the nonlinear optical Kerr effect by shining the signal pulse twice is presented.

DOI
10.1103/physreva.81.053829

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We report on the first experimental demonstration of low-light-level cross-phase modulation (XPM) with double slow light pulses based on the double electromagnetically induced transparency (EIT) in cold cesium atoms. The double EIT is implemented with two control fields and two weak fields that drive populations prepared in the two doubly spin-polarized states. Group velocity matching can be obtained by tuning the intensity of either of the control fields. The XPM is based on the asymmetric M-type five-level system formed by the two sets of EIT. Enhancement in the XPM by group velocity matching is observed. Our work advances studies of low-light-level nonlinear optics based on double slow light pulses.
We investigate, both theoretically and experimentally, the cross-Kerr nonlinearity generated in a four-level tripod system in the 87Rb D1 line. The system exhibits simultaneous electromagnetically induced transparency (EIT) windows for two weak (probe and trigger) fields and the enhanced cross-Kerr nonlinearity by EIT. The cross-Kerr nonlinear phase shifts for probe (trigger) field are measured at several different intensities of trigger (probe) field. The results show that large cross-phase modulation (XPM) coefficients can be achieved at low light intensities.
We experimentally demonstrate a low-light-level cross-phase-modulation (XPM) scheme based on the light-storage technique in laser-cooled 87Rb atoms. The proposed scheme can achieve a similar phase shift and has the same figure of merit as one using static electromagnetically induced transparency under the constant coupling field. Nevertheless, the phase shift and the energy loss of a probe pulse induced by a signal pulse are neither influenced by the coupling intensity nor by the atomic optical density in the light-storage XPM scheme. This scheme enhances the flexibility of the experiment and makes possible conditional phase shifts on the order of pi with single photons.
In third order nonlinear mediums, the intensity of one optical field can modify the phase of another optical field. This is known as cross-phase modulation (XPM) and is important for Quantum Information Processing (QIP) as phase shifts of single-photons that exceed π rad can be used to implement two-qubit quantum logic gates. For a conventional XPM scheme, the Kerr nonlinearity responsible for XPM is too small for appreciable phase shifts to be achieved with low intensity optical fields. However, Electromagnetically Induced Transparency (EIT) can increase this nonlinearity by several orders of magnitude. This thesis discusses the experimental construction of a laser-atomic system capable of EIT modulated XPM. This includes construction of a rubidium magneto-optical trap (RbMOT), characterization of this RbMOT, demonstration of EIT in the RbMOT, and a system capable of detecting optical phase shifts produced by EIT. The talk will conclude with an outlook on further implementations to the experiment that will increase this nonlinearity such that phase shifts at the single-photon level are possible. | 76 pages
A four-level inverted-Y scheme with an electromagnetically induced transparency (EIT) core is investigated for the enhancement of cross-Kerr effect in rubidium atoms. When detunings of the coupling and control fields are appropriately set, an enhanced EIT window is observed, and the induced phase shift of the probe field due to cross-phase modulation (XPM) is obtained by measuring the dispersive property of the probe transition. The maximal XPM phase shift is about 12° under the current experimental conditions. The experimental measurements agree well with the theoretical calculations. The enhanced XPM phase shift in such an atomic system has applications in quantum nonlinear optics and quantum information science.
We report experimental observations on the simultaneous electromagnetically induced transparency (EIT) effects for probe and trigger fields (double EIT) as well as the enhanced cross-phase modulation (XPM) between the two fields in a four-level tripod EIT system of the D1 line of 87Rb atoms. The XPM coefficients (larger than 2 x 10(-5) cm2/W) and the accompanying transmissions (higher than 60%) are measured at a slight detuning of the probe field from the exact EIT-resonance condition. The system and enhanced cross-Kerr nonlinearities presented here can be applied to quantum information processes.