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Journal of Physics Conference Series

Dynamical properties of spatially anisotropic frustrated Heisenberg models in a magnetic field

Masanori Kohno, Leon Balents, Oleg A. Starykh

Published Jan 1, 2009• 5 citations
Publisher

Abstract

We investigate spectral features of spatially anisotropic spin-1/2 frustrated antiferromagnets in a magnetic field by a weak-coupling approach from the one-dimensional (1D) limit. Using exact results of the Heisenberg chain, we calculate dynamical structure factors of spatially anisotropic frustrated antiferromagnets in two dimensions. We obtain rich peak structures depending on the momentum and the strength of magnetic fields. We identify the sharp peaks as bound and antibound states between particles carrying fractional Sz in 1D in a magnetic field, psinons and antipsinons, and those originating from 2-string solutions. We compare these spectral features with available experimental results on Cs2CuCl4, and suggest that the dynamical properties of Cs2CuCl4 in a magnetic field can be interpreted in terms of particles in 1D in a magnetic field.

DOI
10.1088/1742-6596/145/1/012062

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We investigate spectral features of spatially anisotropic spin-1/2 frustrated antiferromagnets in a magnetic field by a weak-coupling approach from the one-dimensional (1D) limit. Using exact results of the Heisenberg chain, we calculate dynamical structure factors of spatially anisotropic frustrated antiferromagnets in two dimensions. We obtain rich peak structures depending on the momentum and the strength of magnetic fields. We identify the sharp peaks as bound and antibound states between particles carrying fractional Sz in 1D in a magnetic field, psinons and antipsinons, and those originating from 2-string solutions. We compare these spectral features with available experimental results on Cs2CuCl4, and suggest that the dynamical properties of Cs2CuCl4 in a magnetic field can be interpreted in terms of particles in 1D in a magnetic field.
We investigate spectral features of spatially anisotropic spin-1/2 frustrated antiferromagnets in a magnetic field by a weak-coupling approach from the one-dimensional (1D) limit. Using exact results of the Heisenberg chain, we calculate dynamical structure factors of spatially anisotropic frustrated antiferromagnets in two dimensions. We obtain rich peak structures depending on the momentum and the strength of magnetic fields. We identify the sharp peaks as bound and antibound states between particles carrying fractional Sz in 1D in a magnetic field, psinons and antipsinons, and those originating from 2-string solutions. We compare these spectral features with available experimental results on Cs2CuCl4, and suggest that the dynamical properties of Cs2CuCl4 in a magnetic field can be interpreted in terms of particles in 1D in a magnetic field.
Spectral properties of the spin-1/2 antiferromagnetic Heisenberg chain in a magnetic field are investigated by using exact Bethe-ansatz solutions. We argue that not only quasiparticles called psinon and antipsinon but also a quasiparticle representing a 2-string in the Bethe ansatz plays an important role for dynamical properties in a magnetic field. Combined with psinon and antipsinon, the quasiparticle for a 2-string forms a continuum in the high-energy regime for transverse dynamical structure factor S +− ( κ,ω ). In the zero-field limit, the continuum is located on the mode of the lowest excited states in zero field called the des Cloizeaux-Pearson mode. In a magnetic field, the continuum separates from other low-energy continua, and reduces to the mode of bound states of overturned spins from the fully polarized state near the saturation field. We confirm the relevance through comparisons with available experimental results on the quasi-one-dimensional antiferromagnet CuCl 2 ·2N(C 5 D 5 ).
Dynamical properties of frustrated XXZ models in the Ising limit on spatially anisotropic two-dimensional lattices are investigated by a weak-coupling approach from the one-dimensional limit. Restricting the Hilbert space to that spanned by exact eigenstates of XXZ chains in the Ising limit, we calculate dynamical structure factor 5 -+ (k,ω) in spatially anisotropic two-dimensional systems. As in the case of frustrated Heisenberg models [M.Kohno, et al. , Nat. Phys. 3, 790 (2007)], spinons form bound states through hopping process between chains. We calculate the density-density correlation function of spinons in the Ising limit, and show that spinons in the bound state hop together as a pair, although those in a continuous spectrum behave almost independently. We discuss possible implications of the present results on fractionalization of bosonic and fermionic particles in spatially anisotropic frustrated systems with strong repulsion.
The T=0T=0T=0 dynamical properties of the one-dimensional (1D) s=12s=\frac{1}{2}s=21​ Heisenberg antiferromagnet in a uniform magnetic field are studied via the Bethe ansatz for cyclic chains of N sites. The ground state at magnetization 0<Mz<N/2,0<{M}_{z}<N/2,0<Mz​<N/2, which can be interpreted as a state with 2Mz{2M}_{z}2Mz​ spinons or as a state of $N/2\ensuremath{-}{M}_{z}$ magnons, is reconfigured here as the vacuum for a different species of quasiparticles, the psinons and antipsinons. We investigate three kinds of quantum fluctuations, namely the spin fluctuations parallel and perpendicular to the direction of the applied magnetic field and the dimer fluctuations. The dynamically dominant excitation spectra are found to be sets of collective excitations composed of two quasiparticles excited from the psinon vacuum in different configurations. The Bethe ansatz provides a framework for (i) the characterization of the new quasiparticles in relation to the more familiar spinons and magnons, (ii) the calculation of spectral boundaries and densities of states for each continuum, (iii) the calculation of transition rates between the ground state and the dynamically dominant collective excitations, (iv) the prediction of line shapes for dynamic structure factors relevant for experiments performed on a variety of quasi-1D antiferromagnetic compounds, including KCuF3,{\mathrm{KCuF}}_{3},KCuF3​, Cu(C4H4N2)(NO3)2,\mathrm{Cu}({\mathrm{C}}_{4}{\mathrm{H}}_{4}{\mathrm{N}}_{2})({\mathrm{NO}}_{3}{)}_{2},Cu(C4​H4​N2​)(NO3​)2​, and CuGeO3.{\mathrm{CuGeO}}_{3}.CuGeO3​.
We study the dynamical response of frustrated, quasi-one-dimensional spin-1/2 Heisenberg antiferromagnets at finite temperatures. We allow for the presence of a Dzyaloshinskii-Moriya interaction. We concentrate on a model of weakly coupled planes of anisotropic triangular lattices. Combining exact results for the dynamical response of one-dimensional Heisenberg chains with a random-phase approximation in the frustrated interchain couplings, we calculate the dynamical susceptibility in the disordered phase. We investigate the instability of the disordered phase to the formation of collective modes. We find a very weak instability to the formation of incommensurate magnetic order and determine the ordering temperature and wave vector. We also determine the effects of uniform magnetic fields on the ordering transition.
We study the dynamical response of frustrated, quasi-one-dimensional spin-12\frac{1}{2}21​ Heisenberg antiferromagnets at finite temperatures. We allow for the presence of a Dzyaloshinskii-Moriya interaction. We concentrate on a model of weakly coupled planes of anisotropic triangular lattices. Combining exact results for the dynamical response of one-dimensional Heisenberg chains with a random-phase approximation in the frustrated interchain couplings, we calculate the dynamical susceptibility in the disordered phase. We investigate the instability of the disordered phase to the formation of collective modes. We find a very weak instability to the formation of incommensurate magnetic order and determine the ordering temperature and wave vector. We also determine the effects of uniform magnetic fields on the ordering transition.