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Physical Review A

Quenching of spontaneous emission via quantum interference

Hwang Lee, Pavel G. Polynkin, Marlan O. Scully, Shi-Yao Zhu

Published Jun 1, 1997• 168 citations
Publisher

Abstract

A four-level atom, driven by a coherent field, is considered. We show that under certain conditions complete quenching of spontaneous emission is possible. Hence the population inversion on some specific atomic transitions can be created using a very weak incoherent pumping. We investigate the physics of the effect using bare and dressed states. The proposed scheme may be useful, in principle, for generation of high-frequency and/or high power laser light.

DOI
10.1103/physreva.55.4454

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A four-level atom, driven by a coherent field, is considered. We show that under certain conditions complete quenching of spontaneous emission is possible. Hence the population inversion on some specific atomic transitions can be created using a very weak incoherent pumping. We investigate the physics of the effect using bare and dressed states. The proposed scheme may be useful, in principle, for generation of high-frequency and/or high power laser light.
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Quantum interference in a decaying three-level system of V type with degenerate upper levels driven by a single incoherent field is shown to lead to a coherent population-trapping state and more generally to a population-locked state. The latter is a state with half the population locked in two upper states regardless of the strength of incoherent pumping and decay rates. We reveal the mechanism by which half the population is pumped to the upper states no matter how weak is the incoherent pumping. Transient regimes of gain without inversion and inversion without gain are demonstrated. Quenching of spontaneous emission due to electron collisions is also discussed in support of the experiments and ideas of Suckewer and [Phys. Rev. Lett. 60, 1122 (1988)].
We study the spontaneous-emission properties of a coherently driven four-level atom, and show a few interesting phenomena such as fluorescence quenching, spectral-line narrowing, spectral-line enhancement, and spectral-line elimination. These phenomena can be observed in experiment since the rigorous condition of near-degenerate levels with nonorthogonal dipole moments is not required here. Qualitatively, these phenomena can be attributed to the quantum interference between competitive spontaneous-decay channels in the bare-state picture or the spontaneously generated coherence between two close-lying levels in the dressed-state picture.
The emergence of laser action from an atomic system without population inversion is beginning to attract theoretical and experimental attention as a possible way of generating useful coherent radiation at unusual wavelengths. The goal of this communication is to clarify the physical origin of this phenomenon using a four-level system whose ground state consists of two quasidegenerate levels that are coupled to a higher-lying state by a Raman-like transition. In the presence of the ground-state coherence induced by the Raman field, we calculate the absorption spectrum of a weak probe whose tunable frequency scans across the transition frequencies between the two ground-state levels and another higher-lying state that may or may not be weakly excited by an incoherent pump mechanism. Our calculation, based on a dressed atomic state approach, clarifies the conditions that must be satisfied to produce gain, identifies the frequency (or frequencies) at which the gain is maximum, and elucidates the functions of the incoherent pump, the Raman field, and the coherence between the ground-state levels in this process. An appropriate set of Maxwell- Bloch equations for a ring-cavity model of this system confirms the appearance of laser action when the small-signal gain conditions are satisfied.
We study the spontaneous emission property of a four-level atomic system driven by two coherent fields. By numerical calculations in the bare state picture, we show that such interesting phenomena as extremely narrow peaks and spontaneous emission quenching can be realized, which are well understood by qualitative explanations in the partially and fully dressed state pictures. Especially, this coherently driven atomic system has two close-lying levels in the partially dressed state picture so that spontaneously generated coherence arises. Using our considered scheme it is feasible to carry out experiments based on spontaneously generated coherence because all rigorous requirements have been avoided in the bare state picture.