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Journal of Experimental and Theoretical Physics

Quantum theory of resonant scattering of atoms by a pulsed field under coherent population trapping conditions

А. В. Тайченачев, Anatolii M Tumaikin, Valeriy I. Yudin

Published Jan 1, 1998• 1 citation
Publisher

Abstract

We develop an entirely quantum mechanical analytical description of scattering of atoms with angular momenta j g →j→j e =j (j is an integer) by a pulsed σ +−σ − field. In the stationary-atom approximation with exact accounting for recoil effects, we solve the problem of the change in the distribution of atoms among the internal and translational degrees of freedom initiated by a single pulse for j g =1, 2. We find in analytical form recurrence formulas that make it possible to calculate the distribution of the atoms after an arbitrary sequence of pulses has acted on the system. We show that for discrete (resonant) values of the time interval between the pulses, the action of N pulses leads to effective formation and narrowing of peaks at discrete points in momentum space and to a broadening of the envelope of these peaks. In the case of a broad initial momentum distribution we derive explicit formulas for the peaks and the envelope and study their asymptotic behavior for N≫1. Finally, in the weak-field limit we study numerically the dependence of the contrast of the scattering diagram on pulse length.

DOI
10.1134/1.558468

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We develop an entirely quantum mechanical analytical description of scattering of atoms with angular momenta j g →j→j e =j (j is an integer) by a pulsed σ +−σ − field. In the stationary-atom approximation with exact accounting for recoil effects, we solve the problem of the change in the distribution of atoms among the internal and translational degrees of freedom initiated by a single pulse for j g =1, 2. We find in analytical form recurrence formulas that make it possible to calculate the distribution of the atoms after an arbitrary sequence of pulses has acted on the system. We show that for discrete (resonant) values of the time interval between the pulses, the action of N pulses leads to effective formation and narrowing of peaks at discrete points in momentum space and to a broadening of the envelope of these peaks. In the case of a broad initial momentum distribution we derive explicit formulas for the peaks and the envelope and study their asymptotic behavior for N≫1. Finally, in the weak-field limit we study numerically the dependence of the contrast of the scattering diagram on pulse length.
A completely quantum-analytical description of the cooling of atoms with angular momenta j g =1→j e =1 by a pulsed σ 1−σ − field is developed. The problem of the change produced in the distribution of the atoms over the internal and translational degrees of freedom by a single field pulse is solved exactly with respect to recoil effects. Recurrence formulas for the distribution after the action of an arbitrary sequence of pulses are found in analytical form. It is shown that N field pulses result in the formation and narrowing of peaks at discrete points in momentum space as well as broadening of the envelope of these peaks. Explicit formulas are obtained for the peaks and envelopes in the case of a wide initial momentum distribution, and their asymptotic behavior for N≫1 is investigated.
A quantum analytic treatment of the resonant scattering of atoms with jg equals j yields je equals j (j is an integer) transitions by a pulsed (sigma) + - (sigma) - field is developed. In the approximation of motionless atoms, the atomic density matrix after action of single light pulse is evaluated with exact consideration of the recoil effects. Recurrent equations, which allow to calculate the distribution after arbitrary pulse sequences are found in the analytic form. It is shown that for discrete pulse frequencies the action of N light pulses leads to the formation and narrowing of peaks in discrete points of the momentum space, and also to the broadening of the envelope of the momentum distribution. In the case of the wide (with respect to the photon momentum) initial distribution the explicit formulae for peaks and envelope are obtained and an asymptotic behavior of the solution is analyzed. In the low-intensity limit a dependence of the scattering pattern contrast on the pulse duration is studied.
A nonperturbative analysis is given for an nnn-level atom or molecule dressed by a Stark field and in single-photon or multiphoton (near) resonant interaction with coherent optical field modes, which may be intense. All the field amplitudes and phases may have nonadiabatic time variation. New formulas for probability amplitudes of states with finite lifetimes are given for atom-field levels swept or optical Stark shifted through resonance or into close approach. One of these includes the Landau-Zener formula as a special case. Power broadening is contained in these formulas. They are useful for both weak- and strong-field interaction. Further, it is shown that many familiar single-photon coherent transient phenomena have their analogs in the intense-field and the multiphoton domains. Two new effects, pulse-shape dependence in final transition probability and population inversion due to the nonadiabatic passage of an asymmetric pulse, are demonstrated with numerical results for the process $\mathrm{Na}(3s)+2\ensuremath{\hbar}\ensuremath{\omega}\ensuremath{\rightarrow}\mathrm{Na}(5s)$. Finally, double resonance (single-photon and/or multiphoton) is analyzed, with discussion of adiabatic following and a derivation of a formula for level crossing. Generalization of an earlier procedure for solving the adiabatic eigenvalue problem of the whole atom-field system is given.
Coherent backscattering of pulsed radiation emitted by optically dense atomic ensembles is considered. The diagrammatic technique is used for deriving analytic expressions for correlation functions of scattered light, which make it possible to take into account all main factors affecting the dynamics of the process, including the hyperfine and Zeeman structure of the ground and first excited states of atoms, polarization of probe radiation, the actual shape and size of an atomic cloud, its spatial inhomogeneity, motion of atoms, and angular-momentum polarization of atoms. On the basis of these relations, the time dependence of the total intensity and the dependence of enhancement factor of backscattered light on the pulse duration, type of polarization of the polarization system of observation, optical thickness of the scattering medium, and the carrier frequency of the pulse are investigated. The calculations are performed for an ensemble of rubidium-85 atoms cooled in magnetooptical traps.
A quantum theory of stimulated Raman scattering is established that takes into account the time-dependence of pump laser pulse, two-photon detuning and atomic populations, allowing the general transient and spatial propagation study of Raman memory. Heisenberg–Langevin and Maxwell equations for the collective atomic operators are solved analytically under adiabatic condition , where the electric field envelopes and the collective atomic operators vary slowly. The analytical solution of Stokes/anti-Stokes signal electric field operator is obtained. The spatial–temporal intensity of quantum signal field is studied numerically and analytically for different two-photon detunings and initial populations.
An analytical theory of optical pumping of velocity-selective coherent population trapping states in three-level Λ-atoms is presented. The theory is based on an atomic density matrix in the superpositional state representation. The representation introduced for the atomic density matrix directly describes coherent population trapping (CPT) states in a three-level Λ-atom and yields an approximate analytical description for the shape of the two-peak momentum (velocity) distribution of atoms. Optical pumping of velocity-selective CPT states is described in the superpositional state representation as a process of redistribution of atoms in the region of small velocities due to the photon recoil. Typical times of formation of velocity-selective CPT states are found to be inversely proportional to the square of the recoil energy.